Thermoelectric performance of PbSnTeSe high-entropy alloys

In our study, we designed the PbSnTeSe high-entropy alloy (HEA) and investigated its microstructure and thermoelectric properties. It was found that the PbSnTeSe HEA has a simple face-centered cubic structure and possesses quite low lattice thermal conductivity at low temperatures, which could be as...

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Main Authors: Zhao Fan, Hui Wang, Yuan Wu, Xiongjun Liu, Zhaoping Lu
Format: Article
Language:English
Published: Taylor & Francis Group 2017-05-01
Series:Materials Research Letters
Subjects:
Online Access:http://dx.doi.org/10.1080/21663831.2016.1244116
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author Zhao Fan
Hui Wang
Yuan Wu
Xiongjun Liu
Zhaoping Lu
author_facet Zhao Fan
Hui Wang
Yuan Wu
Xiongjun Liu
Zhaoping Lu
author_sort Zhao Fan
collection DOAJ
description In our study, we designed the PbSnTeSe high-entropy alloy (HEA) and investigated its microstructure and thermoelectric properties. It was found that the PbSnTeSe HEA has a simple face-centered cubic structure and possesses quite low lattice thermal conductivity at low temperatures, which could be ascribed to the strong phonon scattering due to its severe lattice-distortion. Minor additions of La not only enhanced both Seebeck coefficient and electrical conductivity at high temperatures, but also suppressed the bipolar effect to some degree. Our results indicate that the HEA concept could be applied for developing promising thermoelectric materials, which merits further investigation.
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spelling doaj.art-e603339513bc48eab9befe6bc84d68a42022-12-22T00:08:40ZengTaylor & Francis GroupMaterials Research Letters2166-38312017-05-015318719410.1080/21663831.2016.12441161244116Thermoelectric performance of PbSnTeSe high-entropy alloysZhao Fan0Hui Wang1Yuan Wu2Xiongjun Liu3Zhaoping Lu4University of Science and Technology BeijingUniversity of Science and Technology BeijingUniversity of Science and Technology BeijingUniversity of Science and Technology BeijingUniversity of Science and Technology BeijingIn our study, we designed the PbSnTeSe high-entropy alloy (HEA) and investigated its microstructure and thermoelectric properties. It was found that the PbSnTeSe HEA has a simple face-centered cubic structure and possesses quite low lattice thermal conductivity at low temperatures, which could be ascribed to the strong phonon scattering due to its severe lattice-distortion. Minor additions of La not only enhanced both Seebeck coefficient and electrical conductivity at high temperatures, but also suppressed the bipolar effect to some degree. Our results indicate that the HEA concept could be applied for developing promising thermoelectric materials, which merits further investigation.http://dx.doi.org/10.1080/21663831.2016.1244116High-entropy alloysthermoelectriclow thermal conductivity
spellingShingle Zhao Fan
Hui Wang
Yuan Wu
Xiongjun Liu
Zhaoping Lu
Thermoelectric performance of PbSnTeSe high-entropy alloys
Materials Research Letters
High-entropy alloys
thermoelectric
low thermal conductivity
title Thermoelectric performance of PbSnTeSe high-entropy alloys
title_full Thermoelectric performance of PbSnTeSe high-entropy alloys
title_fullStr Thermoelectric performance of PbSnTeSe high-entropy alloys
title_full_unstemmed Thermoelectric performance of PbSnTeSe high-entropy alloys
title_short Thermoelectric performance of PbSnTeSe high-entropy alloys
title_sort thermoelectric performance of pbsntese high entropy alloys
topic High-entropy alloys
thermoelectric
low thermal conductivity
url http://dx.doi.org/10.1080/21663831.2016.1244116
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AT huiwang thermoelectricperformanceofpbsntesehighentropyalloys
AT yuanwu thermoelectricperformanceofpbsntesehighentropyalloys
AT xiongjunliu thermoelectricperformanceofpbsntesehighentropyalloys
AT zhaopinglu thermoelectricperformanceofpbsntesehighentropyalloys