Constraints on interactions between aerosols and clouds on a global scale from a combination of MODIS-CERES satellite data and climate simulations

Satellite-based cloud top effective radius retrieved by the CERES Science Team were combined with simulated aerosol concentrations from CCCma CanAM4 to examine relationships between aerosol and cloud that underlie the first aerosol indirect (cloud albedo) effect. Evidence of a strong negative relati...

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Main Authors: X. Ma, K. von Salzen, J. Cole
Format: Article
Language:English
Published: Copernicus Publications 2010-10-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/10/9851/2010/acp-10-9851-2010.pdf
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author X. Ma
K. von Salzen
J. Cole
author_facet X. Ma
K. von Salzen
J. Cole
author_sort X. Ma
collection DOAJ
description Satellite-based cloud top effective radius retrieved by the CERES Science Team were combined with simulated aerosol concentrations from CCCma CanAM4 to examine relationships between aerosol and cloud that underlie the first aerosol indirect (cloud albedo) effect. Evidence of a strong negative relationship between sulphate, and organic aerosols, with cloud top effective radius was found for low clouds, indicating both aerosol types are contributing to the first indirect effect on a global scale. Furthermore, effects of aerosol on the cloud droplet effective radius are more pronounced for larger cloud liquid water paths. While CanAM4 broadly reproduces the observed relationship between sulphate aerosols and cloud droplets, it does not reproduce the dependency of cloud top droplet size on organic aerosol concentrations nor the dependency on cloud liquid water path. Simulations with a modified version of the model yield a more realistic dependency of cloud droplets on organic carbon. The robustness of the methods used in the study are investigated by repeating the analysis using aerosol simulated by the GOCART model and cloud top effective radii derived from the MODIS Science Team.
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spelling doaj.art-f6f1dbc0938d4fd1b40819b2068d1d552022-12-21T19:12:19ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242010-10-0110209851986110.5194/acp-10-9851-2010Constraints on interactions between aerosols and clouds on a global scale from a combination of MODIS-CERES satellite data and climate simulationsX. MaK. von SalzenJ. ColeSatellite-based cloud top effective radius retrieved by the CERES Science Team were combined with simulated aerosol concentrations from CCCma CanAM4 to examine relationships between aerosol and cloud that underlie the first aerosol indirect (cloud albedo) effect. Evidence of a strong negative relationship between sulphate, and organic aerosols, with cloud top effective radius was found for low clouds, indicating both aerosol types are contributing to the first indirect effect on a global scale. Furthermore, effects of aerosol on the cloud droplet effective radius are more pronounced for larger cloud liquid water paths. While CanAM4 broadly reproduces the observed relationship between sulphate aerosols and cloud droplets, it does not reproduce the dependency of cloud top droplet size on organic aerosol concentrations nor the dependency on cloud liquid water path. Simulations with a modified version of the model yield a more realistic dependency of cloud droplets on organic carbon. The robustness of the methods used in the study are investigated by repeating the analysis using aerosol simulated by the GOCART model and cloud top effective radii derived from the MODIS Science Team.http://www.atmos-chem-phys.net/10/9851/2010/acp-10-9851-2010.pdf
spellingShingle X. Ma
K. von Salzen
J. Cole
Constraints on interactions between aerosols and clouds on a global scale from a combination of MODIS-CERES satellite data and climate simulations
Atmospheric Chemistry and Physics
title Constraints on interactions between aerosols and clouds on a global scale from a combination of MODIS-CERES satellite data and climate simulations
title_full Constraints on interactions between aerosols and clouds on a global scale from a combination of MODIS-CERES satellite data and climate simulations
title_fullStr Constraints on interactions between aerosols and clouds on a global scale from a combination of MODIS-CERES satellite data and climate simulations
title_full_unstemmed Constraints on interactions between aerosols and clouds on a global scale from a combination of MODIS-CERES satellite data and climate simulations
title_short Constraints on interactions between aerosols and clouds on a global scale from a combination of MODIS-CERES satellite data and climate simulations
title_sort constraints on interactions between aerosols and clouds on a global scale from a combination of modis ceres satellite data and climate simulations
url http://www.atmos-chem-phys.net/10/9851/2010/acp-10-9851-2010.pdf
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