Multiscale Fabrication Process Optimization of DFB Cavities for Organic Laser Diodes

In the context of the quest for the Organic Laser Diode, we present the multiscale fabrication process optimization of mixed-order distributed-feedback micro-cavities integrated in nanosecond-short electrical pulse-ready organic light-emitting diodes (OLEDs). We combine ultra-short pulsed electrical...

Full description

Bibliographic Details
Main Authors: Amani Ouirimi, Alex Chamberlain Chime, Nixson Loganathan, Mahmoud Chakaroun, Quentin Gaimard, Alexis P. A. Fischer
Format: Article
Language:English
Published: MDPI AG 2024-02-01
Series:Micromachines
Subjects:
Online Access:https://www.mdpi.com/2072-666X/15/2/260
_version_ 1797297514609639424
author Amani Ouirimi
Alex Chamberlain Chime
Nixson Loganathan
Mahmoud Chakaroun
Quentin Gaimard
Alexis P. A. Fischer
author_facet Amani Ouirimi
Alex Chamberlain Chime
Nixson Loganathan
Mahmoud Chakaroun
Quentin Gaimard
Alexis P. A. Fischer
author_sort Amani Ouirimi
collection DOAJ
description In the context of the quest for the Organic Laser Diode, we present the multiscale fabrication process optimization of mixed-order distributed-feedback micro-cavities integrated in nanosecond-short electrical pulse-ready organic light-emitting diodes (OLEDs). We combine ultra-short pulsed electrical excitation and laser micro-cavities. This requires the integration of a highly resolved DFB micro-cavity with an OLED stack and with microwave electrodes. In a second challenge, we tune the cavity resonance precisely to the electroluminescence peak of the organic laser gain medium. This requires precise micro-cavity fabrication performed using e-beam lithography to pattern gratings with a precision in the nanometer scale. Optimal DFB micro-cavities are obtained with 300 nm thick hydrogen silsesquioxane negative-tone e-beam resist on 50 nm thin indium tin oxide anode exposed with a charge quantity per area (i.e., dose) of 620 µC/cm<sup>2</sup>, developed over 40 min in tetramethylammonium hydroxide diluted in water. We show that the integration of the DFB micro-cavity does not hinder the pulsed electrical operability of the device, which exhibits a peak current density as high as 14 kA/cm<sup>2</sup>.
first_indexed 2024-03-07T22:21:24Z
format Article
id doaj.art-fcd045d4dc7d4e7a8fe995127dda744b
institution Directory Open Access Journal
issn 2072-666X
language English
last_indexed 2024-03-07T22:21:24Z
publishDate 2024-02-01
publisher MDPI AG
record_format Article
series Micromachines
spelling doaj.art-fcd045d4dc7d4e7a8fe995127dda744b2024-02-23T15:27:49ZengMDPI AGMicromachines2072-666X2024-02-0115226010.3390/mi15020260Multiscale Fabrication Process Optimization of DFB Cavities for Organic Laser DiodesAmani Ouirimi0Alex Chamberlain Chime1Nixson Loganathan2Mahmoud Chakaroun3Quentin Gaimard4Alexis P. A. Fischer5Laboratoire de Physique des Lasers, UMR CNRS 7538, Université Sorbonne Paris Nord, 99 Avenue JB Clément, 93430 Villetaneuse, FranceLaboratoire de Physique des Lasers, UMR CNRS 7538, Université Sorbonne Paris Nord, 99 Avenue JB Clément, 93430 Villetaneuse, FranceCentrale de Proximité en Nanotechnologies de Paris Nord, Université Sorbonne Paris Nord, 99 Avenue JB Clément, 93430 Villetaneuse, FranceLaboratoire de Physique des Lasers, UMR CNRS 7538, Université Sorbonne Paris Nord, 99 Avenue JB Clément, 93430 Villetaneuse, FranceLaboratoire de Physique des Lasers, UMR CNRS 7538, Université Sorbonne Paris Nord, 99 Avenue JB Clément, 93430 Villetaneuse, FranceLaboratoire de Physique des Lasers, UMR CNRS 7538, Université Sorbonne Paris Nord, 99 Avenue JB Clément, 93430 Villetaneuse, FranceIn the context of the quest for the Organic Laser Diode, we present the multiscale fabrication process optimization of mixed-order distributed-feedback micro-cavities integrated in nanosecond-short electrical pulse-ready organic light-emitting diodes (OLEDs). We combine ultra-short pulsed electrical excitation and laser micro-cavities. This requires the integration of a highly resolved DFB micro-cavity with an OLED stack and with microwave electrodes. In a second challenge, we tune the cavity resonance precisely to the electroluminescence peak of the organic laser gain medium. This requires precise micro-cavity fabrication performed using e-beam lithography to pattern gratings with a precision in the nanometer scale. Optimal DFB micro-cavities are obtained with 300 nm thick hydrogen silsesquioxane negative-tone e-beam resist on 50 nm thin indium tin oxide anode exposed with a charge quantity per area (i.e., dose) of 620 µC/cm<sup>2</sup>, developed over 40 min in tetramethylammonium hydroxide diluted in water. We show that the integration of the DFB micro-cavity does not hinder the pulsed electrical operability of the device, which exhibits a peak current density as high as 14 kA/cm<sup>2</sup>.https://www.mdpi.com/2072-666X/15/2/260OLEDmicro-cavityDFBe-beam lithographyprocess optimizationOLD
spellingShingle Amani Ouirimi
Alex Chamberlain Chime
Nixson Loganathan
Mahmoud Chakaroun
Quentin Gaimard
Alexis P. A. Fischer
Multiscale Fabrication Process Optimization of DFB Cavities for Organic Laser Diodes
Micromachines
OLED
micro-cavity
DFB
e-beam lithography
process optimization
OLD
title Multiscale Fabrication Process Optimization of DFB Cavities for Organic Laser Diodes
title_full Multiscale Fabrication Process Optimization of DFB Cavities for Organic Laser Diodes
title_fullStr Multiscale Fabrication Process Optimization of DFB Cavities for Organic Laser Diodes
title_full_unstemmed Multiscale Fabrication Process Optimization of DFB Cavities for Organic Laser Diodes
title_short Multiscale Fabrication Process Optimization of DFB Cavities for Organic Laser Diodes
title_sort multiscale fabrication process optimization of dfb cavities for organic laser diodes
topic OLED
micro-cavity
DFB
e-beam lithography
process optimization
OLD
url https://www.mdpi.com/2072-666X/15/2/260
work_keys_str_mv AT amaniouirimi multiscalefabricationprocessoptimizationofdfbcavitiesfororganiclaserdiodes
AT alexchamberlainchime multiscalefabricationprocessoptimizationofdfbcavitiesfororganiclaserdiodes
AT nixsonloganathan multiscalefabricationprocessoptimizationofdfbcavitiesfororganiclaserdiodes
AT mahmoudchakaroun multiscalefabricationprocessoptimizationofdfbcavitiesfororganiclaserdiodes
AT quentingaimard multiscalefabricationprocessoptimizationofdfbcavitiesfororganiclaserdiodes
AT alexispafischer multiscalefabricationprocessoptimizationofdfbcavitiesfororganiclaserdiodes