Magnetism and Néel skyrmion dynamics in GaV_{4}S_{8-y}Se_{y}

We present an investigation of the influence of low levels of chemical substitution on the magnetic ground state and Néel skyrmion lattice (SkL) state in GaV_{4}S_{8-y}Se_{y}, where y=0,0.1,7.9, and 8. Muon-spin spectroscopy (μSR) measurements on y=0 and 0.1 materials reveal the magnetic ground stat...

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Bibliographic Details
Main Authors: T. J. Hicken, S. J. R. Holt, K. J. A. Franke, Z. Hawkhead, A. Štefančič, M. N. Wilson, M. Gomilšek, B. M. Huddart, S. J. Clark, M. R. Lees, F. L. Pratt, S. J. Blundell, G. Balakrishnan, T. Lancaster
Format: Article
Language:English
Published: American Physical Society 2020-07-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.2.032001
Description
Summary:We present an investigation of the influence of low levels of chemical substitution on the magnetic ground state and Néel skyrmion lattice (SkL) state in GaV_{4}S_{8-y}Se_{y}, where y=0,0.1,7.9, and 8. Muon-spin spectroscopy (μSR) measurements on y=0 and 0.1 materials reveal the magnetic ground state consists of microscopically coexisting incommensurate cycloidal and ferromagnetic environments, whereas chemical substitution leads to the growth of localized regions of increased spin density. μSR measurements of emergent low-frequency skyrmion dynamics show that the SkL exists under low levels of substitution at both ends of the series. Skyrmionic excitations persist to temperatures below the equilibrium SkL in substituted samples, suggesting the presence of skyrmion precursors over a wide range of temperatures.
ISSN:2643-1564