Subgrid-scale variability in clear-sky relative humidity and forcing by aerosol–radiation interactions in an atmosphere model

Atmosphere models with resolutions of several tens of kilometres take subgrid-scale variability in the total specific humidity <i>q</i><sub>t</sub> into account by using a uniform probability density function (PDF) to predict fractional cloud cover. However, usually only m...

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Bibliographic Details
Main Authors: P. Petersik, M. Salzmann, J. Kretzschmar, R. Cherian, D. Mewes, J. Quaas
Format: Article
Language:English
Published: Copernicus Publications 2018-06-01
Series:Atmospheric Chemistry and Physics
Online Access:https://www.atmos-chem-phys.net/18/8589/2018/acp-18-8589-2018.pdf
Description
Summary:Atmosphere models with resolutions of several tens of kilometres take subgrid-scale variability in the total specific humidity <i>q</i><sub>t</sub> into account by using a uniform probability density function (PDF) to predict fractional cloud cover. However, usually only mean relative humidity, <span style="text-decoration: overline;">RH</span>, or mean clear-sky relative humidity, <span style="text-decoration: overline;">RH</span><sub>cls</sub>, is used to compute hygroscopic growth of soluble aerosol particles. While previous studies based on limited-area models and also a global model suggest that subgrid-scale variability in RH should be taken into account for estimating radiative forcing due to aerosol–radiation interactions (RFari), here we present the first estimate of RFari using a global atmospheric model with a parameterization for subgrid-scale variability in RH that is consistent with the assumptions in the model. For this, we sample the subsaturated part of the uniform RH-PDF from the cloud cover scheme for its application in the hygroscopic growth parameterization in the ECHAM6-HAM2 atmosphere model. Due to the non-linear dependence of the hygroscopic growth on RH, this causes an increase in aerosol hygroscopic growth. Aerosol optical depth (AOD) increases by a global mean of 0.009 ( ∼ 7.8 <i>%</i> in comparison to the control run). Especially over the tropics AOD is enhanced with a mean of about 0.013. Due to the increase in AOD, net top of the atmosphere clear-sky solar radiation, SW<sub>net, cls</sub>, decreases by −0.22 W m<sup>−2</sup> ( ∼ −0.08 <i>%</i>). Finally, the RFari changes from −0.15 to −0.19 W m<sup>−2</sup>  by about 31 %. The reason for this very disproportionate effect is that anthropogenic aerosols are disproportionally hygroscopic.
ISSN:1680-7316
1680-7324