Stability of Am(Ⅲ) Colloid and Its Adsorption Behavior on Bentonite Colloids

The formation of Am(Ⅲ) colloid and its adsorption behaviors on bentonite colloid were investigated in Beishan 03 groundwater. A series of influencing factors, such as, pH, CO2 concentration in gas atmosphere, ionic strength and temperature, on colloidal stability and adsorption behavior were explore...

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Main Authors: LIU Chen, FANG Sheng, XU Qiang-wei, XU Yu-wei, LONG Hao-qi, BAO Liang-jin, ZHOU Duo
Format: Article
Language:zho
Published: Editorial Office of Journal of Nuclear and Radiochemistry 2022-12-01
Series:He huaxue yu fangshe huaxue
Subjects:
Online Access:http://www.jnrc.org.cn/CN/10.7538/hhx.2022.YX.2021084
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author LIU Chen
FANG Sheng
XU Qiang-wei
XU Yu-wei
LONG Hao-qi
BAO Liang-jin
ZHOU Duo
author_facet LIU Chen
FANG Sheng
XU Qiang-wei
XU Yu-wei
LONG Hao-qi
BAO Liang-jin
ZHOU Duo
author_sort LIU Chen
collection DOAJ
description The formation of Am(Ⅲ) colloid and its adsorption behaviors on bentonite colloid were investigated in Beishan 03 groundwater. A series of influencing factors, such as, pH, CO2 concentration in gas atmosphere, ionic strength and temperature, on colloidal stability and adsorption behavior were explored using Zeta potential laser particle size analyzer, asymmetric flow field flow fractionation system(AF4) and batch experimental method. The results show that the formation and stability of Am(Ⅲ) are closely dependent on the chemical natures of aqueous solution. Increasing temperature or increasing ionic strength will reduce the stability of Am(Ⅲ) colloids, while the increase of carbon dioxide concentration and pH will be beneficial to the stability of Am(Ⅲ) colloid. In addition, with the increase of pH, the density of Am(Ⅲ)-bentonite colloid particles increases, while the Am(Ⅲ) adsorption rate first decreases and then increases; the increase of ionic strength is favor of Am(Ⅲ) adsorption, but the density of colloidal particles decreases; the increase of CO2 concentration in gas phase has a promoting effect on particle density and Am(Ⅲ) adsorption.
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spelling doaj.art-f49ee73ff6f047f58620a29f5f5f084a2024-04-06T05:48:46ZzhoEditorial Office of Journal of Nuclear and RadiochemistryHe huaxue yu fangshe huaxue0253-99502022-12-0144661061810.7538/hhx.2022.YX.2021084Stability of Am(Ⅲ) Colloid and Its Adsorption Behavior on Bentonite ColloidsLIU Chen0FANG Sheng1XU Qiang-wei2XU Yu-wei3LONG Hao-qi4BAO Liang-jin5ZHOU Duo6China Institute of Atomic EnergyChina Institute of Atomic EnergyChina Institute of Atomic EnergyChina Institute of Atomic EnergyChina Institute of Atomic EnergyChina Institute of Atomic EnergyChina Institute of Atomic EnergyThe formation of Am(Ⅲ) colloid and its adsorption behaviors on bentonite colloid were investigated in Beishan 03 groundwater. A series of influencing factors, such as, pH, CO2 concentration in gas atmosphere, ionic strength and temperature, on colloidal stability and adsorption behavior were explored using Zeta potential laser particle size analyzer, asymmetric flow field flow fractionation system(AF4) and batch experimental method. The results show that the formation and stability of Am(Ⅲ) are closely dependent on the chemical natures of aqueous solution. Increasing temperature or increasing ionic strength will reduce the stability of Am(Ⅲ) colloids, while the increase of carbon dioxide concentration and pH will be beneficial to the stability of Am(Ⅲ) colloid. In addition, with the increase of pH, the density of Am(Ⅲ)-bentonite colloid particles increases, while the Am(Ⅲ) adsorption rate first decreases and then increases; the increase of ionic strength is favor of Am(Ⅲ) adsorption, but the density of colloidal particles decreases; the increase of CO2 concentration in gas phase has a promoting effect on particle density and Am(Ⅲ) adsorption.http://www.jnrc.org.cn/CN/10.7538/hhx.2022.YX.2021084am(ⅲ)colloidsstabilityaf4adsorption
spellingShingle LIU Chen
FANG Sheng
XU Qiang-wei
XU Yu-wei
LONG Hao-qi
BAO Liang-jin
ZHOU Duo
Stability of Am(Ⅲ) Colloid and Its Adsorption Behavior on Bentonite Colloids
He huaxue yu fangshe huaxue
am(ⅲ)
colloids
stability
af4
adsorption
title Stability of Am(Ⅲ) Colloid and Its Adsorption Behavior on Bentonite Colloids
title_full Stability of Am(Ⅲ) Colloid and Its Adsorption Behavior on Bentonite Colloids
title_fullStr Stability of Am(Ⅲ) Colloid and Its Adsorption Behavior on Bentonite Colloids
title_full_unstemmed Stability of Am(Ⅲ) Colloid and Its Adsorption Behavior on Bentonite Colloids
title_short Stability of Am(Ⅲ) Colloid and Its Adsorption Behavior on Bentonite Colloids
title_sort stability of am iii colloid and its adsorption behavior on bentonite colloids
topic am(ⅲ)
colloids
stability
af4
adsorption
url http://www.jnrc.org.cn/CN/10.7538/hhx.2022.YX.2021084
work_keys_str_mv AT liuchen stabilityofamiiicolloidanditsadsorptionbehavioronbentonitecolloids
AT fangsheng stabilityofamiiicolloidanditsadsorptionbehavioronbentonitecolloids
AT xuqiangwei stabilityofamiiicolloidanditsadsorptionbehavioronbentonitecolloids
AT xuyuwei stabilityofamiiicolloidanditsadsorptionbehavioronbentonitecolloids
AT longhaoqi stabilityofamiiicolloidanditsadsorptionbehavioronbentonitecolloids
AT baoliangjin stabilityofamiiicolloidanditsadsorptionbehavioronbentonitecolloids
AT zhouduo stabilityofamiiicolloidanditsadsorptionbehavioronbentonitecolloids