Origin of the exciton mass in the frustrated Mott insulator Na[subscript 2 ]IrO[subscript 3]
We use a three-pulse ultrafast optical spectroscopy to study the relaxation processes in a frustrated Mott insulator Na[subscript 2]IrO[subscript 3]. By being able to independently produce the out-of-equilibrium bound states (excitons) of doublons and holons with the first pulse and suppress the und...
| Main Authors: | , , , , |
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| Other Authors: | |
| Format: | Article |
| Language: | English |
| Published: |
American Physical Society
2018
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| Online Access: | http://hdl.handle.net/1721.1/114259 https://orcid.org/0000-0002-7183-5203 https://orcid.org/0000-0003-3477-6459 https://orcid.org/0000-0002-9641-3453 https://orcid.org/0000-0002-6394-4987 |
| Summary: | We use a three-pulse ultrafast optical spectroscopy to study the relaxation processes in a frustrated Mott insulator Na[subscript 2]IrO[subscript 3]. By being able to independently produce the out-of-equilibrium bound states (excitons) of doublons and holons with the first pulse and suppress the underlying antiferromagnetic order with the second one, we were able to elucidate the relaxation mechanism of quasiparticles in this system. By observing the difference in the exciton dynamics in the magnetically ordered and disordered phases we found that the mass of this quasiparticle is mostly determined by its interaction with the surrounding spins. |
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