Reconfigurable optical assembly of nanostructures

Arrangements of nanostructures in well-defined patterns are the basis of photonic crystals, metamaterials and holograms. Furthermore, rewritable optical materials can be achieved by dynamically manipulating nanoassemblies. Here we demonstrate a mechanism to configure plasmonic nanoparticles (NPs) in...

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Main Authors: Montelongo, Yunuen, Yetisen, Ali K., Butt, Haider, Yun, Seok Hyun (Andy)
Other Authors: Harvard University--MIT Division of Health Sciences and Technology
Format: Article
Language:en_US
Published: Nature Publishing Group 2017
Online Access:http://hdl.handle.net/1721.1/106588
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author Montelongo, Yunuen
Yetisen, Ali K.
Butt, Haider
Yun, Seok Hyun (Andy)
author2 Harvard University--MIT Division of Health Sciences and Technology
author_facet Harvard University--MIT Division of Health Sciences and Technology
Montelongo, Yunuen
Yetisen, Ali K.
Butt, Haider
Yun, Seok Hyun (Andy)
author_sort Montelongo, Yunuen
collection MIT
description Arrangements of nanostructures in well-defined patterns are the basis of photonic crystals, metamaterials and holograms. Furthermore, rewritable optical materials can be achieved by dynamically manipulating nanoassemblies. Here we demonstrate a mechanism to configure plasmonic nanoparticles (NPs) in polymer media using nanosecond laser pulses. The mechanism relies on optical forces produced by the interference of laser beams, which allow NPs to migrate to lower-energy configurations. The resulting NP arrangements are stable without any external energy source, but erasable and rewritable by additional recording pulses. We demonstrate reconfigurable optical elements including multilayer Bragg diffraction gratings, volumetric photonic crystals and lenses, as well as dynamic holograms of three-dimensional virtual objects. We aim to expand the applications of optical forces, which have been mostly restricted to optical tweezers. Holographic assemblies of nanoparticles will allow a new generation of programmable composites for tunable metamaterials, data storage devices, sensors and displays.
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spelling mit-1721.1/1065882022-10-01T21:36:55Z Reconfigurable optical assembly of nanostructures Montelongo, Yunuen Yetisen, Ali K. Butt, Haider Yun, Seok Hyun (Andy) Harvard University--MIT Division of Health Sciences and Technology Yun, Seok Hyun (Andy) Arrangements of nanostructures in well-defined patterns are the basis of photonic crystals, metamaterials and holograms. Furthermore, rewritable optical materials can be achieved by dynamically manipulating nanoassemblies. Here we demonstrate a mechanism to configure plasmonic nanoparticles (NPs) in polymer media using nanosecond laser pulses. The mechanism relies on optical forces produced by the interference of laser beams, which allow NPs to migrate to lower-energy configurations. The resulting NP arrangements are stable without any external energy source, but erasable and rewritable by additional recording pulses. We demonstrate reconfigurable optical elements including multilayer Bragg diffraction gratings, volumetric photonic crystals and lenses, as well as dynamic holograms of three-dimensional virtual objects. We aim to expand the applications of optical forces, which have been mostly restricted to optical tweezers. Holographic assemblies of nanoparticles will allow a new generation of programmable composites for tunable metamaterials, data storage devices, sensors and displays. 2017-01-23T19:13:20Z 2017-01-23T19:13:20Z 2016-06 2015-11 Article http://purl.org/eprint/type/JournalArticle 2041-1723 http://hdl.handle.net/1721.1/106588 Montelongo, Yunuen et al. “Reconfigurable Optical Assembly of Nanostructures.” Nature Communications 7 (2016): 12002. © 2016 Macmillan Publishers Limited en_US http://dx.doi.org/10.1038/ncomms12002 Nature Communications Creative Commons Attribution 4.0 International License http://creativecommons.org/licenses/by/4.0/ application/pdf Nature Publishing Group Nature
spellingShingle Montelongo, Yunuen
Yetisen, Ali K.
Butt, Haider
Yun, Seok Hyun (Andy)
Reconfigurable optical assembly of nanostructures
title Reconfigurable optical assembly of nanostructures
title_full Reconfigurable optical assembly of nanostructures
title_fullStr Reconfigurable optical assembly of nanostructures
title_full_unstemmed Reconfigurable optical assembly of nanostructures
title_short Reconfigurable optical assembly of nanostructures
title_sort reconfigurable optical assembly of nanostructures
url http://hdl.handle.net/1721.1/106588
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