Direct single-shot observation of millimeter-wave superradiance in Rydberg-Rydberg transitions

We have directly detected millimeter-wave (mm-wave) free-space superradiant emission from Rydberg states (principal quantum number n∼30) of barium atoms in single-shot experiments. We trigger the cooperative effects with a weak initial pulse and detect the time-dependent amplitude and phase of the e...

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Bibliographic Details
Main Authors: Zhou, Yan, Yelin, Susanne F., Grimes, David Darrah, Coy, Stephen, Barnum, Timothy James, Field, Robert W
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Language:en_US
Published: American Physical Society 2018
Online Access:http://hdl.handle.net/1721.1/115231
https://orcid.org/0000-0002-5567-7890
https://orcid.org/0000-0002-6991-683X
https://orcid.org/0000-0002-9363-9844
https://orcid.org/0000-0002-7609-4205
Description
Summary:We have directly detected millimeter-wave (mm-wave) free-space superradiant emission from Rydberg states (principal quantum number n∼30) of barium atoms in single-shot experiments. We trigger the cooperative effects with a weak initial pulse and detect the time-dependent amplitude and phase of the emitted radiation with single-shot sensitivity and 20 ps time resolution. This allows measurement and shot-by-shot analysis of the statistical distribution of decay rates, time delays, and time-dependent frequency shifts. Cooperative line shifts and decay rates are observed that exceed the 250 kHz Doppler width by a factor of 20 and the 50 Hz spontaneous emission rate by a factor of 10⁵.