Influence of a Biofiller, Polylactide, on the General Characteristics of Epoxy-Based Materials

The aim of this work was to obtain epoxy-based composite structures with good mechanical performance, high aging resistance, and an improved degradability profile. For this purpose, powdered polylactide in the amount of 5, 10, 20, 30, and 40 phr was introduced into the epoxy resin, and the composite...

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Main Authors: Angelika Plota-Pietrzak, Leszek Czechowski, Anna Masek
Format: Article
Language:English
Published: MDPI AG 2024-02-01
Series:Materials
Subjects:
Online Access:https://www.mdpi.com/1996-1944/17/5/1069
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author Angelika Plota-Pietrzak
Leszek Czechowski
Anna Masek
author_facet Angelika Plota-Pietrzak
Leszek Czechowski
Anna Masek
author_sort Angelika Plota-Pietrzak
collection DOAJ
description The aim of this work was to obtain epoxy-based composite structures with good mechanical performance, high aging resistance, and an improved degradability profile. For this purpose, powdered polylactide in the amount of 5, 10, 20, 30, and 40 phr was introduced into the epoxy resin, and the composites were fabricated by a simple method, which is similar to that used on an industrial scale in the fabrication of these products. The first analysis concerned the study of the effect of PLA addition to epoxy resin-based composites on their mechanical properties. One-directional tensile tests of samples were performed for three directions (0, 90, and 45 degrees referring to the plate edges). Another aspect of this research was the assessment of the resistance of these composites to long-term exposure to solar radiation and elevated temperature. Based on the obtained results, it was observed that the samples containing 20 or 40 phr of polylactide were characterized by the lowest resistance to the solar aging process. It was therefore concluded that the optimal amount of polylactide in the epoxy resin composite should not be greater than 10 phr to maintain its mechanical behavior and high aging resistance. In the available literature, there are many examples in which scientists have proposed the use of various biofillers (e.g., lignin, starch, rice husk, coconut shell powder) in epoxy composites; however, the impact of polylactide on the general characteristics of the epoxy resin has not been described so far. Therefore, this work perfectly fills the gaps in the literature and may contribute to a more widespread use of additives of natural origin, which may constitute an excellent alternative to commonly used non-renewable compounds.
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spelling doaj.art-ef9691868e82425ebf68bc65bdc4d24e2024-03-12T16:49:09ZengMDPI AGMaterials1996-19442024-02-01175106910.3390/ma17051069Influence of a Biofiller, Polylactide, on the General Characteristics of Epoxy-Based MaterialsAngelika Plota-Pietrzak0Leszek Czechowski1Anna Masek2Institute of Polymer and Dye Technology, Faculty of Chemistry, Lodz University of Technology, 90-537 Lodz, PolandDepartment of Strength of Materials, Lodz University of Technology, 90-537 Lodz, PolandInstitute of Polymer and Dye Technology, Faculty of Chemistry, Lodz University of Technology, 90-537 Lodz, PolandThe aim of this work was to obtain epoxy-based composite structures with good mechanical performance, high aging resistance, and an improved degradability profile. For this purpose, powdered polylactide in the amount of 5, 10, 20, 30, and 40 phr was introduced into the epoxy resin, and the composites were fabricated by a simple method, which is similar to that used on an industrial scale in the fabrication of these products. The first analysis concerned the study of the effect of PLA addition to epoxy resin-based composites on their mechanical properties. One-directional tensile tests of samples were performed for three directions (0, 90, and 45 degrees referring to the plate edges). Another aspect of this research was the assessment of the resistance of these composites to long-term exposure to solar radiation and elevated temperature. Based on the obtained results, it was observed that the samples containing 20 or 40 phr of polylactide were characterized by the lowest resistance to the solar aging process. It was therefore concluded that the optimal amount of polylactide in the epoxy resin composite should not be greater than 10 phr to maintain its mechanical behavior and high aging resistance. In the available literature, there are many examples in which scientists have proposed the use of various biofillers (e.g., lignin, starch, rice husk, coconut shell powder) in epoxy composites; however, the impact of polylactide on the general characteristics of the epoxy resin has not been described so far. Therefore, this work perfectly fills the gaps in the literature and may contribute to a more widespread use of additives of natural origin, which may constitute an excellent alternative to commonly used non-renewable compounds.https://www.mdpi.com/1996-1944/17/5/1069epoxy resinpolylactidebiofillersolar aging
spellingShingle Angelika Plota-Pietrzak
Leszek Czechowski
Anna Masek
Influence of a Biofiller, Polylactide, on the General Characteristics of Epoxy-Based Materials
Materials
epoxy resin
polylactide
biofiller
solar aging
title Influence of a Biofiller, Polylactide, on the General Characteristics of Epoxy-Based Materials
title_full Influence of a Biofiller, Polylactide, on the General Characteristics of Epoxy-Based Materials
title_fullStr Influence of a Biofiller, Polylactide, on the General Characteristics of Epoxy-Based Materials
title_full_unstemmed Influence of a Biofiller, Polylactide, on the General Characteristics of Epoxy-Based Materials
title_short Influence of a Biofiller, Polylactide, on the General Characteristics of Epoxy-Based Materials
title_sort influence of a biofiller polylactide on the general characteristics of epoxy based materials
topic epoxy resin
polylactide
biofiller
solar aging
url https://www.mdpi.com/1996-1944/17/5/1069
work_keys_str_mv AT angelikaplotapietrzak influenceofabiofillerpolylactideonthegeneralcharacteristicsofepoxybasedmaterials
AT leszekczechowski influenceofabiofillerpolylactideonthegeneralcharacteristicsofepoxybasedmaterials
AT annamasek influenceofabiofillerpolylactideonthegeneralcharacteristicsofepoxybasedmaterials