Shape-Memory and Anisotropic Carbon Aerogel from Biomass and Graphene Oxide

Biomass, as the most abundant and sustainable resource on the earth, has been regarded as an ideal carbon source to prepare various carbon materials. However, manufacturing shape-memory carbon aerogels with excellent compressibility and elasticity from biomass remains an open challenge. Herein, a ce...

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Main Authors: Zilu Lin, Wenzhao Jiang, Zehong Chen, Linxin Zhong, Chuanfu Liu
Format: Article
Language:English
Published: MDPI AG 2021-09-01
Series:Molecules
Subjects:
Online Access:https://www.mdpi.com/1420-3049/26/18/5715
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author Zilu Lin
Wenzhao Jiang
Zehong Chen
Linxin Zhong
Chuanfu Liu
author_facet Zilu Lin
Wenzhao Jiang
Zehong Chen
Linxin Zhong
Chuanfu Liu
author_sort Zilu Lin
collection DOAJ
description Biomass, as the most abundant and sustainable resource on the earth, has been regarded as an ideal carbon source to prepare various carbon materials. However, manufacturing shape-memory carbon aerogels with excellent compressibility and elasticity from biomass remains an open challenge. Herein, a cellulose-derived carbon aerogel with an anisotropic architecture is fabricated with the assistance of graphene oxide (GO) through a directional freeze-drying process and carbonization. The carbon aerogel displays excellent shape-memory performances, with high stress and height retentions of 93.6% and 95.5% after 1000 compression cycles, respectively. Moreover, the carbon aerogel can identify large ranges of compression strain (10–80%), and demonstrates excellent current stability during cyclic compression. The carbon aerogel can precisely capture a variety of biological signals in the human body, and thus can be used in wearable electronic devices.
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spelling doaj.art-ee79681c453240c892004c9663d24e652023-11-22T14:27:24ZengMDPI AGMolecules1420-30492021-09-012618571510.3390/molecules26185715Shape-Memory and Anisotropic Carbon Aerogel from Biomass and Graphene OxideZilu Lin0Wenzhao Jiang1Zehong Chen2Linxin Zhong3Chuanfu Liu4State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou 510641, ChinaState Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou 510641, ChinaState Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou 510641, ChinaState Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou 510641, ChinaState Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou 510641, ChinaBiomass, as the most abundant and sustainable resource on the earth, has been regarded as an ideal carbon source to prepare various carbon materials. However, manufacturing shape-memory carbon aerogels with excellent compressibility and elasticity from biomass remains an open challenge. Herein, a cellulose-derived carbon aerogel with an anisotropic architecture is fabricated with the assistance of graphene oxide (GO) through a directional freeze-drying process and carbonization. The carbon aerogel displays excellent shape-memory performances, with high stress and height retentions of 93.6% and 95.5% after 1000 compression cycles, respectively. Moreover, the carbon aerogel can identify large ranges of compression strain (10–80%), and demonstrates excellent current stability during cyclic compression. The carbon aerogel can precisely capture a variety of biological signals in the human body, and thus can be used in wearable electronic devices.https://www.mdpi.com/1420-3049/26/18/5715biomassbioresourcecarboxymethyl celluloseaerogelcarbon
spellingShingle Zilu Lin
Wenzhao Jiang
Zehong Chen
Linxin Zhong
Chuanfu Liu
Shape-Memory and Anisotropic Carbon Aerogel from Biomass and Graphene Oxide
Molecules
biomass
bioresource
carboxymethyl cellulose
aerogel
carbon
title Shape-Memory and Anisotropic Carbon Aerogel from Biomass and Graphene Oxide
title_full Shape-Memory and Anisotropic Carbon Aerogel from Biomass and Graphene Oxide
title_fullStr Shape-Memory and Anisotropic Carbon Aerogel from Biomass and Graphene Oxide
title_full_unstemmed Shape-Memory and Anisotropic Carbon Aerogel from Biomass and Graphene Oxide
title_short Shape-Memory and Anisotropic Carbon Aerogel from Biomass and Graphene Oxide
title_sort shape memory and anisotropic carbon aerogel from biomass and graphene oxide
topic biomass
bioresource
carboxymethyl cellulose
aerogel
carbon
url https://www.mdpi.com/1420-3049/26/18/5715
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AT wenzhaojiang shapememoryandanisotropiccarbonaerogelfrombiomassandgrapheneoxide
AT zehongchen shapememoryandanisotropiccarbonaerogelfrombiomassandgrapheneoxide
AT linxinzhong shapememoryandanisotropiccarbonaerogelfrombiomassandgrapheneoxide
AT chuanfuliu shapememoryandanisotropiccarbonaerogelfrombiomassandgrapheneoxide