Anion-enrichment interface enables high-voltage anode-free lithium metal batteries

The implementation of Li metal anode with high-voltage Ni/Co rich cathode is plagued by low coulombic efficiency and inferior cycling stability. Here authors propose an anion-enriched interface to facilitate the columnar-structure of Li deposits to solve this issue.

Bibliographic Details
Main Authors: Minglei Mao, Xiao Ji, Qiyu Wang, Zejing Lin, Meiying Li, Tao Liu, Chengliang Wang, Yong-Sheng Hu, Hong Li, Xuejie Huang, Liquan Chen, Liumin Suo
Format: Article
Language:English
Published: Nature Portfolio 2023-02-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-023-36853-x
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author Minglei Mao
Xiao Ji
Qiyu Wang
Zejing Lin
Meiying Li
Tao Liu
Chengliang Wang
Yong-Sheng Hu
Hong Li
Xuejie Huang
Liquan Chen
Liumin Suo
author_facet Minglei Mao
Xiao Ji
Qiyu Wang
Zejing Lin
Meiying Li
Tao Liu
Chengliang Wang
Yong-Sheng Hu
Hong Li
Xuejie Huang
Liquan Chen
Liumin Suo
author_sort Minglei Mao
collection DOAJ
description The implementation of Li metal anode with high-voltage Ni/Co rich cathode is plagued by low coulombic efficiency and inferior cycling stability. Here authors propose an anion-enriched interface to facilitate the columnar-structure of Li deposits to solve this issue.
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spelling doaj.art-f535c621a6574ca79ce1ea62daf312f72023-03-22T11:47:37ZengNature PortfolioNature Communications2041-17232023-02-0114111310.1038/s41467-023-36853-xAnion-enrichment interface enables high-voltage anode-free lithium metal batteriesMinglei Mao0Xiao Ji1Qiyu Wang2Zejing Lin3Meiying Li4Tao Liu5Chengliang Wang6Yong-Sheng Hu7Hong Li8Xuejie Huang9Liquan Chen10Liumin Suo11Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter PhysicsSchool of Integrated Circuits, School of Optical and Electronic Information, Wuhan National Laboratory for Optoelectronics (WNLO), Optics Valley Laboratory, Huazhong University of Science and TechnologyBeijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter PhysicsBeijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter PhysicsBeijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter PhysicsBeijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter PhysicsSchool of Integrated Circuits, School of Optical and Electronic Information, Wuhan National Laboratory for Optoelectronics (WNLO), Optics Valley Laboratory, Huazhong University of Science and TechnologyBeijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter PhysicsBeijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter PhysicsBeijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter PhysicsBeijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter PhysicsBeijing Advanced Innovation Center for Materials Genome Engineering, Institute of Physics, Chinese Academy of Sciences, Beijing National Laboratory for Condensed Matter PhysicsThe implementation of Li metal anode with high-voltage Ni/Co rich cathode is plagued by low coulombic efficiency and inferior cycling stability. Here authors propose an anion-enriched interface to facilitate the columnar-structure of Li deposits to solve this issue.https://doi.org/10.1038/s41467-023-36853-x
spellingShingle Minglei Mao
Xiao Ji
Qiyu Wang
Zejing Lin
Meiying Li
Tao Liu
Chengliang Wang
Yong-Sheng Hu
Hong Li
Xuejie Huang
Liquan Chen
Liumin Suo
Anion-enrichment interface enables high-voltage anode-free lithium metal batteries
Nature Communications
title Anion-enrichment interface enables high-voltage anode-free lithium metal batteries
title_full Anion-enrichment interface enables high-voltage anode-free lithium metal batteries
title_fullStr Anion-enrichment interface enables high-voltage anode-free lithium metal batteries
title_full_unstemmed Anion-enrichment interface enables high-voltage anode-free lithium metal batteries
title_short Anion-enrichment interface enables high-voltage anode-free lithium metal batteries
title_sort anion enrichment interface enables high voltage anode free lithium metal batteries
url https://doi.org/10.1038/s41467-023-36853-x
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