Dynamics of convective dissolution from a migrating current of carbon dioxide

During geologic storage of carbon dioxide (CO[subscript 2]), trapping of the buoyant CO[subscript 2] after injection is essential in order to minimize the risk of leakage into shallower formations through a fracture or abandoned well. Models for the subsurface behavior of the CO[subscript 2] are use...

Full description

Bibliographic Details
Main Authors: Hidalgo, Juan J., MacMinn, Christopher W., Juanes, Ruben
Other Authors: Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
Format: Article
Language:en_US
Published: Elsevier 2016
Online Access:http://hdl.handle.net/1721.1/101652
https://orcid.org/0000-0002-7370-2332
_version_ 1811090461720313856
author Hidalgo, Juan J.
MacMinn, Christopher W.
Juanes, Ruben
author2 Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
author_facet Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
Hidalgo, Juan J.
MacMinn, Christopher W.
Juanes, Ruben
author_sort Hidalgo, Juan J.
collection MIT
description During geologic storage of carbon dioxide (CO[subscript 2]), trapping of the buoyant CO[subscript 2] after injection is essential in order to minimize the risk of leakage into shallower formations through a fracture or abandoned well. Models for the subsurface behavior of the CO[subscript 2] are useful for the design, implementation, and long-term monitoring of injection sites, but traditional reservoir-simulation tools are currently unable to resolve the impact of small-scale trapping processes on fluid flow at the scale of a geologic basin. Here, we study the impact of solubility trapping from convective dissolution on the up-dip migration of a buoyant gravity current in a sloping aquifer. To do so, we conduct high-resolution numerical simulations of the gravity current that forms from a pair of miscible analogue fluids. Our simulations fully resolve the dense, sinking fingers that drive the convective dissolution process. We analyze the dynamics of the dissolution flux along the moving CO[subscript 2]–brine interface, including its decay as dissolved buoyant fluid accumulates beneath the buoyant current. We show that the dynamics of the dissolution flux and the macroscopic features of the migrating current can be captured with an upscaled sharp-interface model.
first_indexed 2024-09-23T14:46:32Z
format Article
id mit-1721.1/101652
institution Massachusetts Institute of Technology
language en_US
last_indexed 2024-09-23T14:46:32Z
publishDate 2016
publisher Elsevier
record_format dspace
spelling mit-1721.1/1016522022-09-29T10:29:42Z Dynamics of convective dissolution from a migrating current of carbon dioxide Hidalgo, Juan J. MacMinn, Christopher W. Juanes, Ruben Massachusetts Institute of Technology. Department of Civil and Environmental Engineering Juanes, Ruben Hidalgo, Juan J. Juanes, Ruben During geologic storage of carbon dioxide (CO[subscript 2]), trapping of the buoyant CO[subscript 2] after injection is essential in order to minimize the risk of leakage into shallower formations through a fracture or abandoned well. Models for the subsurface behavior of the CO[subscript 2] are useful for the design, implementation, and long-term monitoring of injection sites, but traditional reservoir-simulation tools are currently unable to resolve the impact of small-scale trapping processes on fluid flow at the scale of a geologic basin. Here, we study the impact of solubility trapping from convective dissolution on the up-dip migration of a buoyant gravity current in a sloping aquifer. To do so, we conduct high-resolution numerical simulations of the gravity current that forms from a pair of miscible analogue fluids. Our simulations fully resolve the dense, sinking fingers that drive the convective dissolution process. We analyze the dynamics of the dissolution flux along the moving CO[subscript 2]–brine interface, including its decay as dissolved buoyant fluid accumulates beneath the buoyant current. We show that the dynamics of the dissolution flux and the macroscopic features of the migrating current can be captured with an upscaled sharp-interface model. Seventh Framework Programme (European Commission) (CO2-MATE Project PIOF-GA-2009-253678) Seventh Framework Programme (European Commission) (Project PANACEA Grant Agreement 282900) United States. Dept. of Energy (DE-FE0009738) 2016-03-10T01:45:45Z 2016-03-10T01:45:45Z 2013-07 Article http://purl.org/eprint/type/JournalArticle 03091708 http://hdl.handle.net/1721.1/101652 Hidalgo, Juan J., Christopher W. MacMinn, and Ruben Juanes. “Dynamics of Convective Dissolution from a Migrating Current of Carbon Dioxide.” Advances in Water Resources 62 (December 2013): 511–519. © 2013 Elsevier Ltd. https://orcid.org/0000-0002-7370-2332 en_US http://dx.doi.org/10.1016/j.advwatres.2013.06.013 Advances in Water Resources Creative Commons Attribution-NonCommercial-NoDerivs License http://creativecommons.org/licenses/by-nc-nd/4.0/ application/pdf Elsevier Prof. Juanes
spellingShingle Hidalgo, Juan J.
MacMinn, Christopher W.
Juanes, Ruben
Dynamics of convective dissolution from a migrating current of carbon dioxide
title Dynamics of convective dissolution from a migrating current of carbon dioxide
title_full Dynamics of convective dissolution from a migrating current of carbon dioxide
title_fullStr Dynamics of convective dissolution from a migrating current of carbon dioxide
title_full_unstemmed Dynamics of convective dissolution from a migrating current of carbon dioxide
title_short Dynamics of convective dissolution from a migrating current of carbon dioxide
title_sort dynamics of convective dissolution from a migrating current of carbon dioxide
url http://hdl.handle.net/1721.1/101652
https://orcid.org/0000-0002-7370-2332
work_keys_str_mv AT hidalgojuanj dynamicsofconvectivedissolutionfromamigratingcurrentofcarbondioxide
AT macminnchristopherw dynamicsofconvectivedissolutionfromamigratingcurrentofcarbondioxide
AT juanesruben dynamicsofconvectivedissolutionfromamigratingcurrentofcarbondioxide