Subgrid-scale variability in clear-sky relative humidity and forcing by aerosol–radiation interactions in an atmosphere model

Atmosphere models with resolutions of several tens of kilometres take subgrid-scale variability in the total specific humidity <i>q</i><sub>t</sub> into account by using a uniform probability density function (PDF) to predict fractional cloud cover. However, usually only m...

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Main Authors: P. Petersik, M. Salzmann, J. Kretzschmar, R. Cherian, D. Mewes, J. Quaas
Format: Article
Language:English
Published: Copernicus Publications 2018-06-01
Series:Atmospheric Chemistry and Physics
Online Access:https://www.atmos-chem-phys.net/18/8589/2018/acp-18-8589-2018.pdf
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author P. Petersik
M. Salzmann
J. Kretzschmar
R. Cherian
D. Mewes
J. Quaas
author_facet P. Petersik
M. Salzmann
J. Kretzschmar
R. Cherian
D. Mewes
J. Quaas
author_sort P. Petersik
collection DOAJ
description Atmosphere models with resolutions of several tens of kilometres take subgrid-scale variability in the total specific humidity <i>q</i><sub>t</sub> into account by using a uniform probability density function (PDF) to predict fractional cloud cover. However, usually only mean relative humidity, <span style="text-decoration: overline;">RH</span>, or mean clear-sky relative humidity, <span style="text-decoration: overline;">RH</span><sub>cls</sub>, is used to compute hygroscopic growth of soluble aerosol particles. While previous studies based on limited-area models and also a global model suggest that subgrid-scale variability in RH should be taken into account for estimating radiative forcing due to aerosol–radiation interactions (RFari), here we present the first estimate of RFari using a global atmospheric model with a parameterization for subgrid-scale variability in RH that is consistent with the assumptions in the model. For this, we sample the subsaturated part of the uniform RH-PDF from the cloud cover scheme for its application in the hygroscopic growth parameterization in the ECHAM6-HAM2 atmosphere model. Due to the non-linear dependence of the hygroscopic growth on RH, this causes an increase in aerosol hygroscopic growth. Aerosol optical depth (AOD) increases by a global mean of 0.009 ( ∼ 7.8 <i>%</i> in comparison to the control run). Especially over the tropics AOD is enhanced with a mean of about 0.013. Due to the increase in AOD, net top of the atmosphere clear-sky solar radiation, SW<sub>net, cls</sub>, decreases by −0.22 W m<sup>−2</sup> ( ∼ −0.08 <i>%</i>). Finally, the RFari changes from −0.15 to −0.19 W m<sup>−2</sup>  by about 31 %. The reason for this very disproportionate effect is that anthropogenic aerosols are disproportionally hygroscopic.
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spelling doaj.art-ec7a09b18a954ae49dc123724d6e42c22022-12-22T00:02:21ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242018-06-01188589859910.5194/acp-18-8589-2018Subgrid-scale variability in clear-sky relative humidity and forcing by aerosol–radiation interactions in an atmosphere modelP. Petersik0M. Salzmann1J. Kretzschmar2R. Cherian3D. Mewes4J. Quaas5Leipzig Institute for Meteorology, Universität Leipzig, Leipzig, GermanyLeipzig Institute for Meteorology, Universität Leipzig, Leipzig, GermanyLeipzig Institute for Meteorology, Universität Leipzig, Leipzig, GermanyLeipzig Institute for Meteorology, Universität Leipzig, Leipzig, GermanyLeipzig Institute for Meteorology, Universität Leipzig, Leipzig, GermanyLeipzig Institute for Meteorology, Universität Leipzig, Leipzig, GermanyAtmosphere models with resolutions of several tens of kilometres take subgrid-scale variability in the total specific humidity <i>q</i><sub>t</sub> into account by using a uniform probability density function (PDF) to predict fractional cloud cover. However, usually only mean relative humidity, <span style="text-decoration: overline;">RH</span>, or mean clear-sky relative humidity, <span style="text-decoration: overline;">RH</span><sub>cls</sub>, is used to compute hygroscopic growth of soluble aerosol particles. While previous studies based on limited-area models and also a global model suggest that subgrid-scale variability in RH should be taken into account for estimating radiative forcing due to aerosol–radiation interactions (RFari), here we present the first estimate of RFari using a global atmospheric model with a parameterization for subgrid-scale variability in RH that is consistent with the assumptions in the model. For this, we sample the subsaturated part of the uniform RH-PDF from the cloud cover scheme for its application in the hygroscopic growth parameterization in the ECHAM6-HAM2 atmosphere model. Due to the non-linear dependence of the hygroscopic growth on RH, this causes an increase in aerosol hygroscopic growth. Aerosol optical depth (AOD) increases by a global mean of 0.009 ( ∼ 7.8 <i>%</i> in comparison to the control run). Especially over the tropics AOD is enhanced with a mean of about 0.013. Due to the increase in AOD, net top of the atmosphere clear-sky solar radiation, SW<sub>net, cls</sub>, decreases by −0.22 W m<sup>−2</sup> ( ∼ −0.08 <i>%</i>). Finally, the RFari changes from −0.15 to −0.19 W m<sup>−2</sup>  by about 31 %. The reason for this very disproportionate effect is that anthropogenic aerosols are disproportionally hygroscopic.https://www.atmos-chem-phys.net/18/8589/2018/acp-18-8589-2018.pdf
spellingShingle P. Petersik
M. Salzmann
J. Kretzschmar
R. Cherian
D. Mewes
J. Quaas
Subgrid-scale variability in clear-sky relative humidity and forcing by aerosol–radiation interactions in an atmosphere model
Atmospheric Chemistry and Physics
title Subgrid-scale variability in clear-sky relative humidity and forcing by aerosol–radiation interactions in an atmosphere model
title_full Subgrid-scale variability in clear-sky relative humidity and forcing by aerosol–radiation interactions in an atmosphere model
title_fullStr Subgrid-scale variability in clear-sky relative humidity and forcing by aerosol–radiation interactions in an atmosphere model
title_full_unstemmed Subgrid-scale variability in clear-sky relative humidity and forcing by aerosol–radiation interactions in an atmosphere model
title_short Subgrid-scale variability in clear-sky relative humidity and forcing by aerosol–radiation interactions in an atmosphere model
title_sort subgrid scale variability in clear sky relative humidity and forcing by aerosol radiation interactions in an atmosphere model
url https://www.atmos-chem-phys.net/18/8589/2018/acp-18-8589-2018.pdf
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