Photoluminescence from Two-Phase Nanocomposites Embedded in Polymers

A set of polymer-embedded, two-colored nanocomposites were prepared where the co-existing emission peaks (~578 nm and ~650 nm) had different ratios at their emission thresholds. The nanocomposite samples were simultaneously excited by a 405 nm laser, and the growth of photoluminescence intensities w...

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Main Authors: Mithun Bhowmick, James Christensen, Richard Adjorlolo, Bruno Ullrich
Format: Article
Language:English
Published: MDPI AG 2024-01-01
Series:Micromachines
Subjects:
Online Access:https://www.mdpi.com/2072-666X/15/1/111
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author Mithun Bhowmick
James Christensen
Richard Adjorlolo
Bruno Ullrich
author_facet Mithun Bhowmick
James Christensen
Richard Adjorlolo
Bruno Ullrich
author_sort Mithun Bhowmick
collection DOAJ
description A set of polymer-embedded, two-colored nanocomposites were prepared where the co-existing emission peaks (~578 nm and ~650 nm) had different ratios at their emission thresholds. The nanocomposite samples were simultaneously excited by a 405 nm laser, and the growth of photoluminescence intensities was studied as a function of excitation intensity. The two peaks showed different growth evolution mechanisms. The factors impacting this difference could be (1) energy transfer between the two sized nanoparticles; (2) relaxation mechanism of smaller nanoparticles; and (3) material properties of the polymer.
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spelling doaj.art-f3dce3ebdf9949e28e6b8732503b6f8d2024-01-26T17:45:05ZengMDPI AGMicromachines2072-666X2024-01-0115111110.3390/mi15010111Photoluminescence from Two-Phase Nanocomposites Embedded in PolymersMithun Bhowmick0James Christensen1Richard Adjorlolo2Bruno Ullrich3Mathematical and Physical Sciences, Miami University Regionals, Middletown, OH 45042, USAConstruction Engineering Research Laboratory, United States Army Corps of Engineers, Champaign, IL 61822, USAMathematical and Physical Sciences, Miami University Regionals, Middletown, OH 45042, USAUllrich Photonics LLC, Manistique, MI 49854, USAA set of polymer-embedded, two-colored nanocomposites were prepared where the co-existing emission peaks (~578 nm and ~650 nm) had different ratios at their emission thresholds. The nanocomposite samples were simultaneously excited by a 405 nm laser, and the growth of photoluminescence intensities was studied as a function of excitation intensity. The two peaks showed different growth evolution mechanisms. The factors impacting this difference could be (1) energy transfer between the two sized nanoparticles; (2) relaxation mechanism of smaller nanoparticles; and (3) material properties of the polymer.https://www.mdpi.com/2072-666X/15/1/111quantum dotscompositesCdSephotoluminescencePVAnanoparticles
spellingShingle Mithun Bhowmick
James Christensen
Richard Adjorlolo
Bruno Ullrich
Photoluminescence from Two-Phase Nanocomposites Embedded in Polymers
Micromachines
quantum dots
composites
CdSe
photoluminescence
PVA
nanoparticles
title Photoluminescence from Two-Phase Nanocomposites Embedded in Polymers
title_full Photoluminescence from Two-Phase Nanocomposites Embedded in Polymers
title_fullStr Photoluminescence from Two-Phase Nanocomposites Embedded in Polymers
title_full_unstemmed Photoluminescence from Two-Phase Nanocomposites Embedded in Polymers
title_short Photoluminescence from Two-Phase Nanocomposites Embedded in Polymers
title_sort photoluminescence from two phase nanocomposites embedded in polymers
topic quantum dots
composites
CdSe
photoluminescence
PVA
nanoparticles
url https://www.mdpi.com/2072-666X/15/1/111
work_keys_str_mv AT mithunbhowmick photoluminescencefromtwophasenanocompositesembeddedinpolymers
AT jameschristensen photoluminescencefromtwophasenanocompositesembeddedinpolymers
AT richardadjorlolo photoluminescencefromtwophasenanocompositesembeddedinpolymers
AT brunoullrich photoluminescencefromtwophasenanocompositesembeddedinpolymers