Enhanced Electrochemical Performance of Supercapacitors via Two-Dimensional Indium Sulfide Heterostructure on Carbon Nanotubes

This study reports on the synthesis and characterization of a novel electrode material for supercapacitor applications based on a clustered heterostructure of indium sulfide (In<sub>2</sub>S<sub>3</sub>) and single-walled carbon nanotubes (SWCNTs). The In<sub>2</sub&...

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Main Authors: Niraj Kumar, Dhananjay Mishra, Ajit Kumar, Bidyashakti Dash, Rajneesh Kumar Mishra, Junyoung Song, Sung Hun Jin
Format: Article
Language:English
Published: MDPI AG 2023-03-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/13/6/3678
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author Niraj Kumar
Dhananjay Mishra
Ajit Kumar
Bidyashakti Dash
Rajneesh Kumar Mishra
Junyoung Song
Sung Hun Jin
author_facet Niraj Kumar
Dhananjay Mishra
Ajit Kumar
Bidyashakti Dash
Rajneesh Kumar Mishra
Junyoung Song
Sung Hun Jin
author_sort Niraj Kumar
collection DOAJ
description This study reports on the synthesis and characterization of a novel electrode material for supercapacitor applications based on a clustered heterostructure of indium sulfide (In<sub>2</sub>S<sub>3</sub>) and single-walled carbon nanotubes (SWCNTs). The In<sub>2</sub>S<sub>3</sub>-SWCNT (INSC) sample was prepared using the facile successive ionic layer adsorption and reaction (SILAR) method and demonstrated a higher specific capacitance (258 Fg<sup>−1</sup> at 1 Ag<sup>−1</sup>) compared to the bare indium sulfide (In<sub>2</sub>S<sub>3</sub>) electrode. The enhanced electrochemical performance is attributed to the synergistic effect between the In<sub>2</sub>S<sub>3</sub> and SWCNTs, which improves electron transportation, catalytic nature, and specific capacitance. Moreover, the cyclic stability of the INSC electrode was significantly improved, retaining 96.8% of the initial capacitance after 3000 cycles. The high voltage holding capacity and high cyclic efficiency of the fabricated INSC-based supercapacitor devices suggest their potential for next-generation energy storage devices. Additionally, the INSC electrode-based supercapacitor devices exhibit excellent flexibility and bendability, retaining similar performance even at a bending angle of 180°, making them suitable for flexible energy storage applications.
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spelling doaj.art-efcbfd095ce64c25bede02b01dca32242023-11-17T09:25:14ZengMDPI AGApplied Sciences2076-34172023-03-01136367810.3390/app13063678Enhanced Electrochemical Performance of Supercapacitors via Two-Dimensional Indium Sulfide Heterostructure on Carbon NanotubesNiraj Kumar0Dhananjay Mishra1Ajit Kumar2Bidyashakti Dash3Rajneesh Kumar Mishra4Junyoung Song5Sung Hun Jin6Department of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaDepartment of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaDepartment of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaDepartment of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaDepartment of Physics, Yeungnam University, Gyeongsan 38541, Republic of KoreaDepartment of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaDepartment of Electronics Engineering, Incheon National University, Incheon 22012, Republic of KoreaThis study reports on the synthesis and characterization of a novel electrode material for supercapacitor applications based on a clustered heterostructure of indium sulfide (In<sub>2</sub>S<sub>3</sub>) and single-walled carbon nanotubes (SWCNTs). The In<sub>2</sub>S<sub>3</sub>-SWCNT (INSC) sample was prepared using the facile successive ionic layer adsorption and reaction (SILAR) method and demonstrated a higher specific capacitance (258 Fg<sup>−1</sup> at 1 Ag<sup>−1</sup>) compared to the bare indium sulfide (In<sub>2</sub>S<sub>3</sub>) electrode. The enhanced electrochemical performance is attributed to the synergistic effect between the In<sub>2</sub>S<sub>3</sub> and SWCNTs, which improves electron transportation, catalytic nature, and specific capacitance. Moreover, the cyclic stability of the INSC electrode was significantly improved, retaining 96.8% of the initial capacitance after 3000 cycles. The high voltage holding capacity and high cyclic efficiency of the fabricated INSC-based supercapacitor devices suggest their potential for next-generation energy storage devices. Additionally, the INSC electrode-based supercapacitor devices exhibit excellent flexibility and bendability, retaining similar performance even at a bending angle of 180°, making them suitable for flexible energy storage applications.https://www.mdpi.com/2076-3417/13/6/36782D materialsIn<sub>2</sub>S<sub>3</sub> nanostructureSILAR depositionsupercapacitor
spellingShingle Niraj Kumar
Dhananjay Mishra
Ajit Kumar
Bidyashakti Dash
Rajneesh Kumar Mishra
Junyoung Song
Sung Hun Jin
Enhanced Electrochemical Performance of Supercapacitors via Two-Dimensional Indium Sulfide Heterostructure on Carbon Nanotubes
Applied Sciences
2D materials
In<sub>2</sub>S<sub>3</sub> nanostructure
SILAR deposition
supercapacitor
title Enhanced Electrochemical Performance of Supercapacitors via Two-Dimensional Indium Sulfide Heterostructure on Carbon Nanotubes
title_full Enhanced Electrochemical Performance of Supercapacitors via Two-Dimensional Indium Sulfide Heterostructure on Carbon Nanotubes
title_fullStr Enhanced Electrochemical Performance of Supercapacitors via Two-Dimensional Indium Sulfide Heterostructure on Carbon Nanotubes
title_full_unstemmed Enhanced Electrochemical Performance of Supercapacitors via Two-Dimensional Indium Sulfide Heterostructure on Carbon Nanotubes
title_short Enhanced Electrochemical Performance of Supercapacitors via Two-Dimensional Indium Sulfide Heterostructure on Carbon Nanotubes
title_sort enhanced electrochemical performance of supercapacitors via two dimensional indium sulfide heterostructure on carbon nanotubes
topic 2D materials
In<sub>2</sub>S<sub>3</sub> nanostructure
SILAR deposition
supercapacitor
url https://www.mdpi.com/2076-3417/13/6/3678
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