Orbital and magnetic ordering and domain-wall conduction in ferrimagnet La_{5}Mo_{4}O_{16}

We studied the ferrimagnet La_{5}Mo_{4}O_{16} with Mo ions on quasisquare lattices both experimentally and theoretically. We found that in addition to the antiferromagnetic ordering at T_{N}=200 K, a magnetic phase transition into a ferrimagnetic phase occurs at T_{s1}=60 K, which is caused by the o...

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Main Authors: Takuro Katsufuji, Masayuki Miyake, Makoto Naka, Masahito Mochizuki, Sota Kogo, Tomomasa Kajita, Yasuhiro Shimizu, Masayuki Itoh, Takatoshi Hasegawa, Shunsuke Shimose, Shunta Noguchi, Takuo Saiki, Takuro Sato, Fumitaka Kagawa
Format: Article
Language:English
Published: American Physical Society 2021-02-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.3.013105
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author Takuro Katsufuji
Masayuki Miyake
Makoto Naka
Masahito Mochizuki
Sota Kogo
Tomomasa Kajita
Yasuhiro Shimizu
Masayuki Itoh
Takatoshi Hasegawa
Shunsuke Shimose
Shunta Noguchi
Takuo Saiki
Takuro Sato
Fumitaka Kagawa
author_facet Takuro Katsufuji
Masayuki Miyake
Makoto Naka
Masahito Mochizuki
Sota Kogo
Tomomasa Kajita
Yasuhiro Shimizu
Masayuki Itoh
Takatoshi Hasegawa
Shunsuke Shimose
Shunta Noguchi
Takuo Saiki
Takuro Sato
Fumitaka Kagawa
author_sort Takuro Katsufuji
collection DOAJ
description We studied the ferrimagnet La_{5}Mo_{4}O_{16} with Mo ions on quasisquare lattices both experimentally and theoretically. We found that in addition to the antiferromagnetic ordering at T_{N}=200 K, a magnetic phase transition into a ferrimagnetic phase occurs at T_{s1}=60 K, which is caused by the orbital ordering of the Mo 4d states. We also found that the relatively small size of ferrimagnetic domains despite the large Ising anisotropy of the Mo spins are formed below T_{s1}, which are responsible for the relaxation behavior and the memory effect in the magnetization. Nonvolatile positive magnetoresistance observed in this compound below T_{s1} can be attributed to the fact that such magnetic domains and the electrical conduction along the domain walls disappear with the applied magnetic field.
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spelling doaj.art-e9bebae58fa64a4eb721d520255915a02024-04-12T17:06:56ZengAmerican Physical SocietyPhysical Review Research2643-15642021-02-013101310510.1103/PhysRevResearch.3.013105Orbital and magnetic ordering and domain-wall conduction in ferrimagnet La_{5}Mo_{4}O_{16}Takuro KatsufujiMasayuki MiyakeMakoto NakaMasahito MochizukiSota KogoTomomasa KajitaYasuhiro ShimizuMasayuki ItohTakatoshi HasegawaShunsuke ShimoseShunta NoguchiTakuo SaikiTakuro SatoFumitaka KagawaWe studied the ferrimagnet La_{5}Mo_{4}O_{16} with Mo ions on quasisquare lattices both experimentally and theoretically. We found that in addition to the antiferromagnetic ordering at T_{N}=200 K, a magnetic phase transition into a ferrimagnetic phase occurs at T_{s1}=60 K, which is caused by the orbital ordering of the Mo 4d states. We also found that the relatively small size of ferrimagnetic domains despite the large Ising anisotropy of the Mo spins are formed below T_{s1}, which are responsible for the relaxation behavior and the memory effect in the magnetization. Nonvolatile positive magnetoresistance observed in this compound below T_{s1} can be attributed to the fact that such magnetic domains and the electrical conduction along the domain walls disappear with the applied magnetic field.http://doi.org/10.1103/PhysRevResearch.3.013105
spellingShingle Takuro Katsufuji
Masayuki Miyake
Makoto Naka
Masahito Mochizuki
Sota Kogo
Tomomasa Kajita
Yasuhiro Shimizu
Masayuki Itoh
Takatoshi Hasegawa
Shunsuke Shimose
Shunta Noguchi
Takuo Saiki
Takuro Sato
Fumitaka Kagawa
Orbital and magnetic ordering and domain-wall conduction in ferrimagnet La_{5}Mo_{4}O_{16}
Physical Review Research
title Orbital and magnetic ordering and domain-wall conduction in ferrimagnet La_{5}Mo_{4}O_{16}
title_full Orbital and magnetic ordering and domain-wall conduction in ferrimagnet La_{5}Mo_{4}O_{16}
title_fullStr Orbital and magnetic ordering and domain-wall conduction in ferrimagnet La_{5}Mo_{4}O_{16}
title_full_unstemmed Orbital and magnetic ordering and domain-wall conduction in ferrimagnet La_{5}Mo_{4}O_{16}
title_short Orbital and magnetic ordering and domain-wall conduction in ferrimagnet La_{5}Mo_{4}O_{16}
title_sort orbital and magnetic ordering and domain wall conduction in ferrimagnet la 5 mo 4 o 16
url http://doi.org/10.1103/PhysRevResearch.3.013105
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