A Method for Identification and Assessment of Radioxenon Plumes by Absorption in Polycarbonates

A method for the retrospective evaluation of the integrated activity concentration of <sup>133</sup>Xe during radioxenon plumes and the moment of the plume’s center is proposed and explored by computer modeling. The concept is to use a specimen of polycarbonate material (a stack of Makro...

Full description

Bibliographic Details
Main Authors: Dobromir Pressyanov, Pavel Stavrev
Format: Article
Language:English
Published: MDPI AG 2021-12-01
Series:Sensors
Subjects:
Online Access:https://www.mdpi.com/1424-8220/21/23/8107
_version_ 1797507179577606144
author Dobromir Pressyanov
Pavel Stavrev
author_facet Dobromir Pressyanov
Pavel Stavrev
author_sort Dobromir Pressyanov
collection DOAJ
description A method for the retrospective evaluation of the integrated activity concentration of <sup>133</sup>Xe during radioxenon plumes and the moment of the plume’s center is proposed and explored by computer modeling. The concept is to use a specimen of polycarbonate material (a stack of Makrofol N foils of thickness 120 µm and 40 µm in 1 L non-hermetic Marinelly beaker) that is placed in the environment or in a controlled nuclear or radiopharmaceutical facility. On a regular basis or incidentally, the specimen may be retrieved and gamma spectrometry in two consecutive time intervals with durations of 8 h and 16 h is performed. To assess the performance of the method, <sup>133</sup>Xe plumes of various integrated activity concentrations and with a duration of up to 10 h are simulated and analyzed, assuming that the measurement starts with a delay of up to one day after the moment of the plume center. It is found that the deviation between the estimates by the method and their true values are within a few percent. Depending on the delay, events of integrated <sup>133</sup>Xe activity concentration 250–1000 Bq h m<sup>−3</sup> might be qualitatively identified. At levels >10,000 Bq h m<sup>−3</sup>, the uncertainty of the quantitative estimates might be ≤10%.
first_indexed 2024-03-10T04:44:57Z
format Article
id doaj.art-e7156bf741b4458693cf1593ba55145c
institution Directory Open Access Journal
issn 1424-8220
language English
last_indexed 2024-03-10T04:44:57Z
publishDate 2021-12-01
publisher MDPI AG
record_format Article
series Sensors
spelling doaj.art-e7156bf741b4458693cf1593ba55145c2023-11-23T03:04:05ZengMDPI AGSensors1424-82202021-12-012123810710.3390/s21238107A Method for Identification and Assessment of Radioxenon Plumes by Absorption in PolycarbonatesDobromir Pressyanov0Pavel Stavrev1Faculty of Physics, University of Sofia “St. Kliment Ohridski”, 5 James Bourchier Blvd., 1164 Sofia, BulgariaFaculty of Physics, University of Sofia “St. Kliment Ohridski”, 5 James Bourchier Blvd., 1164 Sofia, BulgariaA method for the retrospective evaluation of the integrated activity concentration of <sup>133</sup>Xe during radioxenon plumes and the moment of the plume’s center is proposed and explored by computer modeling. The concept is to use a specimen of polycarbonate material (a stack of Makrofol N foils of thickness 120 µm and 40 µm in 1 L non-hermetic Marinelly beaker) that is placed in the environment or in a controlled nuclear or radiopharmaceutical facility. On a regular basis or incidentally, the specimen may be retrieved and gamma spectrometry in two consecutive time intervals with durations of 8 h and 16 h is performed. To assess the performance of the method, <sup>133</sup>Xe plumes of various integrated activity concentrations and with a duration of up to 10 h are simulated and analyzed, assuming that the measurement starts with a delay of up to one day after the moment of the plume center. It is found that the deviation between the estimates by the method and their true values are within a few percent. Depending on the delay, events of integrated <sup>133</sup>Xe activity concentration 250–1000 Bq h m<sup>−3</sup> might be qualitatively identified. At levels >10,000 Bq h m<sup>−3</sup>, the uncertainty of the quantitative estimates might be ≤10%.https://www.mdpi.com/1424-8220/21/23/8107radioxenon plumes<sup>133</sup>Xeabsorption in polycarbonatesMakrofolretrospective estimatesnuclear accidents
spellingShingle Dobromir Pressyanov
Pavel Stavrev
A Method for Identification and Assessment of Radioxenon Plumes by Absorption in Polycarbonates
Sensors
radioxenon plumes
<sup>133</sup>Xe
absorption in polycarbonates
Makrofol
retrospective estimates
nuclear accidents
title A Method for Identification and Assessment of Radioxenon Plumes by Absorption in Polycarbonates
title_full A Method for Identification and Assessment of Radioxenon Plumes by Absorption in Polycarbonates
title_fullStr A Method for Identification and Assessment of Radioxenon Plumes by Absorption in Polycarbonates
title_full_unstemmed A Method for Identification and Assessment of Radioxenon Plumes by Absorption in Polycarbonates
title_short A Method for Identification and Assessment of Radioxenon Plumes by Absorption in Polycarbonates
title_sort method for identification and assessment of radioxenon plumes by absorption in polycarbonates
topic radioxenon plumes
<sup>133</sup>Xe
absorption in polycarbonates
Makrofol
retrospective estimates
nuclear accidents
url https://www.mdpi.com/1424-8220/21/23/8107
work_keys_str_mv AT dobromirpressyanov amethodforidentificationandassessmentofradioxenonplumesbyabsorptioninpolycarbonates
AT pavelstavrev amethodforidentificationandassessmentofradioxenonplumesbyabsorptioninpolycarbonates
AT dobromirpressyanov methodforidentificationandassessmentofradioxenonplumesbyabsorptioninpolycarbonates
AT pavelstavrev methodforidentificationandassessmentofradioxenonplumesbyabsorptioninpolycarbonates