The impact of precipitation evaporation on the atmospheric aerosol distribution in EC-Earth v3.2.0

The representation of aerosol–cloud interaction in global climate models (GCMs) remains a large source of uncertainty in climate projections. Due to its complexity, precipitation evaporation is either ignored or taken into account in a simplified manner in GCMs. This research explores various way...

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Main Authors: M. de Bruine, M. Krol, T. van Noije, P. Le Sager, T. Röckmann
Format: Article
Language:English
Published: Copernicus Publications 2018-04-01
Series:Geoscientific Model Development
Online Access:https://www.geosci-model-dev.net/11/1443/2018/gmd-11-1443-2018.pdf
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author M. de Bruine
M. Krol
M. Krol
M. Krol
T. van Noije
P. Le Sager
T. Röckmann
author_facet M. de Bruine
M. Krol
M. Krol
M. Krol
T. van Noije
P. Le Sager
T. Röckmann
author_sort M. de Bruine
collection DOAJ
description The representation of aerosol–cloud interaction in global climate models (GCMs) remains a large source of uncertainty in climate projections. Due to its complexity, precipitation evaporation is either ignored or taken into account in a simplified manner in GCMs. This research explores various ways to treat aerosol resuspension and determines the possible impact of precipitation evaporation and subsequent aerosol resuspension on global aerosol burdens and distribution. The representation of aerosol wet deposition by large-scale precipitation in the EC-Earth model has been improved by utilising additional precipitation-related 3-D fields from the dynamical core, the Integrated Forecasting System (IFS) general circulation model, in the chemistry and aerosol module Tracer Model, version 5 (TM5). A simple approach of scaling aerosol release with evaporated precipitation fraction leads to an increase in the global aerosol burden (+7.8 to +15 % for different aerosol species). However, when taking into account the different sizes and evaporation rate of raindrops following Gong et al. (2006), the release of aerosols is strongly reduced, and the total aerosol burden decreases by −3.0 to −8.5 %. Moreover, inclusion of cloud processing based on observations by Mitra et al. (1992) transforms scavenged small aerosol to coarse particles, which enhances removal by sedimentation and hence leads to a −10 to −11 % lower aerosol burden. Finally, when these two effects are combined, the global aerosol burden decreases by −11 to −19 %. Compared to the Moderate Resolution Imaging Spectroradiometer (MODIS) satellite observations, aerosol optical depth (AOD) is generally underestimated in most parts of the world in all configurations of the TM5 model and although the representation is now physically more realistic, global AOD shows no large improvements in spatial patterns. Similarly, the agreement of the vertical profile with Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) satellite measurements does not improve significantly. We show, however, that aerosol resuspension has a considerable impact on the modelled aerosol distribution and needs to be taken into account.
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spelling doaj.art-f5c7f1d05e3b445b8c282edf0d8215f62022-12-21T18:48:04ZengCopernicus PublicationsGeoscientific Model Development1991-959X1991-96032018-04-01111443146510.5194/gmd-11-1443-2018The impact of precipitation evaporation on the atmospheric aerosol distribution in EC-Earth v3.2.0M. de Bruine0M. Krol1M. Krol2M. Krol3T. van Noije4P. Le Sager5T. Röckmann6Institute for Marine and Atmospheric Research Utrecht, Utrecht University, Utrecht, the NetherlandsInstitute for Marine and Atmospheric Research Utrecht, Utrecht University, Utrecht, the NetherlandsDepartment of Meteorology and Air Quality, Wageningen University, Wageningen, the NetherlandsNetherlands Institute for Space Research SRON, Utrecht, the NetherlandsRoyal Netherlands Meteorological Institute, De Bilt, the NetherlandsRoyal Netherlands Meteorological Institute, De Bilt, the NetherlandsInstitute for Marine and Atmospheric Research Utrecht, Utrecht University, Utrecht, the NetherlandsThe representation of aerosol–cloud interaction in global climate models (GCMs) remains a large source of uncertainty in climate projections. Due to its complexity, precipitation evaporation is either ignored or taken into account in a simplified manner in GCMs. This research explores various ways to treat aerosol resuspension and determines the possible impact of precipitation evaporation and subsequent aerosol resuspension on global aerosol burdens and distribution. The representation of aerosol wet deposition by large-scale precipitation in the EC-Earth model has been improved by utilising additional precipitation-related 3-D fields from the dynamical core, the Integrated Forecasting System (IFS) general circulation model, in the chemistry and aerosol module Tracer Model, version 5 (TM5). A simple approach of scaling aerosol release with evaporated precipitation fraction leads to an increase in the global aerosol burden (+7.8 to +15 % for different aerosol species). However, when taking into account the different sizes and evaporation rate of raindrops following Gong et al. (2006), the release of aerosols is strongly reduced, and the total aerosol burden decreases by −3.0 to −8.5 %. Moreover, inclusion of cloud processing based on observations by Mitra et al. (1992) transforms scavenged small aerosol to coarse particles, which enhances removal by sedimentation and hence leads to a −10 to −11 % lower aerosol burden. Finally, when these two effects are combined, the global aerosol burden decreases by −11 to −19 %. Compared to the Moderate Resolution Imaging Spectroradiometer (MODIS) satellite observations, aerosol optical depth (AOD) is generally underestimated in most parts of the world in all configurations of the TM5 model and although the representation is now physically more realistic, global AOD shows no large improvements in spatial patterns. Similarly, the agreement of the vertical profile with Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) satellite measurements does not improve significantly. We show, however, that aerosol resuspension has a considerable impact on the modelled aerosol distribution and needs to be taken into account.https://www.geosci-model-dev.net/11/1443/2018/gmd-11-1443-2018.pdf
spellingShingle M. de Bruine
M. Krol
M. Krol
M. Krol
T. van Noije
P. Le Sager
T. Röckmann
The impact of precipitation evaporation on the atmospheric aerosol distribution in EC-Earth v3.2.0
Geoscientific Model Development
title The impact of precipitation evaporation on the atmospheric aerosol distribution in EC-Earth v3.2.0
title_full The impact of precipitation evaporation on the atmospheric aerosol distribution in EC-Earth v3.2.0
title_fullStr The impact of precipitation evaporation on the atmospheric aerosol distribution in EC-Earth v3.2.0
title_full_unstemmed The impact of precipitation evaporation on the atmospheric aerosol distribution in EC-Earth v3.2.0
title_short The impact of precipitation evaporation on the atmospheric aerosol distribution in EC-Earth v3.2.0
title_sort impact of precipitation evaporation on the atmospheric aerosol distribution in ec earth v3 2 0
url https://www.geosci-model-dev.net/11/1443/2018/gmd-11-1443-2018.pdf
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