Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern Poland

This study assesses the air quality in Zabrze (southern Poland) based on the ambient concentrations of equivalent black carbon (eBC). eBC measurement campaigns were carried out from April 2019 to March 2020 using a modern AE33 Aethalometer, accompanied by parallel measurements of gaseous pollutants,...

Full description

Bibliographic Details
Main Authors: Natalia Zioła, Barbara Błaszczak, Krzysztof Klejnowski
Format: Article
Language:English
Published: MDPI AG 2021-01-01
Series:Atmosphere
Subjects:
Online Access:https://www.mdpi.com/2073-4433/12/1/119
_version_ 1797410925914882048
author Natalia Zioła
Barbara Błaszczak
Krzysztof Klejnowski
author_facet Natalia Zioła
Barbara Błaszczak
Krzysztof Klejnowski
author_sort Natalia Zioła
collection DOAJ
description This study assesses the air quality in Zabrze (southern Poland) based on the ambient concentrations of equivalent black carbon (eBC). eBC measurement campaigns were carried out from April 2019 to March 2020 using a modern AE33 Aethalometer, accompanied by parallel measurements of gaseous pollutants, PM<sub>10</sub> and meteorological parameters. The use of the two-component AE33 model allows for the determination of the eBC from fossil fuel combustion (eBC<sub>ff</sub>) and biomass burning (eBC<sub>bb</sub>). The obtained results showed a clear seasonal variability of eBC concentrations, with higher average levels in the heating season (4.70 µg·m<sup>−3</sup>) compared to the non-heating one (1.79 µg·m<sup>−3</sup>). In both seasons, the eBC<sub>ff</sub> component had a dominant share in total eBC, which indicates significant emissions from the combustion of fossil fuels for heating purposes and from local traffic sources. The obtained results showed high correlation coefficients with gaseous and particulate pollutants, with the strongest relationship for eBC and carbon monoxide (CO). During the non-heating and heating period, both anticyclone and cyclone systems played an important role in shaping eBC, eBC<sub>ff</sub> and eBC<sub>bb</sub> concentrations. High concentrations of all components occurred with a significant decrease in air temperature and solar radiation in winter.
first_indexed 2024-03-09T04:37:30Z
format Article
id doaj.art-e8b81ba520ed49119fb4908f356ff266
institution Directory Open Access Journal
issn 2073-4433
language English
last_indexed 2024-03-09T04:37:30Z
publishDate 2021-01-01
publisher MDPI AG
record_format Article
series Atmosphere
spelling doaj.art-e8b81ba520ed49119fb4908f356ff2662023-12-03T13:26:16ZengMDPI AGAtmosphere2073-44332021-01-0112111910.3390/atmos12010119Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern PolandNatalia Zioła0Barbara Błaszczak1Krzysztof Klejnowski2Institute of Environmental Engineering of the Polish Academy of Sciences, 34 M. Skłodowska-Curie Str., 41-819 Zabrze, PolandInstitute of Environmental Engineering of the Polish Academy of Sciences, 34 M. Skłodowska-Curie Str., 41-819 Zabrze, PolandInstitute of Environmental Engineering of the Polish Academy of Sciences, 34 M. Skłodowska-Curie Str., 41-819 Zabrze, PolandThis study assesses the air quality in Zabrze (southern Poland) based on the ambient concentrations of equivalent black carbon (eBC). eBC measurement campaigns were carried out from April 2019 to March 2020 using a modern AE33 Aethalometer, accompanied by parallel measurements of gaseous pollutants, PM<sub>10</sub> and meteorological parameters. The use of the two-component AE33 model allows for the determination of the eBC from fossil fuel combustion (eBC<sub>ff</sub>) and biomass burning (eBC<sub>bb</sub>). The obtained results showed a clear seasonal variability of eBC concentrations, with higher average levels in the heating season (4.70 µg·m<sup>−3</sup>) compared to the non-heating one (1.79 µg·m<sup>−3</sup>). In both seasons, the eBC<sub>ff</sub> component had a dominant share in total eBC, which indicates significant emissions from the combustion of fossil fuels for heating purposes and from local traffic sources. The obtained results showed high correlation coefficients with gaseous and particulate pollutants, with the strongest relationship for eBC and carbon monoxide (CO). During the non-heating and heating period, both anticyclone and cyclone systems played an important role in shaping eBC, eBC<sub>ff</sub> and eBC<sub>bb</sub> concentrations. High concentrations of all components occurred with a significant decrease in air temperature and solar radiation in winter.https://www.mdpi.com/2073-4433/12/1/119black carbonsootcarbonaceous matterfossil fuelsbiomass burningsoot
spellingShingle Natalia Zioła
Barbara Błaszczak
Krzysztof Klejnowski
Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern Poland
Atmosphere
black carbon
soot
carbonaceous matter
fossil fuels
biomass burning
soot
title Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern Poland
title_full Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern Poland
title_fullStr Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern Poland
title_full_unstemmed Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern Poland
title_short Temporal Variability of Equivalent Black Carbon Components in Atmospheric Air in Southern Poland
title_sort temporal variability of equivalent black carbon components in atmospheric air in southern poland
topic black carbon
soot
carbonaceous matter
fossil fuels
biomass burning
soot
url https://www.mdpi.com/2073-4433/12/1/119
work_keys_str_mv AT nataliazioła temporalvariabilityofequivalentblackcarboncomponentsinatmosphericairinsouthernpoland
AT barbarabłaszczak temporalvariabilityofequivalentblackcarboncomponentsinatmosphericairinsouthernpoland
AT krzysztofklejnowski temporalvariabilityofequivalentblackcarboncomponentsinatmosphericairinsouthernpoland