Helium-Ion-Implantation in Tungsten: Progress towards a Coherent Understanding of the Damage Formed and its Effects on Properties

Tungsten is a likely material for divertor armour in fusion reactors. We describe recent progress combining multi-technique experiments with atomistic modelling to understand how injected helium interacts with displacement damage and modifies the physical properties of tungsten. Using X-ray micro-di...

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Main Authors: Hofmann, F., Nguyen-Manh, D., Mason, D.R., Gilbert, M.R., Dudarev, S.L., Eliason, J.K., Beck, C.E., Liu, W., Duncan, Ryan Andrew, Maznev, Alexei, Nelson, Keith Adam
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Published: Elsevier 2018
Online Access:http://hdl.handle.net/1721.1/113411
https://orcid.org/0000-0002-8574-6033
https://orcid.org/0000-0001-7804-5418
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author Hofmann, F.
Nguyen-Manh, D.
Mason, D.R.
Gilbert, M.R.
Dudarev, S.L.
Eliason, J.K.
Beck, C.E.
Liu, W.
Duncan, Ryan Andrew
Maznev, Alexei
Nelson, Keith Adam
author2 Massachusetts Institute of Technology. Department of Chemistry
author_facet Massachusetts Institute of Technology. Department of Chemistry
Hofmann, F.
Nguyen-Manh, D.
Mason, D.R.
Gilbert, M.R.
Dudarev, S.L.
Eliason, J.K.
Beck, C.E.
Liu, W.
Duncan, Ryan Andrew
Maznev, Alexei
Nelson, Keith Adam
author_sort Hofmann, F.
collection MIT
description Tungsten is a likely material for divertor armour in fusion reactors. We describe recent progress combining multi-technique experiments with atomistic modelling to understand how injected helium interacts with displacement damage and modifies the physical properties of tungsten. Using X-ray micro-diffraction and laser-induced transient grating measurements, we observe both a lattice swelling and modulus change after helium implantation. Surprisingly, a fraction of a percent lattice expansion is associated with an order of magnitude larger reduction in elastic modulus. These observations are interpreted using a combined elasticity and density functional theory model. We also measure a large reduction of thermal diffusivity due to helium implantation. This can be explained in terms of the underlying damage microstructure using a new atomistic kinetic theory model. Together our observations and calculations allow us to begin to form a joined-up picture of helium-implantation-induced damage in tungsten and its diverse effects on microstructure and physical properties. Keywords: tungsten; ion implantation; helium laue micro-diffraction; surface acoustic waves; thermal transport
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spelling mit-1721.1/1134112022-10-02T08:07:18Z Helium-Ion-Implantation in Tungsten: Progress towards a Coherent Understanding of the Damage Formed and its Effects on Properties Hofmann, F. Nguyen-Manh, D. Mason, D.R. Gilbert, M.R. Dudarev, S.L. Eliason, J.K. Beck, C.E. Liu, W. Duncan, Ryan Andrew Maznev, Alexei Nelson, Keith Adam Massachusetts Institute of Technology. Department of Chemistry Duncan, Ryan Andrew Maznev, Alexei Nelson, Keith Adam Tungsten is a likely material for divertor armour in fusion reactors. We describe recent progress combining multi-technique experiments with atomistic modelling to understand how injected helium interacts with displacement damage and modifies the physical properties of tungsten. Using X-ray micro-diffraction and laser-induced transient grating measurements, we observe both a lattice swelling and modulus change after helium implantation. Surprisingly, a fraction of a percent lattice expansion is associated with an order of magnitude larger reduction in elastic modulus. These observations are interpreted using a combined elasticity and density functional theory model. We also measure a large reduction of thermal diffusivity due to helium implantation. This can be explained in terms of the underlying damage microstructure using a new atomistic kinetic theory model. Together our observations and calculations allow us to begin to form a joined-up picture of helium-implantation-induced damage in tungsten and its diverse effects on microstructure and physical properties. Keywords: tungsten; ion implantation; helium laue micro-diffraction; surface acoustic waves; thermal transport National Science Foundation (U.S.) (Grant CHE-1111557) 2018-02-05T15:28:02Z 2018-02-05T15:28:02Z 2017-06 2018-01-31T14:41:14Z Article http://purl.org/eprint/type/JournalArticle 2210-9838 http://hdl.handle.net/1721.1/113411 Hofmann, F. et al. “Helium-Ion-Implantation in Tungsten: Progress Towards a Coherent Understanding of the Damage Formed and Its Effects on Properties.” Procedia IUTAM 21 (June 2017): 78–85 © 2017 The Author(s) https://orcid.org/0000-0002-8574-6033 https://orcid.org/0000-0001-7804-5418 http://dx.doi.org/10.1016/J.PIUTAM.2017.03.040 Procedia IUTAM Creative Commons Attribution-NonCommercial-NoDerivs License http://creativecommons.org/licenses/by-nc-nd/4.0/ application/pdf Elsevier Elsevier
spellingShingle Hofmann, F.
Nguyen-Manh, D.
Mason, D.R.
Gilbert, M.R.
Dudarev, S.L.
Eliason, J.K.
Beck, C.E.
Liu, W.
Duncan, Ryan Andrew
Maznev, Alexei
Nelson, Keith Adam
Helium-Ion-Implantation in Tungsten: Progress towards a Coherent Understanding of the Damage Formed and its Effects on Properties
title Helium-Ion-Implantation in Tungsten: Progress towards a Coherent Understanding of the Damage Formed and its Effects on Properties
title_full Helium-Ion-Implantation in Tungsten: Progress towards a Coherent Understanding of the Damage Formed and its Effects on Properties
title_fullStr Helium-Ion-Implantation in Tungsten: Progress towards a Coherent Understanding of the Damage Formed and its Effects on Properties
title_full_unstemmed Helium-Ion-Implantation in Tungsten: Progress towards a Coherent Understanding of the Damage Formed and its Effects on Properties
title_short Helium-Ion-Implantation in Tungsten: Progress towards a Coherent Understanding of the Damage Formed and its Effects on Properties
title_sort helium ion implantation in tungsten progress towards a coherent understanding of the damage formed and its effects on properties
url http://hdl.handle.net/1721.1/113411
https://orcid.org/0000-0002-8574-6033
https://orcid.org/0000-0001-7804-5418
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