Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC

Modified structure along latent tracks and track formation process have been investigated in poly (allyl diglycol carbonate), PADC, which is well recognized as a sensitive etched track detector. This knowledge is essential to develop novel detectors with improved track registration property. The tra...

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Main Authors: Tomoya Yamauchi, Masato Kanasaki, Rémi Barillon
Format: Article
Language:English
Published: MDPI AG 2021-08-01
Series:Polymers
Subjects:
Online Access:https://www.mdpi.com/2073-4360/13/16/2665
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author Tomoya Yamauchi
Masato Kanasaki
Rémi Barillon
author_facet Tomoya Yamauchi
Masato Kanasaki
Rémi Barillon
author_sort Tomoya Yamauchi
collection DOAJ
description Modified structure along latent tracks and track formation process have been investigated in poly (allyl diglycol carbonate), PADC, which is well recognized as a sensitive etched track detector. This knowledge is essential to develop novel detectors with improved track registration property. The track structures of protons and heavy ions (He, C, Ne, Ar, Fe, Kr and Xe) have been examined by means of FT-IR spectrometry, covering the stopping power region between 1.2 to 12,000 eV/nm. Through a set of experiments on low-<i>LET</i> radiations—such as gamma ray-, multi-step damage process by electron hits was confirmed in the radiation-sensitive parts of the PADC repeat-unit. From this result, we unveiled for the first-time the layered structure in tracks, in relation with the number of secondary electrons. We also proved that the etch pit was formed when at least two repeat-units were destroyed along the track radial direction. To evaluate the number of secondary electrons around the tracks, a series of numerical simulations were performed with Geant4-DNA. Therefore, we are proposing new physical criterions to describe the detection thresholds. Furthermore, we propose a present issue of the definition of detection threshold for semi-relativistic C ions. Additionally, as a possible chemical criterion, formation density of hydroxyl group is suggested to express the response of PADC.
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spelling doaj.art-f3f4a04dbc72476ba915e647e97de6342023-11-22T09:22:28ZengMDPI AGPolymers2073-43602021-08-011316266510.3390/polym13162665Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADCTomoya Yamauchi0Masato Kanasaki1Rémi Barillon2Graduate School of Maritime Sciences, Kobe University, Hyogo 657-8501, JapanGraduate School of Maritime Sciences, Kobe University, Hyogo 657-8501, JapanInstitut Pluridisiplinaire Hubert Curien, UMR 7178, CNRS, The University of Strasbourg, 67081 Strasbourg, FranceModified structure along latent tracks and track formation process have been investigated in poly (allyl diglycol carbonate), PADC, which is well recognized as a sensitive etched track detector. This knowledge is essential to develop novel detectors with improved track registration property. The track structures of protons and heavy ions (He, C, Ne, Ar, Fe, Kr and Xe) have been examined by means of FT-IR spectrometry, covering the stopping power region between 1.2 to 12,000 eV/nm. Through a set of experiments on low-<i>LET</i> radiations—such as gamma ray-, multi-step damage process by electron hits was confirmed in the radiation-sensitive parts of the PADC repeat-unit. From this result, we unveiled for the first-time the layered structure in tracks, in relation with the number of secondary electrons. We also proved that the etch pit was formed when at least two repeat-units were destroyed along the track radial direction. To evaluate the number of secondary electrons around the tracks, a series of numerical simulations were performed with Geant4-DNA. Therefore, we are proposing new physical criterions to describe the detection thresholds. Furthermore, we propose a present issue of the definition of detection threshold for semi-relativistic C ions. Additionally, as a possible chemical criterion, formation density of hydroxyl group is suggested to express the response of PADC.https://www.mdpi.com/2073-4360/13/16/2665PADCpoly (allyl diglycol carbonate)latent tracktrack core radius<i>G</i>–valuelayered structure
spellingShingle Tomoya Yamauchi
Masato Kanasaki
Rémi Barillon
Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
Polymers
PADC
poly (allyl diglycol carbonate)
latent track
track core radius
<i>G</i>–value
layered structure
title Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title_full Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title_fullStr Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title_full_unstemmed Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title_short Methodological and Conceptual Progresses in Studies on the Latent Tracks in PADC
title_sort methodological and conceptual progresses in studies on the latent tracks in padc
topic PADC
poly (allyl diglycol carbonate)
latent track
track core radius
<i>G</i>–value
layered structure
url https://www.mdpi.com/2073-4360/13/16/2665
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AT masatokanasaki methodologicalandconceptualprogressesinstudiesonthelatenttracksinpadc
AT remibarillon methodologicalandconceptualprogressesinstudiesonthelatenttracksinpadc