The effect of hydrogen and oxygen contents on hydride reorientations of zirconium alloy cladding tubes

To investigate the effect of hydrogen and oxygen contents on hydride reorientations during cool-down processes, zirconium–niobium cladding tube specimens were hydrogen-charged before some specimens were oxidized, resulting in 250 ppm and 500 ppm hydrogen-charged specimens containing no oxide and an...

Full description

Bibliographic Details
Main Authors: Hyun-Jin Cha, Ki-Nam Jang, Ji-Hyeong An, Kyu-Tae Kim
Format: Article
Language:English
Published: Elsevier 2015-10-01
Series:Nuclear Engineering and Technology
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S1738573315001552
_version_ 1818484782682603520
author Hyun-Jin Cha
Ki-Nam Jang
Ji-Hyeong An
Kyu-Tae Kim
author_facet Hyun-Jin Cha
Ki-Nam Jang
Ji-Hyeong An
Kyu-Tae Kim
author_sort Hyun-Jin Cha
collection DOAJ
description To investigate the effect of hydrogen and oxygen contents on hydride reorientations during cool-down processes, zirconium–niobium cladding tube specimens were hydrogen-charged before some specimens were oxidized, resulting in 250 ppm and 500 ppm hydrogen-charged specimens containing no oxide and an oxide thickness of 3.8 μm at each surface. The nonoxidized and oxidized hydrogen-charged specimens were heated up to 400°C and then cooled down to room temperature at cooling rates of 0.3°C/min and 8.0°C/min under a tensile hoop stress of 150 MPa. The lower hydrogen contents and the slower cooling rate generated a larger fraction of radial hydrides, a longer radial hydride length, and a lower ultimate tensile strength and plastic elongation. In addition, the oxidized specimens generated a smaller fraction of radial hydrides and a lower ultimate tensile strength and plastic elongation than the nonoxidized specimens. This may be due to: a solubility difference between room temperature and 400°C; an oxygen-induced increase in hydrogen solubility and radial hydride nucleation energy; high temperature residence time during the cool-down; or undissolved circumferential hydrides at 400°C.
first_indexed 2024-12-10T15:59:31Z
format Article
id doaj.art-fd2d5911ad4d43edb99a73c884ad8ecb
institution Directory Open Access Journal
issn 1738-5733
language English
last_indexed 2024-12-10T15:59:31Z
publishDate 2015-10-01
publisher Elsevier
record_format Article
series Nuclear Engineering and Technology
spelling doaj.art-fd2d5911ad4d43edb99a73c884ad8ecb2022-12-22T01:42:32ZengElsevierNuclear Engineering and Technology1738-57332015-10-0147674675510.1016/j.net.2015.06.004The effect of hydrogen and oxygen contents on hydride reorientations of zirconium alloy cladding tubesHyun-Jin ChaKi-Nam JangJi-Hyeong AnKyu-Tae KimTo investigate the effect of hydrogen and oxygen contents on hydride reorientations during cool-down processes, zirconium–niobium cladding tube specimens were hydrogen-charged before some specimens were oxidized, resulting in 250 ppm and 500 ppm hydrogen-charged specimens containing no oxide and an oxide thickness of 3.8 μm at each surface. The nonoxidized and oxidized hydrogen-charged specimens were heated up to 400°C and then cooled down to room temperature at cooling rates of 0.3°C/min and 8.0°C/min under a tensile hoop stress of 150 MPa. The lower hydrogen contents and the slower cooling rate generated a larger fraction of radial hydrides, a longer radial hydride length, and a lower ultimate tensile strength and plastic elongation. In addition, the oxidized specimens generated a smaller fraction of radial hydrides and a lower ultimate tensile strength and plastic elongation than the nonoxidized specimens. This may be due to: a solubility difference between room temperature and 400°C; an oxygen-induced increase in hydrogen solubility and radial hydride nucleation energy; high temperature residence time during the cool-down; or undissolved circumferential hydrides at 400°C.http://www.sciencedirect.com/science/article/pii/S1738573315001552Hydride precipitationHydrogen solubilityMechanical propertyZirconium alloy
spellingShingle Hyun-Jin Cha
Ki-Nam Jang
Ji-Hyeong An
Kyu-Tae Kim
The effect of hydrogen and oxygen contents on hydride reorientations of zirconium alloy cladding tubes
Nuclear Engineering and Technology
Hydride precipitation
Hydrogen solubility
Mechanical property
Zirconium alloy
title The effect of hydrogen and oxygen contents on hydride reorientations of zirconium alloy cladding tubes
title_full The effect of hydrogen and oxygen contents on hydride reorientations of zirconium alloy cladding tubes
title_fullStr The effect of hydrogen and oxygen contents on hydride reorientations of zirconium alloy cladding tubes
title_full_unstemmed The effect of hydrogen and oxygen contents on hydride reorientations of zirconium alloy cladding tubes
title_short The effect of hydrogen and oxygen contents on hydride reorientations of zirconium alloy cladding tubes
title_sort effect of hydrogen and oxygen contents on hydride reorientations of zirconium alloy cladding tubes
topic Hydride precipitation
Hydrogen solubility
Mechanical property
Zirconium alloy
url http://www.sciencedirect.com/science/article/pii/S1738573315001552
work_keys_str_mv AT hyunjincha theeffectofhydrogenandoxygencontentsonhydridereorientationsofzirconiumalloycladdingtubes
AT kinamjang theeffectofhydrogenandoxygencontentsonhydridereorientationsofzirconiumalloycladdingtubes
AT jihyeongan theeffectofhydrogenandoxygencontentsonhydridereorientationsofzirconiumalloycladdingtubes
AT kyutaekim theeffectofhydrogenandoxygencontentsonhydridereorientationsofzirconiumalloycladdingtubes
AT hyunjincha effectofhydrogenandoxygencontentsonhydridereorientationsofzirconiumalloycladdingtubes
AT kinamjang effectofhydrogenandoxygencontentsonhydridereorientationsofzirconiumalloycladdingtubes
AT jihyeongan effectofhydrogenandoxygencontentsonhydridereorientationsofzirconiumalloycladdingtubes
AT kyutaekim effectofhydrogenandoxygencontentsonhydridereorientationsofzirconiumalloycladdingtubes