Highly tensile-strained Ge/InAlAs nanocomposites

Self-assembled nanocomposites have been extensively investigated due to the novel properties that can emerge when multiple material phases are combined. Growth of epitaxial nanocomposites using lattice-mismatched constituents also enables strain-engineering, which can be used to further enhance mate...

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Main Authors: Jung, Daehwan, Faucher, Joseph, Mukherjee, Samik, Ironside, Daniel J., Cabral, Matthew, Sang, Xiahan, Lebeau, James, Bank, Seth R., Buonassisi, Tonio, Moutanabbir, Oussama, Lee, Minjoo Larry, Akey, Austin J
Other Authors: Massachusetts Institute of Technology. Department of Mechanical Engineering
Format: Article
Language:en_US
Published: Nature Publishing Group 2017
Online Access:http://hdl.handle.net/1721.1/110156
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author Jung, Daehwan
Faucher, Joseph
Mukherjee, Samik
Ironside, Daniel J.
Cabral, Matthew
Sang, Xiahan
Lebeau, James
Bank, Seth R.
Buonassisi, Tonio
Moutanabbir, Oussama
Lee, Minjoo Larry
Akey, Austin J
author2 Massachusetts Institute of Technology. Department of Mechanical Engineering
author_facet Massachusetts Institute of Technology. Department of Mechanical Engineering
Jung, Daehwan
Faucher, Joseph
Mukherjee, Samik
Ironside, Daniel J.
Cabral, Matthew
Sang, Xiahan
Lebeau, James
Bank, Seth R.
Buonassisi, Tonio
Moutanabbir, Oussama
Lee, Minjoo Larry
Akey, Austin J
author_sort Jung, Daehwan
collection MIT
description Self-assembled nanocomposites have been extensively investigated due to the novel properties that can emerge when multiple material phases are combined. Growth of epitaxial nanocomposites using lattice-mismatched constituents also enables strain-engineering, which can be used to further enhance material properties. Here, we report self-assembled growth of highly tensile-strained Ge/In[subscript 0.52]Al[subscript 0.48]As (InAlAs) nanocomposites by using spontaneous phase separation. Transmission electron microscopy shows a high density of single-crystalline germanium nanostructures coherently embedded in InAlAs without extended defects, and Raman spectroscopy reveals a 3.8% biaxial tensile strain in the germanium nanostructures. We also show that the strain in the germanium nanostructures can be tuned to 5.3% by altering the lattice constant of the matrix material, illustrating the versatility of epitaxial nanocomposites for strain engineering. Photoluminescence and electroluminescence results are then discussed to illustrate the potential for realizing devices based on this nanocomposite material.
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spelling mit-1721.1/1101562022-09-29T11:10:38Z Highly tensile-strained Ge/InAlAs nanocomposites Jung, Daehwan Faucher, Joseph Mukherjee, Samik Ironside, Daniel J. Cabral, Matthew Sang, Xiahan Lebeau, James Bank, Seth R. Buonassisi, Tonio Moutanabbir, Oussama Lee, Minjoo Larry Akey, Austin J Massachusetts Institute of Technology. Department of Mechanical Engineering Akey, Austin J Self-assembled nanocomposites have been extensively investigated due to the novel properties that can emerge when multiple material phases are combined. Growth of epitaxial nanocomposites using lattice-mismatched constituents also enables strain-engineering, which can be used to further enhance material properties. Here, we report self-assembled growth of highly tensile-strained Ge/In[subscript 0.52]Al[subscript 0.48]As (InAlAs) nanocomposites by using spontaneous phase separation. Transmission electron microscopy shows a high density of single-crystalline germanium nanostructures coherently embedded in InAlAs without extended defects, and Raman spectroscopy reveals a 3.8% biaxial tensile strain in the germanium nanostructures. We also show that the strain in the germanium nanostructures can be tuned to 5.3% by altering the lattice constant of the matrix material, illustrating the versatility of epitaxial nanocomposites for strain engineering. Photoluminescence and electroluminescence results are then discussed to illustrate the potential for realizing devices based on this nanocomposite material. National Science Foundation (U.S.) (DMR 1506371) 2017-06-21T20:08:52Z 2017-06-21T20:08:52Z 2017-01 2016-02 Article http://purl.org/eprint/type/JournalArticle 2041-1723 http://hdl.handle.net/1721.1/110156 Jung, Daehwan; Faucher, Joseph; Mukherjee, Samik; Akey, Austin; Ironside, Daniel J.; Cabral, Matthew and Sang, Xiahan et al. “Highly Tensile-Strained Ge/InAlAs Nanocomposites.” Nature Communications 8 (January 2017): 14204 © 2017 The Author(s) en_US http://dx.doi.org/10.1038/ncomms14204 Nature Communications Creative Commons Attribution 4.0 International License http://creativecommons.org/licenses/by/4.0/ application/pdf Nature Publishing Group Nature
spellingShingle Jung, Daehwan
Faucher, Joseph
Mukherjee, Samik
Ironside, Daniel J.
Cabral, Matthew
Sang, Xiahan
Lebeau, James
Bank, Seth R.
Buonassisi, Tonio
Moutanabbir, Oussama
Lee, Minjoo Larry
Akey, Austin J
Highly tensile-strained Ge/InAlAs nanocomposites
title Highly tensile-strained Ge/InAlAs nanocomposites
title_full Highly tensile-strained Ge/InAlAs nanocomposites
title_fullStr Highly tensile-strained Ge/InAlAs nanocomposites
title_full_unstemmed Highly tensile-strained Ge/InAlAs nanocomposites
title_short Highly tensile-strained Ge/InAlAs nanocomposites
title_sort highly tensile strained ge inalas nanocomposites
url http://hdl.handle.net/1721.1/110156
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