Strong absorption and ultrafast localisation in NaBiS2 nanocrystals with slow charge-carrier recombination

Ternary chalcogenides are gaining interest as nontoxic, stable solar absorbers. Here, the authors investigate NaBiS2, finding cation disorder to be a critical parameter that enables its high absorption strength and unusual charge-carrier kinetics.

Bibliographic Details
Main Authors: Yi-Teng Huang, Seán R. Kavanagh, Marcello Righetto, Marin Rusu, Igal Levine, Thomas Unold, Szymon J. Zelewski, Alexander J. Sneyd, Kaiwen Zhang, Linjie Dai, Andrew J. Britton, Junzhi Ye, Jaakko Julin, Mari Napari, Zhilong Zhang, James Xiao, Mikko Laitinen, Laura Torrente-Murciano, Samuel D. Stranks, Akshay Rao, Laura M. Herz, David O. Scanlon, Aron Walsh, Robert L. Z. Hoye
Format: Article
Language:English
Published: Nature Portfolio 2022-08-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-022-32669-3
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author Yi-Teng Huang
Seán R. Kavanagh
Marcello Righetto
Marin Rusu
Igal Levine
Thomas Unold
Szymon J. Zelewski
Alexander J. Sneyd
Kaiwen Zhang
Linjie Dai
Andrew J. Britton
Junzhi Ye
Jaakko Julin
Mari Napari
Zhilong Zhang
James Xiao
Mikko Laitinen
Laura Torrente-Murciano
Samuel D. Stranks
Akshay Rao
Laura M. Herz
David O. Scanlon
Aron Walsh
Robert L. Z. Hoye
author_facet Yi-Teng Huang
Seán R. Kavanagh
Marcello Righetto
Marin Rusu
Igal Levine
Thomas Unold
Szymon J. Zelewski
Alexander J. Sneyd
Kaiwen Zhang
Linjie Dai
Andrew J. Britton
Junzhi Ye
Jaakko Julin
Mari Napari
Zhilong Zhang
James Xiao
Mikko Laitinen
Laura Torrente-Murciano
Samuel D. Stranks
Akshay Rao
Laura M. Herz
David O. Scanlon
Aron Walsh
Robert L. Z. Hoye
author_sort Yi-Teng Huang
collection DOAJ
description Ternary chalcogenides are gaining interest as nontoxic, stable solar absorbers. Here, the authors investigate NaBiS2, finding cation disorder to be a critical parameter that enables its high absorption strength and unusual charge-carrier kinetics.
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spelling doaj.art-ed96a07e628742a5bca386c73c53182b2022-12-22T01:36:29ZengNature PortfolioNature Communications2041-17232022-08-0113111310.1038/s41467-022-32669-3Strong absorption and ultrafast localisation in NaBiS2 nanocrystals with slow charge-carrier recombinationYi-Teng Huang0Seán R. Kavanagh1Marcello Righetto2Marin Rusu3Igal Levine4Thomas Unold5Szymon J. Zelewski6Alexander J. Sneyd7Kaiwen Zhang8Linjie Dai9Andrew J. Britton10Junzhi Ye11Jaakko Julin12Mari Napari13Zhilong Zhang14James Xiao15Mikko Laitinen16Laura Torrente-Murciano17Samuel D. Stranks18Akshay Rao19Laura M. Herz20David O. Scanlon21Aron Walsh22Robert L. Z. Hoye23Cavendish Laboratory, University of CambridgeDepartment of Chemistry, University College LondonDepartment of Physics, University of Oxford, Clarendon LaboratoryStruktur und Dynamik von Energiematerialien, Helmholtz-Zentrum Berlin für Materialien und EnergieHelmholtz-Zentrum Berlin für Materialien und Energie GmbHStruktur und Dynamik von Energiematerialien, Helmholtz-Zentrum Berlin für Materialien und EnergieCavendish Laboratory, University of CambridgeCavendish Laboratory, University of CambridgeDepartment of Chemical Engineering and Biotechnology, University of CambridgeCavendish Laboratory, University of CambridgeSchool of Chemical and Process Engineering, University of LeedsCavendish Laboratory, University of CambridgeDepartment of Physics, University of JyväskyläSchool of Electronics and Computer Science, University of SouthamptonCavendish Laboratory, University of CambridgeCavendish Laboratory, University of CambridgeInstitute for Advanced Study, Technical University of MunichDepartment of Chemical Engineering and Biotechnology, University of CambridgeCavendish Laboratory, University of CambridgeCavendish Laboratory, University of CambridgeDepartment of Physics, University of Oxford, Clarendon LaboratoryDepartment of Chemistry, University College LondonDepartment of Materials, Imperial College LondonDepartment of Materials, Imperial College LondonTernary chalcogenides are gaining interest as nontoxic, stable solar absorbers. Here, the authors investigate NaBiS2, finding cation disorder to be a critical parameter that enables its high absorption strength and unusual charge-carrier kinetics.https://doi.org/10.1038/s41467-022-32669-3
spellingShingle Yi-Teng Huang
Seán R. Kavanagh
Marcello Righetto
Marin Rusu
Igal Levine
Thomas Unold
Szymon J. Zelewski
Alexander J. Sneyd
Kaiwen Zhang
Linjie Dai
Andrew J. Britton
Junzhi Ye
Jaakko Julin
Mari Napari
Zhilong Zhang
James Xiao
Mikko Laitinen
Laura Torrente-Murciano
Samuel D. Stranks
Akshay Rao
Laura M. Herz
David O. Scanlon
Aron Walsh
Robert L. Z. Hoye
Strong absorption and ultrafast localisation in NaBiS2 nanocrystals with slow charge-carrier recombination
Nature Communications
title Strong absorption and ultrafast localisation in NaBiS2 nanocrystals with slow charge-carrier recombination
title_full Strong absorption and ultrafast localisation in NaBiS2 nanocrystals with slow charge-carrier recombination
title_fullStr Strong absorption and ultrafast localisation in NaBiS2 nanocrystals with slow charge-carrier recombination
title_full_unstemmed Strong absorption and ultrafast localisation in NaBiS2 nanocrystals with slow charge-carrier recombination
title_short Strong absorption and ultrafast localisation in NaBiS2 nanocrystals with slow charge-carrier recombination
title_sort strong absorption and ultrafast localisation in nabis2 nanocrystals with slow charge carrier recombination
url https://doi.org/10.1038/s41467-022-32669-3
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