Time-resolved, dual heterodyne phase collection transient grating spectroscopy

The application of optical heterodyne detection for transient grating spectroscopy (TGS) using a fixed, binary phase mask often relies on taking the difference between signals captured at multiple heterodyne phases. To date, this has been accomplished by manually controlling the heterodyne phase bet...

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Main Authors: Dennett, Cody Andrew, Short, Michael P
Other Authors: Massachusetts Institute of Technology. Department of Materials Science and Engineering
Format: Article
Language:en_US
Published: American Institute of Physics (AIP) 2017
Online Access:http://hdl.handle.net/1721.1/109513
https://orcid.org/0000-0003-2989-9550
https://orcid.org/0000-0002-9216-2482
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author Dennett, Cody Andrew
Short, Michael P
author2 Massachusetts Institute of Technology. Department of Materials Science and Engineering
author_facet Massachusetts Institute of Technology. Department of Materials Science and Engineering
Dennett, Cody Andrew
Short, Michael P
author_sort Dennett, Cody Andrew
collection MIT
description The application of optical heterodyne detection for transient grating spectroscopy (TGS) using a fixed, binary phase mask often relies on taking the difference between signals captured at multiple heterodyne phases. To date, this has been accomplished by manually controlling the heterodyne phase between measurements with an optical flat. In this letter, an optical configuration is presented which allows for collection of TGS measurements at two heterodyne phases concurrently through the use of two independently phase controlled interrogation paths. This arrangement allows for complete, heterodyne amplified TGS measurements to be made in a manner not constrained by a mechanical actuation time. Measurements are instead constrained only by the desired signal-to-noise ratio. A temporal resolution of between 1 and 10 s, demonstrated here on single crystal metallic samples, will allow TGS experiments to be used as an in-situ, time-resolved monitoring technique for many material processing applications.
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spelling mit-1721.1/1095132022-09-30T16:48:05Z Time-resolved, dual heterodyne phase collection transient grating spectroscopy Dennett, Cody Andrew Short, Michael P Massachusetts Institute of Technology. Department of Materials Science and Engineering Massachusetts Institute of Technology. Department of Nuclear Science and Engineering Short, Michael Dennett, Cody Andrew Short, Michael P The application of optical heterodyne detection for transient grating spectroscopy (TGS) using a fixed, binary phase mask often relies on taking the difference between signals captured at multiple heterodyne phases. To date, this has been accomplished by manually controlling the heterodyne phase between measurements with an optical flat. In this letter, an optical configuration is presented which allows for collection of TGS measurements at two heterodyne phases concurrently through the use of two independently phase controlled interrogation paths. This arrangement allows for complete, heterodyne amplified TGS measurements to be made in a manner not constrained by a mechanical actuation time. Measurements are instead constrained only by the desired signal-to-noise ratio. A temporal resolution of between 1 and 10 s, demonstrated here on single crystal metallic samples, will allow TGS experiments to be used as an in-situ, time-resolved monitoring technique for many material processing applications. National Science Foundation (U.S.) (Graduate Research Fellowship under Grant No. 1122374) United States. National Nuclear Security Administration (Stewardship Science Graduate Fellowship under cooperative agreement No. DE-NA000213) SUTD-MIT International Design Centre (IDC) U.S. Nuclear Regulatory Commission (MIT Nuclear Education Faculty Development Program under Grant No. NRC-HQ-84-15-G-0045) 2017-06-01T18:12:46Z 2017-06-01T18:12:46Z 2017-05 2017-03 Article http://purl.org/eprint/type/JournalArticle 0003-6951 1077-3118 http://hdl.handle.net/1721.1/109513 Dennett, Cody A., and Michael P. Short. “Time-Resolved, Dual Heterodyne Phase Collection Transient Grating Spectroscopy.” Applied Physics Letters 110, no. 21 (May 22, 2017): 211106. https://orcid.org/0000-0003-2989-9550 https://orcid.org/0000-0002-9216-2482 en_US http://dx.doi.org/10.1063/1.4983716 Applied Physics Letters Creative Commons Attribution 4.0 International License http://creativecommons.org/licenses/by/4.0/ application/pdf American Institute of Physics (AIP) American Institute of Physics (AIP)
spellingShingle Dennett, Cody Andrew
Short, Michael P
Time-resolved, dual heterodyne phase collection transient grating spectroscopy
title Time-resolved, dual heterodyne phase collection transient grating spectroscopy
title_full Time-resolved, dual heterodyne phase collection transient grating spectroscopy
title_fullStr Time-resolved, dual heterodyne phase collection transient grating spectroscopy
title_full_unstemmed Time-resolved, dual heterodyne phase collection transient grating spectroscopy
title_short Time-resolved, dual heterodyne phase collection transient grating spectroscopy
title_sort time resolved dual heterodyne phase collection transient grating spectroscopy
url http://hdl.handle.net/1721.1/109513
https://orcid.org/0000-0003-2989-9550
https://orcid.org/0000-0002-9216-2482
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