Recent Progress in the Use of Perovskites for Electrochemical, Photoelectrochemical, and Photovoltaic–Electrochemical CO<sub>2</sub> Reduction
Developing novel functional materials to advance the technological level of clean and renewable energy systems is the focus of much research. Due to their outstanding operational and compositional properties, perovskite-based structures have already been studied as an important class of solid-state...
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MDPI AG
2023-11-01
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| Series: | Energies |
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| Online Access: | https://www.mdpi.com/1996-1073/16/22/7632 |
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| author | Mina Ahmadi-Kashani Mahmoud Zendehdel Luigi Schirone Mohammad Mahdi Abolhasani Narges Yaghoobi Nia |
| author_facet | Mina Ahmadi-Kashani Mahmoud Zendehdel Luigi Schirone Mohammad Mahdi Abolhasani Narges Yaghoobi Nia |
| author_sort | Mina Ahmadi-Kashani |
| collection | DOAJ |
| description | Developing novel functional materials to advance the technological level of clean and renewable energy systems is the focus of much research. Due to their outstanding operational and compositional properties, perovskite-based structures have already been studied as an important class of solid-state components for electrochemical (EC), photoelectrochemical (PEC), and photovoltaic–electrochemical (PV-EC) CO<sub>2</sub> reduction, showing great potential in their catalytic activity and device stability and with a promising window for further technological developments. In this review, the different kinds of perovskites in the context of their structural features, which lead to their different applications, are first investigated. Then, we summarize the recent progress in the use of perovskites in EC, PEC, and PV-EC CO<sub>2</sub>-reduction devices. The research demonstrates that the mechanism and kinetics of intermediate formation have a significant effect on the creation of the final product. Investigations show that appropriate surface modifications, such as through the use of doping agents, alloy construction, and composites, can considerably improve the electrocatalytic activity and stability of perovskites. Finally, the perspectives on, and limitations of, the commercial and large-scale production of perovskites for CO<sub>2</sub> reduction are stated. |
| first_indexed | 2024-03-09T16:52:24Z |
| format | Article |
| id | doaj.art-fcfacd9306a745df909ec8f0042f339a |
| institution | Directory Open Access Journal |
| issn | 1996-1073 |
| language | English |
| last_indexed | 2024-03-09T16:52:24Z |
| publishDate | 2023-11-01 |
| publisher | MDPI AG |
| record_format | Article |
| series | Energies |
| spelling | doaj.art-fcfacd9306a745df909ec8f0042f339a2023-11-24T14:40:36ZengMDPI AGEnergies1996-10732023-11-011622763210.3390/en16227632Recent Progress in the Use of Perovskites for Electrochemical, Photoelectrochemical, and Photovoltaic–Electrochemical CO<sub>2</sub> ReductionMina Ahmadi-Kashani0Mahmoud Zendehdel1Luigi Schirone2Mohammad Mahdi Abolhasani3Narges Yaghoobi Nia4Chemical Engineering Department, University of Kashan, Kashan 8731753153, IranKimia Solar Research Institute (K.S.R.I), Kimia Solar Company, Kashan 8713745868, IranSchool of Aerospace Engineering, Sapienza University of Rome, Via Salaria 851, 00138 Rome, ItalyChemical Engineering Department, University of Kashan, Kashan 8731753153, IranSchool of Aerospace Engineering, Sapienza University of Rome, Via Salaria 851, 00138 Rome, ItalyDeveloping novel functional materials to advance the technological level of clean and renewable energy systems is the focus of much research. Due to their outstanding operational and compositional properties, perovskite-based structures have already been studied as an important class of solid-state components for electrochemical (EC), photoelectrochemical (PEC), and photovoltaic–electrochemical (PV-EC) CO<sub>2</sub> reduction, showing great potential in their catalytic activity and device stability and with a promising window for further technological developments. In this review, the different kinds of perovskites in the context of their structural features, which lead to their different applications, are first investigated. Then, we summarize the recent progress in the use of perovskites in EC, PEC, and PV-EC CO<sub>2</sub>-reduction devices. The research demonstrates that the mechanism and kinetics of intermediate formation have a significant effect on the creation of the final product. Investigations show that appropriate surface modifications, such as through the use of doping agents, alloy construction, and composites, can considerably improve the electrocatalytic activity and stability of perovskites. Finally, the perspectives on, and limitations of, the commercial and large-scale production of perovskites for CO<sub>2</sub> reduction are stated.https://www.mdpi.com/1996-1073/16/22/7632perovskiteelectrochemicalphotoelectrochemicalphotovoltaic–electrochemicalCO<sub>2</sub> reduction |
| spellingShingle | Mina Ahmadi-Kashani Mahmoud Zendehdel Luigi Schirone Mohammad Mahdi Abolhasani Narges Yaghoobi Nia Recent Progress in the Use of Perovskites for Electrochemical, Photoelectrochemical, and Photovoltaic–Electrochemical CO<sub>2</sub> Reduction Energies perovskite electrochemical photoelectrochemical photovoltaic–electrochemical CO<sub>2</sub> reduction |
| title | Recent Progress in the Use of Perovskites for Electrochemical, Photoelectrochemical, and Photovoltaic–Electrochemical CO<sub>2</sub> Reduction |
| title_full | Recent Progress in the Use of Perovskites for Electrochemical, Photoelectrochemical, and Photovoltaic–Electrochemical CO<sub>2</sub> Reduction |
| title_fullStr | Recent Progress in the Use of Perovskites for Electrochemical, Photoelectrochemical, and Photovoltaic–Electrochemical CO<sub>2</sub> Reduction |
| title_full_unstemmed | Recent Progress in the Use of Perovskites for Electrochemical, Photoelectrochemical, and Photovoltaic–Electrochemical CO<sub>2</sub> Reduction |
| title_short | Recent Progress in the Use of Perovskites for Electrochemical, Photoelectrochemical, and Photovoltaic–Electrochemical CO<sub>2</sub> Reduction |
| title_sort | recent progress in the use of perovskites for electrochemical photoelectrochemical and photovoltaic electrochemical co sub 2 sub reduction |
| topic | perovskite electrochemical photoelectrochemical photovoltaic–electrochemical CO<sub>2</sub> reduction |
| url | https://www.mdpi.com/1996-1073/16/22/7632 |
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