Non-diffusive relaxation of a transient thermal grating analyzed with the Boltzmann transport equation

The relaxation of an one-dimensional transient thermal grating (TTG) in a medium with phonon-mediated thermal transport is analyzed within the framework of the Boltzmann transport equation (BTE), with the goal of extracting phonon mean free path (MFP) information from TTG measurements of non-diffusi...

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Main Authors: Esfarjani, Keivan, Chen, Gang, Collins, Kimberlee C, Maznev, Alexei, Tian, Zhiting, Nelson, Keith Adam
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Published: American Institute of Physics (AIP) 2018
Online Access:http://hdl.handle.net/1721.1/118931
https://orcid.org/0000-0001-7804-5418
https://orcid.org/0000-0002-3968-8530
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author Esfarjani, Keivan
Chen, Gang
Collins, Kimberlee C
Maznev, Alexei
Tian, Zhiting
Nelson, Keith Adam
author2 Massachusetts Institute of Technology. Department of Chemistry
author_facet Massachusetts Institute of Technology. Department of Chemistry
Esfarjani, Keivan
Chen, Gang
Collins, Kimberlee C
Maznev, Alexei
Tian, Zhiting
Nelson, Keith Adam
author_sort Esfarjani, Keivan
collection MIT
description The relaxation of an one-dimensional transient thermal grating (TTG) in a medium with phonon-mediated thermal transport is analyzed within the framework of the Boltzmann transport equation (BTE), with the goal of extracting phonon mean free path (MFP) information from TTG measurements of non-diffusive phonon transport. Both gray-medium (constant MFP) and spectrally dependent MFP models are considered. In the gray-medium approximation, an analytical solution is derived. For large TTG periods compared to the MFP, the model yields an exponential decay of grating amplitude with time in agreement with Fourier's heat diffusion equation, and at shorter periods, phonon transport transitions to the ballistic regime, with the decay becoming strongly non-exponential. Spectral solutions are obtained for Si and PbSe at 300 K using phonon dispersion and lifetime data from density functional theory calculations. The spectral decay behaviors are compared to several approximate models: a single MFP solution, a frequency-integrated gray-medium model, and a "two-fluid" BTE solution. We investigate the utility of using the approximate models for the reconstruction of phonon MFP distributions from non-diffusive TTG measurements.
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spelling mit-1721.1/1189312022-09-27T15:40:21Z Non-diffusive relaxation of a transient thermal grating analyzed with the Boltzmann transport equation Esfarjani, Keivan Chen, Gang Collins, Kimberlee C Maznev, Alexei Tian, Zhiting Nelson, Keith Adam Massachusetts Institute of Technology. Department of Chemistry Massachusetts Institute of Technology. Department of Mechanical Engineering Collins, Kimberlee C Maznev, Alexei Tian, Zhiting Nelson, Keith Adam Chen, Gang The relaxation of an one-dimensional transient thermal grating (TTG) in a medium with phonon-mediated thermal transport is analyzed within the framework of the Boltzmann transport equation (BTE), with the goal of extracting phonon mean free path (MFP) information from TTG measurements of non-diffusive phonon transport. Both gray-medium (constant MFP) and spectrally dependent MFP models are considered. In the gray-medium approximation, an analytical solution is derived. For large TTG periods compared to the MFP, the model yields an exponential decay of grating amplitude with time in agreement with Fourier's heat diffusion equation, and at shorter periods, phonon transport transitions to the ballistic regime, with the decay becoming strongly non-exponential. Spectral solutions are obtained for Si and PbSe at 300 K using phonon dispersion and lifetime data from density functional theory calculations. The spectral decay behaviors are compared to several approximate models: a single MFP solution, a frequency-integrated gray-medium model, and a "two-fluid" BTE solution. We investigate the utility of using the approximate models for the reconstruction of phonon MFP distributions from non-diffusive TTG measurements. 2018-11-06T20:39:36Z 2018-11-06T20:39:36Z 2013-09 2013-06 2018-11-06T19:13:51Z Article http://purl.org/eprint/type/JournalArticle 0021-8979 1089-7550 http://hdl.handle.net/1721.1/118931 Collins, Kimberlee C. et al. “Non-Diffusive Relaxation of a Transient Thermal Grating Analyzed with the Boltzmann Transport Equation.” Journal of Applied Physics 114, 10 (September 2013): 104302 © 2013 AIP Publishing LLC https://orcid.org/0000-0001-7804-5418 https://orcid.org/0000-0002-3968-8530 http://dx.doi.org/10.1063/1.4820572 Journal of Applied Physics Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. application/pdf American Institute of Physics (AIP) Other repository
spellingShingle Esfarjani, Keivan
Chen, Gang
Collins, Kimberlee C
Maznev, Alexei
Tian, Zhiting
Nelson, Keith Adam
Non-diffusive relaxation of a transient thermal grating analyzed with the Boltzmann transport equation
title Non-diffusive relaxation of a transient thermal grating analyzed with the Boltzmann transport equation
title_full Non-diffusive relaxation of a transient thermal grating analyzed with the Boltzmann transport equation
title_fullStr Non-diffusive relaxation of a transient thermal grating analyzed with the Boltzmann transport equation
title_full_unstemmed Non-diffusive relaxation of a transient thermal grating analyzed with the Boltzmann transport equation
title_short Non-diffusive relaxation of a transient thermal grating analyzed with the Boltzmann transport equation
title_sort non diffusive relaxation of a transient thermal grating analyzed with the boltzmann transport equation
url http://hdl.handle.net/1721.1/118931
https://orcid.org/0000-0001-7804-5418
https://orcid.org/0000-0002-3968-8530
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