The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring
Single-atom catalysts maximize atom usage within supports, but preparations can be complex. Here, authors show a facile impregnation-adsorption method to attach single noble-metal atoms to N-doped porous carbon and demonstrate strong electrocatalytic hydrogen evolution performances for Pt catalysts.
| Main Authors: | , , , , , , , , , , , , , |
|---|---|
| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2019-04-01
|
| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-019-09596-x |
| _version_ | 1818342737741611008 |
|---|---|
| author | Zhiqi Zhang Yugang Chen Liqi Zhou Chi Chen Zhen Han Bingsen Zhang Qiang Wu Lijun Yang Lingyu Du Yongfeng Bu Peng Wang Xizhang Wang Hui Yang Zheng Hu |
| author_facet | Zhiqi Zhang Yugang Chen Liqi Zhou Chi Chen Zhen Han Bingsen Zhang Qiang Wu Lijun Yang Lingyu Du Yongfeng Bu Peng Wang Xizhang Wang Hui Yang Zheng Hu |
| author_sort | Zhiqi Zhang |
| collection | DOAJ |
| description | Single-atom catalysts maximize atom usage within supports, but preparations can be complex. Here, authors show a facile impregnation-adsorption method to attach single noble-metal atoms to N-doped porous carbon and demonstrate strong electrocatalytic hydrogen evolution performances for Pt catalysts. |
| first_indexed | 2024-12-13T16:19:27Z |
| format | Article |
| id | doaj.art-fc336d38f8944fe5a236c875eb0a9ced |
| institution | Directory Open Access Journal |
| issn | 2041-1723 |
| language | English |
| last_indexed | 2024-12-13T16:19:27Z |
| publishDate | 2019-04-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj.art-fc336d38f8944fe5a236c875eb0a9ced2022-12-21T23:38:45ZengNature PortfolioNature Communications2041-17232019-04-011011710.1038/s41467-019-09596-xThe simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoringZhiqi Zhang0Yugang Chen1Liqi Zhou2Chi Chen3Zhen Han4Bingsen Zhang5Qiang Wu6Lijun Yang7Lingyu Du8Yongfeng Bu9Peng Wang10Xizhang Wang11Hui Yang12Zheng Hu13Key Laboratory of Mesoscopic Chemistry of MOE and Jiangsu Provincial Lab for Nanotechnology, School of Chemistry and Chemical Engineering, Nanjing UniversityKey Laboratory of Mesoscopic Chemistry of MOE and Jiangsu Provincial Lab for Nanotechnology, School of Chemistry and Chemical Engineering, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityShanghai Advanced Research Institute, Chinese Academy of SciencesNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityShenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of SciencesKey Laboratory of Mesoscopic Chemistry of MOE and Jiangsu Provincial Lab for Nanotechnology, School of Chemistry and Chemical Engineering, Nanjing UniversityKey Laboratory of Mesoscopic Chemistry of MOE and Jiangsu Provincial Lab for Nanotechnology, School of Chemistry and Chemical Engineering, Nanjing UniversityKey Laboratory of Mesoscopic Chemistry of MOE and Jiangsu Provincial Lab for Nanotechnology, School of Chemistry and Chemical Engineering, Nanjing UniversityKey Laboratory of Mesoscopic Chemistry of MOE and Jiangsu Provincial Lab for Nanotechnology, School of Chemistry and Chemical Engineering, Nanjing UniversityNational Laboratory of Solid State Microstructures, College of Engineering and Applied Sciences, and Collaborative Innovation Center of Advanced Microstructures, Nanjing UniversityKey Laboratory of Mesoscopic Chemistry of MOE and Jiangsu Provincial Lab for Nanotechnology, School of Chemistry and Chemical Engineering, Nanjing UniversityShanghai Advanced Research Institute, Chinese Academy of SciencesKey Laboratory of Mesoscopic Chemistry of MOE and Jiangsu Provincial Lab for Nanotechnology, School of Chemistry and Chemical Engineering, Nanjing UniversitySingle-atom catalysts maximize atom usage within supports, but preparations can be complex. Here, authors show a facile impregnation-adsorption method to attach single noble-metal atoms to N-doped porous carbon and demonstrate strong electrocatalytic hydrogen evolution performances for Pt catalysts.https://doi.org/10.1038/s41467-019-09596-x |
| spellingShingle | Zhiqi Zhang Yugang Chen Liqi Zhou Chi Chen Zhen Han Bingsen Zhang Qiang Wu Lijun Yang Lingyu Du Yongfeng Bu Peng Wang Xizhang Wang Hui Yang Zheng Hu The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring Nature Communications |
| title | The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring |
| title_full | The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring |
| title_fullStr | The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring |
| title_full_unstemmed | The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring |
| title_short | The simplest construction of single-site catalysts by the synergism of micropore trapping and nitrogen anchoring |
| title_sort | simplest construction of single site catalysts by the synergism of micropore trapping and nitrogen anchoring |
| url | https://doi.org/10.1038/s41467-019-09596-x |
| work_keys_str_mv | AT zhiqizhang thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT yugangchen thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT liqizhou thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT chichen thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT zhenhan thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT bingsenzhang thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT qiangwu thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT lijunyang thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT lingyudu thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT yongfengbu thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT pengwang thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT xizhangwang thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT huiyang thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT zhenghu thesimplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT zhiqizhang simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT yugangchen simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT liqizhou simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT chichen simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT zhenhan simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT bingsenzhang simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT qiangwu simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT lijunyang simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT lingyudu simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT yongfengbu simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT pengwang simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT xizhangwang simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT huiyang simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring AT zhenghu simplestconstructionofsinglesitecatalystsbythesynergismofmicroporetrappingandnitrogenanchoring |