Defect-driven selective metal oxidation at atomic scale
Crystal defects critically influence surface chemical reactions in nanomaterials, yet the basic mechanisms at play are still elusive. Here, the authors show the atomic-scale dynamics of surface oxidation at coherent planar defects in Ag and Pd, revealing how twins and stacking-faults selectively oxi...
Main Authors: | , , , , , , , , , |
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Format: | Article |
Language: | English |
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Nature Portfolio
2021-01-01
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Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-020-20876-9 |
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author | Qi Zhu Zhiliang Pan Zhiyu Zhao Guang Cao Langli Luo Chaolun Ni Hua Wei Ze Zhang Frederic Sansoz Jiangwei Wang |
author_facet | Qi Zhu Zhiliang Pan Zhiyu Zhao Guang Cao Langli Luo Chaolun Ni Hua Wei Ze Zhang Frederic Sansoz Jiangwei Wang |
author_sort | Qi Zhu |
collection | DOAJ |
description | Crystal defects critically influence surface chemical reactions in nanomaterials, yet the basic mechanisms at play are still elusive. Here, the authors show the atomic-scale dynamics of surface oxidation at coherent planar defects in Ag and Pd, revealing how twins and stacking-faults selectively oxidize metallic nanocrystals. |
first_indexed | 2024-12-17T20:30:48Z |
format | Article |
id | doaj.art-f20a96e6c1dc49c78fd03740b5f93f11 |
institution | Directory Open Access Journal |
issn | 2041-1723 |
language | English |
last_indexed | 2024-12-17T20:30:48Z |
publishDate | 2021-01-01 |
publisher | Nature Portfolio |
record_format | Article |
series | Nature Communications |
spelling | doaj.art-f20a96e6c1dc49c78fd03740b5f93f112022-12-21T21:33:36ZengNature PortfolioNature Communications2041-17232021-01-011211810.1038/s41467-020-20876-9Defect-driven selective metal oxidation at atomic scaleQi Zhu0Zhiliang Pan1Zhiyu Zhao2Guang Cao3Langli Luo4Chaolun Ni5Hua Wei6Ze Zhang7Frederic Sansoz8Jiangwei Wang9Center of Electron Microscopy and State Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversitySchool of Mechanical and Electrical Engineering, Guilin University of Electronic TechnologyCenter of Electron Microscopy and State Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityCenter of Electron Microscopy and State Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityInstitute of Molecular Plus, Tianjin UniversityCenter of Electron Microscopy and State Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityCenter for Hypergravity Experimental and Interdisciplinary Research, Zhejiang UniversityCenter of Electron Microscopy and State Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityDepartment of Mechanical Engineering and Materials Science Program, The University of VermontCenter of Electron Microscopy and State Key Laboratory of Silicon Materials, School of Materials Science and Engineering, Zhejiang UniversityCrystal defects critically influence surface chemical reactions in nanomaterials, yet the basic mechanisms at play are still elusive. Here, the authors show the atomic-scale dynamics of surface oxidation at coherent planar defects in Ag and Pd, revealing how twins and stacking-faults selectively oxidize metallic nanocrystals.https://doi.org/10.1038/s41467-020-20876-9 |
spellingShingle | Qi Zhu Zhiliang Pan Zhiyu Zhao Guang Cao Langli Luo Chaolun Ni Hua Wei Ze Zhang Frederic Sansoz Jiangwei Wang Defect-driven selective metal oxidation at atomic scale Nature Communications |
title | Defect-driven selective metal oxidation at atomic scale |
title_full | Defect-driven selective metal oxidation at atomic scale |
title_fullStr | Defect-driven selective metal oxidation at atomic scale |
title_full_unstemmed | Defect-driven selective metal oxidation at atomic scale |
title_short | Defect-driven selective metal oxidation at atomic scale |
title_sort | defect driven selective metal oxidation at atomic scale |
url | https://doi.org/10.1038/s41467-020-20876-9 |
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