Linear and Nonlinear Optical Absorption of CdSe/CdS Core/Shell Quantum Dots in the Presence of Donor Impurity

Linear and nonlinear optical properties in colloidal CdSe/CdS core/shell quantum dots with different sizes have been theoretically investigated in the framework of effective mass approximation. The electron states in colloidal CdSe/CdS core/shell quantum dots have been calculated using the finite el...

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Main Authors: Grigor A. Mantashian, Nare A. Zaqaryan, Paytsar A. Mantashyan, Hayk A. Sarkisyan, Sotirios Baskoutas, David B. Hayrapetyan
Format: Article
Language:English
Published: MDPI AG 2021-10-01
Series:Atoms
Subjects:
Online Access:https://www.mdpi.com/2218-2004/9/4/75
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author Grigor A. Mantashian
Nare A. Zaqaryan
Paytsar A. Mantashyan
Hayk A. Sarkisyan
Sotirios Baskoutas
David B. Hayrapetyan
author_facet Grigor A. Mantashian
Nare A. Zaqaryan
Paytsar A. Mantashyan
Hayk A. Sarkisyan
Sotirios Baskoutas
David B. Hayrapetyan
author_sort Grigor A. Mantashian
collection DOAJ
description Linear and nonlinear optical properties in colloidal CdSe/CdS core/shell quantum dots with different sizes have been theoretically investigated in the framework of effective mass approximation. The electron states in colloidal CdSe/CdS core/shell quantum dots have been calculated using the finite element method. The intraband linear and nonlinear absorption spectra have been calculated for colloidal CdSe/CdS core/shell quantum dots with different sizes. In addition, the dependences of the linear and nonlinear refractive index change on the incident light energy have been calculated. In the last section of the paper the second- and third-order harmonic generation spectra have been presented.
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spelling doaj.art-f9e3e0c15515484aa9bd4f0956a28f342023-11-23T03:47:48ZengMDPI AGAtoms2218-20042021-10-01947510.3390/atoms9040075Linear and Nonlinear Optical Absorption of CdSe/CdS Core/Shell Quantum Dots in the Presence of Donor ImpurityGrigor A. Mantashian0Nare A. Zaqaryan1Paytsar A. Mantashyan2Hayk A. Sarkisyan3Sotirios Baskoutas4David B. Hayrapetyan5Department of General Physics and Quantum Nanostructures, Russian-Armenian University, Yerevan 0051, ArmeniaDepartment of General Physics and Quantum Nanostructures, Russian-Armenian University, Yerevan 0051, ArmeniaDepartment of General Physics and Quantum Nanostructures, Russian-Armenian University, Yerevan 0051, ArmeniaDepartment of General Physics and Quantum Nanostructures, Russian-Armenian University, Yerevan 0051, ArmeniaDepartment of Materials Science, University of Patras, GR-26504 Patras, GreeceDepartment of General Physics and Quantum Nanostructures, Russian-Armenian University, Yerevan 0051, ArmeniaLinear and nonlinear optical properties in colloidal CdSe/CdS core/shell quantum dots with different sizes have been theoretically investigated in the framework of effective mass approximation. The electron states in colloidal CdSe/CdS core/shell quantum dots have been calculated using the finite element method. The intraband linear and nonlinear absorption spectra have been calculated for colloidal CdSe/CdS core/shell quantum dots with different sizes. In addition, the dependences of the linear and nonlinear refractive index change on the incident light energy have been calculated. In the last section of the paper the second- and third-order harmonic generation spectra have been presented.https://www.mdpi.com/2218-2004/9/4/75CdSe/CdS core/shell quantum dotlinear and nonlinear absorptionintraband absorptionrefractive index changesecond- and third-order harmonic generation
spellingShingle Grigor A. Mantashian
Nare A. Zaqaryan
Paytsar A. Mantashyan
Hayk A. Sarkisyan
Sotirios Baskoutas
David B. Hayrapetyan
Linear and Nonlinear Optical Absorption of CdSe/CdS Core/Shell Quantum Dots in the Presence of Donor Impurity
Atoms
CdSe/CdS core/shell quantum dot
linear and nonlinear absorption
intraband absorption
refractive index change
second- and third-order harmonic generation
title Linear and Nonlinear Optical Absorption of CdSe/CdS Core/Shell Quantum Dots in the Presence of Donor Impurity
title_full Linear and Nonlinear Optical Absorption of CdSe/CdS Core/Shell Quantum Dots in the Presence of Donor Impurity
title_fullStr Linear and Nonlinear Optical Absorption of CdSe/CdS Core/Shell Quantum Dots in the Presence of Donor Impurity
title_full_unstemmed Linear and Nonlinear Optical Absorption of CdSe/CdS Core/Shell Quantum Dots in the Presence of Donor Impurity
title_short Linear and Nonlinear Optical Absorption of CdSe/CdS Core/Shell Quantum Dots in the Presence of Donor Impurity
title_sort linear and nonlinear optical absorption of cdse cds core shell quantum dots in the presence of donor impurity
topic CdSe/CdS core/shell quantum dot
linear and nonlinear absorption
intraband absorption
refractive index change
second- and third-order harmonic generation
url https://www.mdpi.com/2218-2004/9/4/75
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