Quintet formation, exchange fluctuations, and the role of stochastic resonance in singlet fission
Quintet formation is a part of a photochemical energy conversion process, which could be exploited to help achieve higher efficiency values for photovoltaics. Here, the authors propose a stochastic and coherent resonance mechanism for formation of the quintet spin state in singlet fission materials,...
| Main Authors: | , , , , |
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| Format: | Article |
| Sprog: | English |
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Nature Portfolio
2023-04-01
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| Serier: | Communications Physics |
| Online adgang: | https://doi.org/10.1038/s42005-023-01177-1 |
| _version_ | 1827970478602452992 |
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| author | Miles I. Collins Francesco Campaioli Murad J. Y. Tayebjee Jared H. Cole Dane R. McCamey |
| author_facet | Miles I. Collins Francesco Campaioli Murad J. Y. Tayebjee Jared H. Cole Dane R. McCamey |
| author_sort | Miles I. Collins |
| collection | DOAJ |
| description | Quintet formation is a part of a photochemical energy conversion process, which could be exploited to help achieve higher efficiency values for photovoltaics. Here, the authors propose a stochastic and coherent resonance mechanism for formation of the quintet spin state in singlet fission materials, that is still viable in the strong-exchange regime. |
| first_indexed | 2024-04-09T18:54:29Z |
| format | Article |
| id | doaj.art-ffc9e87d5ae04582b64a0a785c1b26d6 |
| institution | Directory Open Access Journal |
| issn | 2399-3650 |
| language | English |
| last_indexed | 2024-04-09T18:54:29Z |
| publishDate | 2023-04-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Communications Physics |
| spelling | doaj.art-ffc9e87d5ae04582b64a0a785c1b26d62023-04-09T11:18:30ZengNature PortfolioCommunications Physics2399-36502023-04-01611810.1038/s42005-023-01177-1Quintet formation, exchange fluctuations, and the role of stochastic resonance in singlet fissionMiles I. Collins0Francesco Campaioli1Murad J. Y. Tayebjee2Jared H. Cole3Dane R. McCamey4School of Physics and ARC Centre of Excellence in Exciton Science, UNSW SydneyChemical and Quantum Physics, and ARC Centre of Excellence in Exciton Science, School of Science, RMIT UniversitySchool of Photovoltaic and Renewable Energy Engineering, UNSW SydneyChemical and Quantum Physics, and ARC Centre of Excellence in Exciton Science, School of Science, RMIT UniversitySchool of Physics and ARC Centre of Excellence in Exciton Science, UNSW SydneyQuintet formation is a part of a photochemical energy conversion process, which could be exploited to help achieve higher efficiency values for photovoltaics. Here, the authors propose a stochastic and coherent resonance mechanism for formation of the quintet spin state in singlet fission materials, that is still viable in the strong-exchange regime.https://doi.org/10.1038/s42005-023-01177-1 |
| spellingShingle | Miles I. Collins Francesco Campaioli Murad J. Y. Tayebjee Jared H. Cole Dane R. McCamey Quintet formation, exchange fluctuations, and the role of stochastic resonance in singlet fission Communications Physics |
| title | Quintet formation, exchange fluctuations, and the role of stochastic resonance in singlet fission |
| title_full | Quintet formation, exchange fluctuations, and the role of stochastic resonance in singlet fission |
| title_fullStr | Quintet formation, exchange fluctuations, and the role of stochastic resonance in singlet fission |
| title_full_unstemmed | Quintet formation, exchange fluctuations, and the role of stochastic resonance in singlet fission |
| title_short | Quintet formation, exchange fluctuations, and the role of stochastic resonance in singlet fission |
| title_sort | quintet formation exchange fluctuations and the role of stochastic resonance in singlet fission |
| url | https://doi.org/10.1038/s42005-023-01177-1 |
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