Influence of layer architecture on fracture toughness and specimen stiffness in polymer multilayer composites

The objective of this contribution was to increase the fracture toughness of talcum reinforced polypropylene (PP) while preserving specimen stiffness. This was accomplished by introducing soft interlayers (ILs) made of standard PP (PP-St) or very compliant PP (PP-Soft) and utilizing the so-called ma...

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Main Authors: Johannes Wiener, Florian Arbeiter, Otmar Kolednik, Gerald Pinter
Format: Article
Language:English
Published: Elsevier 2022-07-01
Series:Materials & Design
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S0264127522004506
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author Johannes Wiener
Florian Arbeiter
Otmar Kolednik
Gerald Pinter
author_facet Johannes Wiener
Florian Arbeiter
Otmar Kolednik
Gerald Pinter
author_sort Johannes Wiener
collection DOAJ
description The objective of this contribution was to increase the fracture toughness of talcum reinforced polypropylene (PP) while preserving specimen stiffness. This was accomplished by introducing soft interlayers (ILs) made of standard PP (PP-St) or very compliant PP (PP-Soft) and utilizing the so-called material inhomogeneity effect. Architectures with one or two ILs of either 0.3 or 0.9 mm thickness were tested in single edge notched bending experiments. Layers of PP-Soft always arrested growing cracks due to their low Young’s modulus, E, and yield stress, σy, which is called an (E-σy)-inhomogeneity. However, the increase in fracture toughness came at the cost of specimen stiffness. For ILs made of PP-St, E was still lower compared to the matrix material, but σy was similar (pure E-inhomogeneity). Specimen stiffness remained high for these composites, but crack arrest could not be achieved in most cases, which could be explained by plastic deformation of the soft layers. Plastic deformation could be contained within the ILs in one of the architectures, where two large ILs were used. Crack arrest could be achieved in this adapted IL design, leading to excellent fracture toughness in combination with high stiffness.
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spelling doaj.art-fdd885120504435ab7af71a4c4fa77292022-12-22T02:38:57ZengElsevierMaterials & Design0264-12752022-07-01219110828Influence of layer architecture on fracture toughness and specimen stiffness in polymer multilayer compositesJohannes Wiener0Florian Arbeiter1Otmar Kolednik2Gerald Pinter3Materials Science and Testing of Polymers, Montanuniversitaet Leoben, 8700 Leoben, AustriaMaterials Science and Testing of Polymers, Montanuniversitaet Leoben, 8700 Leoben, Austria; Corresponding author.Erich-Schmid-Institute of Materials Science, Austrian Academy of Science, 8700 Leoben, AustriaMaterials Science and Testing of Polymers, Montanuniversitaet Leoben, 8700 Leoben, AustriaThe objective of this contribution was to increase the fracture toughness of talcum reinforced polypropylene (PP) while preserving specimen stiffness. This was accomplished by introducing soft interlayers (ILs) made of standard PP (PP-St) or very compliant PP (PP-Soft) and utilizing the so-called material inhomogeneity effect. Architectures with one or two ILs of either 0.3 or 0.9 mm thickness were tested in single edge notched bending experiments. Layers of PP-Soft always arrested growing cracks due to their low Young’s modulus, E, and yield stress, σy, which is called an (E-σy)-inhomogeneity. However, the increase in fracture toughness came at the cost of specimen stiffness. For ILs made of PP-St, E was still lower compared to the matrix material, but σy was similar (pure E-inhomogeneity). Specimen stiffness remained high for these composites, but crack arrest could not be achieved in most cases, which could be explained by plastic deformation of the soft layers. Plastic deformation could be contained within the ILs in one of the architectures, where two large ILs were used. Crack arrest could be achieved in this adapted IL design, leading to excellent fracture toughness in combination with high stiffness.http://www.sciencedirect.com/science/article/pii/S0264127522004506PolypropyleneMultilayerFracture mechanicsBiomimetic designMaterial inhomogeneity effect
spellingShingle Johannes Wiener
Florian Arbeiter
Otmar Kolednik
Gerald Pinter
Influence of layer architecture on fracture toughness and specimen stiffness in polymer multilayer composites
Materials & Design
Polypropylene
Multilayer
Fracture mechanics
Biomimetic design
Material inhomogeneity effect
title Influence of layer architecture on fracture toughness and specimen stiffness in polymer multilayer composites
title_full Influence of layer architecture on fracture toughness and specimen stiffness in polymer multilayer composites
title_fullStr Influence of layer architecture on fracture toughness and specimen stiffness in polymer multilayer composites
title_full_unstemmed Influence of layer architecture on fracture toughness and specimen stiffness in polymer multilayer composites
title_short Influence of layer architecture on fracture toughness and specimen stiffness in polymer multilayer composites
title_sort influence of layer architecture on fracture toughness and specimen stiffness in polymer multilayer composites
topic Polypropylene
Multilayer
Fracture mechanics
Biomimetic design
Material inhomogeneity effect
url http://www.sciencedirect.com/science/article/pii/S0264127522004506
work_keys_str_mv AT johanneswiener influenceoflayerarchitectureonfracturetoughnessandspecimenstiffnessinpolymermultilayercomposites
AT florianarbeiter influenceoflayerarchitectureonfracturetoughnessandspecimenstiffnessinpolymermultilayercomposites
AT otmarkolednik influenceoflayerarchitectureonfracturetoughnessandspecimenstiffnessinpolymermultilayercomposites
AT geraldpinter influenceoflayerarchitectureonfracturetoughnessandspecimenstiffnessinpolymermultilayercomposites