Two-Dimensional Layered Double Hydroxides for Reactions of Methanation and Methane Reforming in C1 Chemistry
CH4 as the paramount ingredient of natural gas plays an eminent role in C1 chemistry. CH4 catalytically converted to syngas is a significant route to transmute methane into high value-added chemicals. Moreover, the CO/CO2 methanation reaction is one of the potent technologies for CO2 valorization an...
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MDPI AG
2018-01-01
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| Series: | Materials |
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| Online Access: | http://www.mdpi.com/1996-1944/11/2/221 |
| _version_ | 1798044755693666304 |
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| author | Panpan Li Feng Yu Naveed Altaf Mingyuan Zhu Jiangbing Li Bin Dai Qiang Wang |
| author_facet | Panpan Li Feng Yu Naveed Altaf Mingyuan Zhu Jiangbing Li Bin Dai Qiang Wang |
| author_sort | Panpan Li |
| collection | DOAJ |
| description | CH4 as the paramount ingredient of natural gas plays an eminent role in C1 chemistry. CH4 catalytically converted to syngas is a significant route to transmute methane into high value-added chemicals. Moreover, the CO/CO2 methanation reaction is one of the potent technologies for CO2 valorization and the coal-derived natural gas production process. Due to the high thermal stability and high extent of dispersion of metallic particles, two-dimensional mixed metal oxides through calcined layered double hydroxides (LDHs) precursors are considered as the suitable supports or catalysts for both the reaction of methanation and methane reforming. The LDHs displayed compositional flexibility, small crystal sizes, high surface area and excellent basic properties. In this paper, we review previous works of LDHs applied in the reaction of both methanation and methane reforming, focus on the LDH-derived catalysts, which exhibit better catalytic performance and thermal stability than conventional catalysts prepared by impregnation method and also discuss the anti-coke ability and anti-sintering ability of LDH-derived catalysts. We believe that LDH-derived catalysts are promising materials in the heterogeneous catalytic field and provide new insight for the design of advance LDH-derived catalysts worthy of future research. |
| first_indexed | 2024-04-11T23:10:29Z |
| format | Article |
| id | doaj.art-feecdb6e92af4f539296980d2028753f |
| institution | Directory Open Access Journal |
| issn | 1996-1944 |
| language | English |
| last_indexed | 2024-04-11T23:10:29Z |
| publishDate | 2018-01-01 |
| publisher | MDPI AG |
| record_format | Article |
| series | Materials |
| spelling | doaj.art-feecdb6e92af4f539296980d2028753f2022-12-22T03:57:53ZengMDPI AGMaterials1996-19442018-01-0111222110.3390/ma11020221ma11020221Two-Dimensional Layered Double Hydroxides for Reactions of Methanation and Methane Reforming in C1 ChemistryPanpan Li0Feng Yu1Naveed Altaf2Mingyuan Zhu3Jiangbing Li4Bin Dai5Qiang Wang6Key Laboratory for Green Processing of Chemical Engineering of Xinjiang Bingtuan, School of Chemistry and Chemical Engineering, Shihezi University, Shihezi 832003, ChinaKey Laboratory for Green Processing of Chemical Engineering of Xinjiang Bingtuan, School of Chemistry and Chemical Engineering, Shihezi University, Shihezi 832003, ChinaEnvironmental Functional Nanomaterials (EFN) Laboratory, College of Environmental Science and Engineering, Beijing Forestry University, Beijing 100083, ChinaKey Laboratory for Green Processing of Chemical Engineering of Xinjiang Bingtuan, School of Chemistry and Chemical Engineering, Shihezi University, Shihezi 832003, ChinaKey Laboratory for Green Processing of Chemical Engineering of Xinjiang Bingtuan, School of Chemistry and Chemical Engineering, Shihezi University, Shihezi 832003, ChinaKey Laboratory for Green Processing of Chemical Engineering of Xinjiang Bingtuan, School of Chemistry and Chemical Engineering, Shihezi University, Shihezi 832003, ChinaKey Laboratory for Green Processing of Chemical Engineering of Xinjiang Bingtuan, School of Chemistry and Chemical Engineering, Shihezi University, Shihezi 832003, ChinaCH4 as the paramount ingredient of natural gas plays an eminent role in C1 chemistry. CH4 catalytically converted to syngas is a significant route to transmute methane into high value-added chemicals. Moreover, the CO/CO2 methanation reaction is one of the potent technologies for CO2 valorization and the coal-derived natural gas production process. Due to the high thermal stability and high extent of dispersion of metallic particles, two-dimensional mixed metal oxides through calcined layered double hydroxides (LDHs) precursors are considered as the suitable supports or catalysts for both the reaction of methanation and methane reforming. The LDHs displayed compositional flexibility, small crystal sizes, high surface area and excellent basic properties. In this paper, we review previous works of LDHs applied in the reaction of both methanation and methane reforming, focus on the LDH-derived catalysts, which exhibit better catalytic performance and thermal stability than conventional catalysts prepared by impregnation method and also discuss the anti-coke ability and anti-sintering ability of LDH-derived catalysts. We believe that LDH-derived catalysts are promising materials in the heterogeneous catalytic field and provide new insight for the design of advance LDH-derived catalysts worthy of future research.http://www.mdpi.com/1996-1944/11/2/221layered double hydroxidestwo-dimensional materialsmethanation reactionmethane reformingC1 chemistry |
| spellingShingle | Panpan Li Feng Yu Naveed Altaf Mingyuan Zhu Jiangbing Li Bin Dai Qiang Wang Two-Dimensional Layered Double Hydroxides for Reactions of Methanation and Methane Reforming in C1 Chemistry Materials layered double hydroxides two-dimensional materials methanation reaction methane reforming C1 chemistry |
| title | Two-Dimensional Layered Double Hydroxides for Reactions of Methanation and Methane Reforming in C1 Chemistry |
| title_full | Two-Dimensional Layered Double Hydroxides for Reactions of Methanation and Methane Reforming in C1 Chemistry |
| title_fullStr | Two-Dimensional Layered Double Hydroxides for Reactions of Methanation and Methane Reforming in C1 Chemistry |
| title_full_unstemmed | Two-Dimensional Layered Double Hydroxides for Reactions of Methanation and Methane Reforming in C1 Chemistry |
| title_short | Two-Dimensional Layered Double Hydroxides for Reactions of Methanation and Methane Reforming in C1 Chemistry |
| title_sort | two dimensional layered double hydroxides for reactions of methanation and methane reforming in c1 chemistry |
| topic | layered double hydroxides two-dimensional materials methanation reaction methane reforming C1 chemistry |
| url | http://www.mdpi.com/1996-1944/11/2/221 |
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