Role of electron scattering on the high-order harmonic generation from solids

We extend the semiclassical trajectory description for the high-order harmonic generation (HHG) from solids by integrating the effect of electron-scattering. Comparing the extended semiclassical trajectory model with a one-dimensional quantum mechanical simulation, we find that the multiplateau feat...

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Main Authors: Chang-Ming Wang, Nicolas Tancogne-Dejean, Massimo Altarelli, Angel Rubio, Shunsuke A. Sato
Format: Article
Language:English
Published: American Physical Society 2020-08-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.2.033333
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author Chang-Ming Wang
Nicolas Tancogne-Dejean
Massimo Altarelli
Angel Rubio
Shunsuke A. Sato
author_facet Chang-Ming Wang
Nicolas Tancogne-Dejean
Massimo Altarelli
Angel Rubio
Shunsuke A. Sato
author_sort Chang-Ming Wang
collection DOAJ
description We extend the semiclassical trajectory description for the high-order harmonic generation (HHG) from solids by integrating the effect of electron-scattering. Comparing the extended semiclassical trajectory model with a one-dimensional quantum mechanical simulation, we find that the multiplateau feature of the HHG spectrum is formed by Umklapp scattering under the electron-hole acceleration dynamics by laser fields. Furthermore, by tracing the scattered trajectories in real-space, the model fairly describes the emitted photon energy and the emission timing of the HHG even in the higher plateau regions. We further consider the loss of trajectories by scattering processes with a mean-free-path approximation and evaluate the HHG cutoff energy as a function of laser wavelength. As a result, we find that the trajectory loss by scattering causes the wavelength independence of the HHG from solids.
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spelling doaj.art-f6912e216e9240cbb64ea3b06f4282722024-04-12T16:59:41ZengAmerican Physical SocietyPhysical Review Research2643-15642020-08-012303333310.1103/PhysRevResearch.2.033333Role of electron scattering on the high-order harmonic generation from solidsChang-Ming WangNicolas Tancogne-DejeanMassimo AltarelliAngel RubioShunsuke A. SatoWe extend the semiclassical trajectory description for the high-order harmonic generation (HHG) from solids by integrating the effect of electron-scattering. Comparing the extended semiclassical trajectory model with a one-dimensional quantum mechanical simulation, we find that the multiplateau feature of the HHG spectrum is formed by Umklapp scattering under the electron-hole acceleration dynamics by laser fields. Furthermore, by tracing the scattered trajectories in real-space, the model fairly describes the emitted photon energy and the emission timing of the HHG even in the higher plateau regions. We further consider the loss of trajectories by scattering processes with a mean-free-path approximation and evaluate the HHG cutoff energy as a function of laser wavelength. As a result, we find that the trajectory loss by scattering causes the wavelength independence of the HHG from solids.http://doi.org/10.1103/PhysRevResearch.2.033333
spellingShingle Chang-Ming Wang
Nicolas Tancogne-Dejean
Massimo Altarelli
Angel Rubio
Shunsuke A. Sato
Role of electron scattering on the high-order harmonic generation from solids
Physical Review Research
title Role of electron scattering on the high-order harmonic generation from solids
title_full Role of electron scattering on the high-order harmonic generation from solids
title_fullStr Role of electron scattering on the high-order harmonic generation from solids
title_full_unstemmed Role of electron scattering on the high-order harmonic generation from solids
title_short Role of electron scattering on the high-order harmonic generation from solids
title_sort role of electron scattering on the high order harmonic generation from solids
url http://doi.org/10.1103/PhysRevResearch.2.033333
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