Observing the Impact of Calbuco Volcanic Aerosols on South Polar Ozone Depletion in 2015

The Southern Hemisphere Antarctic stratosphere experienced two noteworthy events in 2015: a significant injection of sulfur from the Calbuco volcanic eruption in Chile in April and a record-large Antarctic ozone hole in October and November. Here we quantify Calbuco's influence on stratospheric...

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Main Authors: Kinnison, Doug E., Pitts, Michael C., Poole, Lamont R., Mills, Michael J., Schmidt, Anja, Neely, Ryan R., Schwartz, Michael J., Vernier, Jean-Paul, Johnson, Bryan J., Tully, Matthew B., Klekociuk, Andrew R., König-Langlo, Gert, Hagiya, Satoshi, Stone, Kane Adam, Solomon, Susan, Ivy, Diane J
Other Authors: Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences
Format: Article
Published: American Geophysical Union (AGU) 2018
Online Access:http://hdl.handle.net/1721.1/118616
https://orcid.org/0000-0002-2020-7581
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author Kinnison, Doug E.
Pitts, Michael C.
Poole, Lamont R.
Mills, Michael J.
Schmidt, Anja
Neely, Ryan R.
Schwartz, Michael J.
Vernier, Jean-Paul
Johnson, Bryan J.
Tully, Matthew B.
Klekociuk, Andrew R.
König-Langlo, Gert
Hagiya, Satoshi
Stone, Kane Adam
Solomon, Susan
Ivy, Diane J
author2 Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences
author_facet Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences
Kinnison, Doug E.
Pitts, Michael C.
Poole, Lamont R.
Mills, Michael J.
Schmidt, Anja
Neely, Ryan R.
Schwartz, Michael J.
Vernier, Jean-Paul
Johnson, Bryan J.
Tully, Matthew B.
Klekociuk, Andrew R.
König-Langlo, Gert
Hagiya, Satoshi
Stone, Kane Adam
Solomon, Susan
Ivy, Diane J
author_sort Kinnison, Doug E.
collection MIT
description The Southern Hemisphere Antarctic stratosphere experienced two noteworthy events in 2015: a significant injection of sulfur from the Calbuco volcanic eruption in Chile in April and a record-large Antarctic ozone hole in October and November. Here we quantify Calbuco's influence on stratospheric ozone depletion in austral spring 2015 using observations and an Earth system model. We analyze ozonesondes, as well as data from the Microwave Limb Sounder. We employ the Community Earth System Model, version 1, with the Whole Atmosphere Community Climate Model (WACCM) in a specified dynamics setup, which includes calculations of volcanic effects. The Cloud-Aerosol Lidar with Orthogonal Polarization data indicate enhanced volcanic liquid sulfate 532 nm backscatter values as far poleward as 68°S during October and November (in broad agreement with WACCM). Comparison of the location of the enhanced aerosols to ozone data supports the view that aerosols played a major role in increasing the ozone hole size, especially at pressure levels between 150 and 100 hPa. Ozonesonde vertical ozone profiles from the sites of Syowa, South Pole, and Neumayer display the lowest individual October or November measurements at 150 hPa since the 1991 Mount Pinatubo eruption period, with Davis showing similarly low values, but no available 1990 data. The analysis suggests that under the cold conditions ideal for ozone depletion, stratospheric volcanic aerosol particles from the moderate-magnitude eruption of Calbuco in 2015 greatly enhanced austral ozone depletion, particularly at 55–68°S, where liquid binary sulfate aerosols have a large influence on ozone concentrations.
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spelling mit-1721.1/1186162022-09-28T00:36:25Z Observing the Impact of Calbuco Volcanic Aerosols on South Polar Ozone Depletion in 2015 Kinnison, Doug E. Pitts, Michael C. Poole, Lamont R. Mills, Michael J. Schmidt, Anja Neely, Ryan R. Schwartz, Michael J. Vernier, Jean-Paul Johnson, Bryan J. Tully, Matthew B. Klekociuk, Andrew R. König-Langlo, Gert Hagiya, Satoshi Stone, Kane Adam Solomon, Susan Ivy, Diane J Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences Stone, Kane Adam Solomon, Susan Ivy, Diane J The Southern Hemisphere Antarctic stratosphere experienced two noteworthy events in 2015: a significant injection of sulfur from the Calbuco volcanic eruption in Chile in April and a record-large Antarctic ozone hole in October and November. Here we quantify Calbuco's influence on stratospheric ozone depletion in austral spring 2015 using observations and an Earth system model. We analyze ozonesondes, as well as data from the Microwave Limb Sounder. We employ the Community Earth System Model, version 1, with the Whole Atmosphere Community Climate Model (WACCM) in a specified dynamics setup, which includes calculations of volcanic effects. The Cloud-Aerosol Lidar with Orthogonal Polarization data indicate enhanced volcanic liquid sulfate 532 nm backscatter values as far poleward as 68°S during October and November (in broad agreement with WACCM). Comparison of the location of the enhanced aerosols to ozone data supports the view that aerosols played a major role in increasing the ozone hole size, especially at pressure levels between 150 and 100 hPa. Ozonesonde vertical ozone profiles from the sites of Syowa, South Pole, and Neumayer display the lowest individual October or November measurements at 150 hPa since the 1991 Mount Pinatubo eruption period, with Davis showing similarly low values, but no available 1990 data. The analysis suggests that under the cold conditions ideal for ozone depletion, stratospheric volcanic aerosol particles from the moderate-magnitude eruption of Calbuco in 2015 greatly enhanced austral ozone depletion, particularly at 55–68°S, where liquid binary sulfate aerosols have a large influence on ozone concentrations. 2018-10-18T18:56:19Z 2018-10-18T18:56:19Z 2017-10 2018-10-02T16:40:17Z Article http://purl.org/eprint/type/JournalArticle 2169-8996 2169-897X http://hdl.handle.net/1721.1/118616 Stone, Kane A., et al. “Observing the Impact of Calbuco Volcanic Aerosols on South Polar Ozone Depletion in 2015: Calbuco’s Impact on Antarctic Ozone Hole.” Journal of Geophysical Research: Atmospheres, vol. 122, no. 21, Nov. 2017, pp. 11,862-11,879. https://orcid.org/0000-0002-2020-7581 http://dx.doi.org/10.1002/2017JD026987 Journal of Geophysical Research: Atmospheres Creative Commons Attribution-Noncommercial-Share Alike http://creativecommons.org/licenses/by-nc-sa/4.0/ application/pdf American Geophysical Union (AGU) Other repository
spellingShingle Kinnison, Doug E.
Pitts, Michael C.
Poole, Lamont R.
Mills, Michael J.
Schmidt, Anja
Neely, Ryan R.
Schwartz, Michael J.
Vernier, Jean-Paul
Johnson, Bryan J.
Tully, Matthew B.
Klekociuk, Andrew R.
König-Langlo, Gert
Hagiya, Satoshi
Stone, Kane Adam
Solomon, Susan
Ivy, Diane J
Observing the Impact of Calbuco Volcanic Aerosols on South Polar Ozone Depletion in 2015
title Observing the Impact of Calbuco Volcanic Aerosols on South Polar Ozone Depletion in 2015
title_full Observing the Impact of Calbuco Volcanic Aerosols on South Polar Ozone Depletion in 2015
title_fullStr Observing the Impact of Calbuco Volcanic Aerosols on South Polar Ozone Depletion in 2015
title_full_unstemmed Observing the Impact of Calbuco Volcanic Aerosols on South Polar Ozone Depletion in 2015
title_short Observing the Impact of Calbuco Volcanic Aerosols on South Polar Ozone Depletion in 2015
title_sort observing the impact of calbuco volcanic aerosols on south polar ozone depletion in 2015
url http://hdl.handle.net/1721.1/118616
https://orcid.org/0000-0002-2020-7581
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