Ultrafast Multiharmonic Plasmon Generation by Optically Dressed Electrons

Interactions between electrons and photons are a source of rich physics from atomic to astronomical scales. Here, we examine a new kind of electron-photon interaction in which an electron, modulated by light, radiates multiple harmonics of plasmons. The emitted plasmons can be femtosecond in duratio...

Full description

Bibliographic Details
Main Authors: Wong, Liang Jie, Rivera, Nicholas H., Soljacic, Marin, Kaminer, Ido Efraim
Other Authors: Massachusetts Institute of Technology. Department of Physics
Format: Article
Language:English
Published: American Physical Society 2019
Online Access:http://hdl.handle.net/1721.1/120702
https://orcid.org/0000-0002-7184-5831
https://orcid.org/0000-0003-2691-1892
_version_ 1826209208705482752
author Wong, Liang Jie
Rivera, Nicholas H.
Soljacic, Marin
Kaminer, Ido Efraim
author2 Massachusetts Institute of Technology. Department of Physics
author_facet Massachusetts Institute of Technology. Department of Physics
Wong, Liang Jie
Rivera, Nicholas H.
Soljacic, Marin
Kaminer, Ido Efraim
author_sort Wong, Liang Jie
collection MIT
description Interactions between electrons and photons are a source of rich physics from atomic to astronomical scales. Here, we examine a new kind of electron-photon interaction in which an electron, modulated by light, radiates multiple harmonics of plasmons. The emitted plasmons can be femtosecond in duration and nanometer in spatial scale. The extreme subwavelength nature of the plasmons lowers the necessary input light intensity by at least 4 orders of magnitude relative to state-of-the-art strong-field processes involving bound or free electrons. The results presented here reveal a new means of ultrafast (10–1000 fs) interconversion between photonic and plasmonic energy, and a general scheme for generating spatiotemporally shaped ultrashort pulses in optical materials. More generally, our results suggest a route towards realizing analogues of fascinating physical phenomena like nonlinear Compton scattering in plasmonics and nanophotonics with relatively low intensities, slow electrons, and on nanometer length scales.
first_indexed 2024-09-23T14:18:53Z
format Article
id mit-1721.1/120702
institution Massachusetts Institute of Technology
language English
last_indexed 2024-09-23T14:18:53Z
publishDate 2019
publisher American Physical Society
record_format dspace
spelling mit-1721.1/1207022022-10-01T20:34:29Z Ultrafast Multiharmonic Plasmon Generation by Optically Dressed Electrons Wong, Liang Jie Rivera, Nicholas H. Soljacic, Marin Kaminer, Ido Efraim Massachusetts Institute of Technology. Department of Physics Rivera, Nicholas H. Soljacic, Marin Kaminer, Ido Efraim Interactions between electrons and photons are a source of rich physics from atomic to astronomical scales. Here, we examine a new kind of electron-photon interaction in which an electron, modulated by light, radiates multiple harmonics of plasmons. The emitted plasmons can be femtosecond in duration and nanometer in spatial scale. The extreme subwavelength nature of the plasmons lowers the necessary input light intensity by at least 4 orders of magnitude relative to state-of-the-art strong-field processes involving bound or free electrons. The results presented here reveal a new means of ultrafast (10–1000 fs) interconversion between photonic and plasmonic energy, and a general scheme for generating spatiotemporally shaped ultrashort pulses in optical materials. More generally, our results suggest a route towards realizing analogues of fascinating physical phenomena like nonlinear Compton scattering in plasmonics and nanophotonics with relatively low intensities, slow electrons, and on nanometer length scales. United States. Department of Energy (Grant DE-FG02-97ER25308) United States. Army Research Office (Contract W911NF-18-2-0048) United States. Army Research Office (Contract W911NF-13-D-0001) 2019-03-01T20:18:46Z 2019-03-01T20:18:46Z 2019-02 2018-05 2019-02-08T18:00:26Z Article http://purl.org/eprint/type/JournalArticle 0031-9007 1079-7114 http://hdl.handle.net/1721.1/120702 Rivera, Nicholas et al. "Ultrafast Multiharmonic Plasmon Generation by Optically Dressed Electrons". Physical Review Letters 122, 5 (February 2019): 053901 © 2019 American Physical Society https://orcid.org/0000-0002-7184-5831 https://orcid.org/0000-0003-2691-1892 en http://dx.doi.org/10.1103/PhysRevLett.122.053901 Physical Review Letters Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. American Physical Society application/pdf American Physical Society American Physical Society
spellingShingle Wong, Liang Jie
Rivera, Nicholas H.
Soljacic, Marin
Kaminer, Ido Efraim
Ultrafast Multiharmonic Plasmon Generation by Optically Dressed Electrons
title Ultrafast Multiharmonic Plasmon Generation by Optically Dressed Electrons
title_full Ultrafast Multiharmonic Plasmon Generation by Optically Dressed Electrons
title_fullStr Ultrafast Multiharmonic Plasmon Generation by Optically Dressed Electrons
title_full_unstemmed Ultrafast Multiharmonic Plasmon Generation by Optically Dressed Electrons
title_short Ultrafast Multiharmonic Plasmon Generation by Optically Dressed Electrons
title_sort ultrafast multiharmonic plasmon generation by optically dressed electrons
url http://hdl.handle.net/1721.1/120702
https://orcid.org/0000-0002-7184-5831
https://orcid.org/0000-0003-2691-1892
work_keys_str_mv AT wongliangjie ultrafastmultiharmonicplasmongenerationbyopticallydressedelectrons
AT riveranicholash ultrafastmultiharmonicplasmongenerationbyopticallydressedelectrons
AT soljacicmarin ultrafastmultiharmonicplasmongenerationbyopticallydressedelectrons
AT kamineridoefraim ultrafastmultiharmonicplasmongenerationbyopticallydressedelectrons