Ferrimagnetic-ferromagnetic phase transition in Au-doped Mn4N epitaxial films confirmed by x-ray magnetic circular dichroism

The antiperovskite ferrimagnet Mn4N has perpendicular magnetic anisotropy and small spontaneous magnetization, both of which are favorable properties for current induced domain wall motion. Previously we have investigated the magnetic structure of 3d-element-doped Mn4N thin films and demonstrated ul...

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Main Authors: Takumi Horiuchi, Taro Komori, Tomohiro Yasuda, Taku Hirose, Kaoru Toko, Kenta Amemiya, Takashi Suemasu
Format: Article
Language:English
Published: AIP Publishing LLC 2023-02-01
Series:AIP Advances
Online Access:http://dx.doi.org/10.1063/9.0000412
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author Takumi Horiuchi
Taro Komori
Tomohiro Yasuda
Taku Hirose
Kaoru Toko
Kenta Amemiya
Takashi Suemasu
author_facet Takumi Horiuchi
Taro Komori
Tomohiro Yasuda
Taku Hirose
Kaoru Toko
Kenta Amemiya
Takashi Suemasu
author_sort Takumi Horiuchi
collection DOAJ
description The antiperovskite ferrimagnet Mn4N has perpendicular magnetic anisotropy and small spontaneous magnetization, both of which are favorable properties for current induced domain wall motion. Previously we have investigated the magnetic structure of 3d-element-doped Mn4N thin films and demonstrated ultrafast domain wall velocities reaching 3000 m s−1 in the vicinity of the magnetic compensation composition of Ni-doped Mn4N at the current density of j = 1.2 × 1012 A m−2 at room temperature (RT). In this study, we investigate the effect of Au doping on the magnetic structure of Mn4N films, and present a composition ratio-dependent sign reversal of the anomalous Hall effect at RT. X-ray magnetic circular dichroism measurement revealed that the magnetic moment of the face-centered Mn atoms of Mn4−xAuxN reversed between x = 0.1 and 0.2, and became parallel to that of the corner-site Mn atoms for x = 0.2 and 0.3. This result suggests that the ferrimagnetic-ferromagnetic phase transition occurred in Au-doped Mn4N epitaxial films as in the In-doped Mn4N epitaxial films.
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spelling doaj.art-f1a5db6225dd43ff8b429eca7cca4f7d2023-03-10T17:26:20ZengAIP Publishing LLCAIP Advances2158-32262023-02-01132025107025107-510.1063/9.0000412Ferrimagnetic-ferromagnetic phase transition in Au-doped Mn4N epitaxial films confirmed by x-ray magnetic circular dichroismTakumi Horiuchi0Taro Komori1Tomohiro Yasuda2Taku Hirose3Kaoru Toko4Kenta Amemiya5Takashi Suemasu6Graduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanGraduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanGraduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanGraduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanFaculty of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanKEK, Institute of Materials Structure Science, Tsukuba 305-0801, JapanFaculty of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, JapanThe antiperovskite ferrimagnet Mn4N has perpendicular magnetic anisotropy and small spontaneous magnetization, both of which are favorable properties for current induced domain wall motion. Previously we have investigated the magnetic structure of 3d-element-doped Mn4N thin films and demonstrated ultrafast domain wall velocities reaching 3000 m s−1 in the vicinity of the magnetic compensation composition of Ni-doped Mn4N at the current density of j = 1.2 × 1012 A m−2 at room temperature (RT). In this study, we investigate the effect of Au doping on the magnetic structure of Mn4N films, and present a composition ratio-dependent sign reversal of the anomalous Hall effect at RT. X-ray magnetic circular dichroism measurement revealed that the magnetic moment of the face-centered Mn atoms of Mn4−xAuxN reversed between x = 0.1 and 0.2, and became parallel to that of the corner-site Mn atoms for x = 0.2 and 0.3. This result suggests that the ferrimagnetic-ferromagnetic phase transition occurred in Au-doped Mn4N epitaxial films as in the In-doped Mn4N epitaxial films.http://dx.doi.org/10.1063/9.0000412
spellingShingle Takumi Horiuchi
Taro Komori
Tomohiro Yasuda
Taku Hirose
Kaoru Toko
Kenta Amemiya
Takashi Suemasu
Ferrimagnetic-ferromagnetic phase transition in Au-doped Mn4N epitaxial films confirmed by x-ray magnetic circular dichroism
AIP Advances
title Ferrimagnetic-ferromagnetic phase transition in Au-doped Mn4N epitaxial films confirmed by x-ray magnetic circular dichroism
title_full Ferrimagnetic-ferromagnetic phase transition in Au-doped Mn4N epitaxial films confirmed by x-ray magnetic circular dichroism
title_fullStr Ferrimagnetic-ferromagnetic phase transition in Au-doped Mn4N epitaxial films confirmed by x-ray magnetic circular dichroism
title_full_unstemmed Ferrimagnetic-ferromagnetic phase transition in Au-doped Mn4N epitaxial films confirmed by x-ray magnetic circular dichroism
title_short Ferrimagnetic-ferromagnetic phase transition in Au-doped Mn4N epitaxial films confirmed by x-ray magnetic circular dichroism
title_sort ferrimagnetic ferromagnetic phase transition in au doped mn4n epitaxial films confirmed by x ray magnetic circular dichroism
url http://dx.doi.org/10.1063/9.0000412
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