Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer
Abstract Planar perovskite solar cells using low‐temperature atomic layer deposition (ALD) of the SnO2 electron transporting layer (ETL), with excellent electron extraction and hole‐blocking ability, offer significant advantages compared with high‐temperature deposition methods. The optical, chemica...
| Main Authors: | , , , , , , , , , , , , |
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| Format: | Article |
| Language: | English |
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Wiley
2018-06-01
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| Series: | Advanced Science |
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| Online Access: | https://doi.org/10.1002/advs.201800130 |
| _version_ | 1797754272227524608 |
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| author | Yonghui Lee Seunghwan Lee Gabseok Seo Sanghyun Paek Kyung Taek Cho Aron J. Huckaba Marco Calizzi Dong‐won Choi Jin‐Seong Park Dongwook Lee Hyo Joong Lee Abdullah M. Asiri Mohammad Khaja Nazeeruddin |
| author_facet | Yonghui Lee Seunghwan Lee Gabseok Seo Sanghyun Paek Kyung Taek Cho Aron J. Huckaba Marco Calizzi Dong‐won Choi Jin‐Seong Park Dongwook Lee Hyo Joong Lee Abdullah M. Asiri Mohammad Khaja Nazeeruddin |
| author_sort | Yonghui Lee |
| collection | DOAJ |
| description | Abstract Planar perovskite solar cells using low‐temperature atomic layer deposition (ALD) of the SnO2 electron transporting layer (ETL), with excellent electron extraction and hole‐blocking ability, offer significant advantages compared with high‐temperature deposition methods. The optical, chemical, and electrical properties of the ALD SnO2 layer and its influence on the device performance are investigated. It is found that surface passivation of SnO2 is essential to reduce charge recombination at the perovskite and ETL interface and show that the fabricated planar perovskite solar cells exhibit high reproducibility, stability, and power conversion efficiency of 20%. |
| first_indexed | 2024-03-12T17:30:07Z |
| format | Article |
| id | doaj.art-e865dff216b74995966da1b5537171af |
| institution | Directory Open Access Journal |
| issn | 2198-3844 |
| language | English |
| last_indexed | 2024-03-12T17:30:07Z |
| publishDate | 2018-06-01 |
| publisher | Wiley |
| record_format | Article |
| series | Advanced Science |
| spelling | doaj.art-e865dff216b74995966da1b5537171af2023-08-05T03:41:20ZengWileyAdvanced Science2198-38442018-06-0156n/an/a10.1002/advs.201800130Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport LayerYonghui Lee0Seunghwan Lee1Gabseok Seo2Sanghyun Paek3Kyung Taek Cho4Aron J. Huckaba5Marco Calizzi6Dong‐won Choi7Jin‐Seong Park8Dongwook Lee9Hyo Joong Lee10Abdullah M. Asiri11Mohammad Khaja Nazeeruddin12Group for Molecular Engineering of Functional Materials Ecole Polytechnique Fédérale de Lausanne CH‐1951 Sion SwitzerlandDivision of Materials Science and Engineering Hanyang University 222 Wangsimni‐ro Seongdong‐gu Seoul 133‐791 KoreaGroup for Molecular Engineering of Functional Materials Ecole Polytechnique Fédérale de Lausanne CH‐1951 Sion SwitzerlandGroup for Molecular Engineering of Functional Materials Ecole Polytechnique Fédérale de Lausanne CH‐1951 Sion SwitzerlandGroup for Molecular Engineering of Functional Materials Ecole Polytechnique Fédérale de Lausanne CH‐1951 Sion SwitzerlandGroup for Molecular Engineering of Functional Materials Ecole Polytechnique Fédérale de Lausanne CH‐1951 Sion SwitzerlandLaboratory of Materials for Renewable Energy Ecole Polytechnique Fédérale de Lausanne CH‐1951 Sion SwitzerlandDivision of Materials Science and Engineering Hanyang University 222 Wangsimni‐ro Seongdong‐gu Seoul 133‐791 KoreaDivision of Materials Science and Engineering Hanyang University 222 Wangsimni‐ro Seongdong‐gu Seoul 133‐791 KoreaDivision of Physics and Applied Physics School of Physical and Mathematical Science Nanyang Technological University Singapore 637371 SingaporeGroup for Molecular Engineering of Functional Materials Ecole Polytechnique Fédérale de Lausanne CH‐1951 Sion SwitzerlandCenter of Excellence for Advanced Materials Research (CEAMR) King Abdulaziz University P. O. Box 80203 Jeddah 21589 Saudi ArabiaGroup for Molecular Engineering of Functional Materials Ecole Polytechnique Fédérale de Lausanne CH‐1951 Sion SwitzerlandAbstract Planar perovskite solar cells using low‐temperature atomic layer deposition (ALD) of the SnO2 electron transporting layer (ETL), with excellent electron extraction and hole‐blocking ability, offer significant advantages compared with high‐temperature deposition methods. The optical, chemical, and electrical properties of the ALD SnO2 layer and its influence on the device performance are investigated. It is found that surface passivation of SnO2 is essential to reduce charge recombination at the perovskite and ETL interface and show that the fabricated planar perovskite solar cells exhibit high reproducibility, stability, and power conversion efficiency of 20%.https://doi.org/10.1002/advs.201800130atomic layer depositionpassivationperovskitesplanar perovskite solar cellsSnO2 electron transporting layers |
| spellingShingle | Yonghui Lee Seunghwan Lee Gabseok Seo Sanghyun Paek Kyung Taek Cho Aron J. Huckaba Marco Calizzi Dong‐won Choi Jin‐Seong Park Dongwook Lee Hyo Joong Lee Abdullah M. Asiri Mohammad Khaja Nazeeruddin Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer Advanced Science atomic layer deposition passivation perovskites planar perovskite solar cells SnO2 electron transporting layers |
| title | Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer |
| title_full | Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer |
| title_fullStr | Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer |
| title_full_unstemmed | Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer |
| title_short | Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer |
| title_sort | efficient planar perovskite solar cells using passivated tin oxide as an electron transport layer |
| topic | atomic layer deposition passivation perovskites planar perovskite solar cells SnO2 electron transporting layers |
| url | https://doi.org/10.1002/advs.201800130 |
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