Chronology of anthropogenic impacts reconstructed from sediment records of trace metals and Pb isotopes in Todos os Santos Bay (NE Brazil)

The evolution of the impacts of anthropogenic activities in Todos os Santos Bay was evaluated by profiles of trace metals and Pb isotopes determined in sediment cores. Fluxes of metals increased up to 12, 4 and 2 times for Cu, Pb, and Zn, respectively, compared to those recorded in the beginning of...

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Main Authors: Andrade, R.L.B., Hatje, V., Masqué, P., Zurbrick, Cheryl M, Boyle, Edward A, Santos, W.P.C.
Other Authors: Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences
Format: Article
Language:en_US
Published: Elsevier BV 2020
Online Access:https://hdl.handle.net/1721.1/123813
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author Andrade, R.L.B.
Hatje, V.
Masqué, P.
Zurbrick, Cheryl M
Boyle, Edward A
Santos, W.P.C.
author2 Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences
author_facet Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences
Andrade, R.L.B.
Hatje, V.
Masqué, P.
Zurbrick, Cheryl M
Boyle, Edward A
Santos, W.P.C.
author_sort Andrade, R.L.B.
collection MIT
description The evolution of the impacts of anthropogenic activities in Todos os Santos Bay was evaluated by profiles of trace metals and Pb isotopes determined in sediment cores. Fluxes of metals increased up to 12, 4 and 2 times for Cu, Pb, and Zn, respectively, compared to those recorded in the beginning of the 20th century. Stable Pb isotopes identified a decommissioned lead smelter and burning of fossil fuels as the main sources of Pb. Most metals showed minor to moderate enrichment factors (EF < 4), but Cu and Pb were highly enriched (EF = 28 and 6, respectively) at the Aratu harbor. Temporal changes in sediments were associated to different activities, namely Pb smelting, burning of fossil fuels, maritime traffic, petroleum related activities, inputs of domestic effluents, and changes in land uses. The effects of the implementation of environmental policies to improve the waters of the bay could not be identified in the evaluated cores. Keywords: Contamination; Sediment pollution record; Trace elements; Pb isotopes; Sedimentation rates; Todos os Santos Bay
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spelling mit-1721.1/1238132022-10-01T00:12:16Z Chronology of anthropogenic impacts reconstructed from sediment records of trace metals and Pb isotopes in Todos os Santos Bay (NE Brazil) Chronology of anthropogenic impacts reconstructed from sediment records of trace metals and Pb isotopes in Todos os Santos Bay (NE Brazil) Andrade, R.L.B. Hatje, V. Masqué, P. Zurbrick, Cheryl M Boyle, Edward A Santos, W.P.C. Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences Boyle, Edward The evolution of the impacts of anthropogenic activities in Todos os Santos Bay was evaluated by profiles of trace metals and Pb isotopes determined in sediment cores. Fluxes of metals increased up to 12, 4 and 2 times for Cu, Pb, and Zn, respectively, compared to those recorded in the beginning of the 20th century. Stable Pb isotopes identified a decommissioned lead smelter and burning of fossil fuels as the main sources of Pb. Most metals showed minor to moderate enrichment factors (EF < 4), but Cu and Pb were highly enriched (EF = 28 and 6, respectively) at the Aratu harbor. Temporal changes in sediments were associated to different activities, namely Pb smelting, burning of fossil fuels, maritime traffic, petroleum related activities, inputs of domestic effluents, and changes in land uses. The effects of the implementation of environmental policies to improve the waters of the bay could not be identified in the evaluated cores. Keywords: Contamination; Sediment pollution record; Trace elements; Pb isotopes; Sedimentation rates; Todos os Santos Bay 2020-02-14T18:28:06Z 2020-02-14T18:28:06Z 2017-12 2017-06 Article http://purl.org/eprint/type/JournalArticle 0025-326X https://hdl.handle.net/1721.1/123813 Andrade, R. L. B. et al. "Chronology of anthropogenic impacts reconstructed from sediment records of trace metals and Pb isotopes in Todos os Santos Bay (NE Brazil)." Marine Pollution Bulletin 125, 1-2 (December 2017): 459-471 © 2017 Elsevier en_US https://doi.org/10.1016/j.marpolbul.2017.07.053 Marine Pollution Bulletin Creative Commons Attribution-NonCommercial-NoDerivs License http://creativecommons.org/licenses/by-nc-nd/4.0/ application/octet-stream application/pdf Elsevier BV Prof. Boyle via Chris Sherratt
spellingShingle Andrade, R.L.B.
Hatje, V.
Masqué, P.
Zurbrick, Cheryl M
Boyle, Edward A
Santos, W.P.C.
Chronology of anthropogenic impacts reconstructed from sediment records of trace metals and Pb isotopes in Todos os Santos Bay (NE Brazil)
title Chronology of anthropogenic impacts reconstructed from sediment records of trace metals and Pb isotopes in Todos os Santos Bay (NE Brazil)
title_full Chronology of anthropogenic impacts reconstructed from sediment records of trace metals and Pb isotopes in Todos os Santos Bay (NE Brazil)
title_fullStr Chronology of anthropogenic impacts reconstructed from sediment records of trace metals and Pb isotopes in Todos os Santos Bay (NE Brazil)
title_full_unstemmed Chronology of anthropogenic impacts reconstructed from sediment records of trace metals and Pb isotopes in Todos os Santos Bay (NE Brazil)
title_short Chronology of anthropogenic impacts reconstructed from sediment records of trace metals and Pb isotopes in Todos os Santos Bay (NE Brazil)
title_sort chronology of anthropogenic impacts reconstructed from sediment records of trace metals and pb isotopes in todos os santos bay ne brazil
url https://hdl.handle.net/1721.1/123813
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