Polarized neutron scattering studies of the kagome lattice antiferromagnet KFe[subscript 3](OH)[subscript 6](SO[subscript 4])[subscript 2]

We report polarized neutron scattering studies of spin-wave excitations and spin fluctuations in the S = 5/2 kagome lattice antiferromagnet KFe[subscript 3](OH)[subscript 6](SO[subscript 4])[subscript 2] (jarosite). Inelastic polarized neutron scattering measurements at 10 K on a single crystal samp...

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Bibliographic Details
Main Authors: Grohol, D., Wakimoto, S., Kakurai, K., Matan, Kittiwit, Helton, Joel S., Nocera, Daniel G., Lee, Young S.
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Language:en_US
Published: Elsevier 2016
Online Access:http://hdl.handle.net/1721.1/102198
https://orcid.org/0000-0002-4507-1115
https://orcid.org/0000-0002-7022-8313
Description
Summary:We report polarized neutron scattering studies of spin-wave excitations and spin fluctuations in the S = 5/2 kagome lattice antiferromagnet KFe[subscript 3](OH)[subscript 6](SO[subscript 4])[subscript 2] (jarosite). Inelastic polarized neutron scattering measurements at 10 K on a single crystal sample reveal two spin gaps, associated with in-plane and out-of-plane excitations. The polarization analysis of quasi-elastic scattering at 67 K shows in-plane spin fluctuations with XY symmetry, consistent with the disappearance of the in-plane gap above the Neel temperature T[subscript N] = 65 K. Our results suggest that jarosite is a promising candidate for studying the 2D XY universality class in magnetic systems.