Scaling and data collapse from local moments in frustrated disordered quantum spin systems

Recently measurements on various spin–1/2 quantum magnets such as H3LiIr2O6, LiZn2Mo3O8, ZnCu3(OH)6Cl2 and 1T-TaS2—all described by magnetic frustration and quenched disorder but with no other common relation—nevertheless showed apparently universal scaling features at low temperature. In particular...

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Bibliographic Details
Main Authors: Kimchi, Itamar, Sheckelton, John P., McQueen, Tyrel M., Lee, Patrick A.
Other Authors: Massachusetts Institute of Technology. Department of Physics
Format: Article
Published: Springer Nature 2020
Online Access:https://hdl.handle.net/1721.1/124809
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Summary:Recently measurements on various spin–1/2 quantum magnets such as H3LiIr2O6, LiZn2Mo3O8, ZnCu3(OH)6Cl2 and 1T-TaS2—all described by magnetic frustration and quenched disorder but with no other common relation—nevertheless showed apparently universal scaling features at low temperature. In particular the heat capacity C[H, T] in temperature T and magnetic field H exhibits T/H data collapse reminiscent of scaling near a critical point. Here we propose a theory for this scaling collapse based on an emergent random-singlet regime extended to include spin-orbit coupling and antisymmetric Dzyaloshinskii-Moriya (DM) interactions. We derive the scaling C[H, T]/T ~ H−γFq[T/H] with Fq[x] = xq at small x, with q ∈ {0, 1, 2} an integer exponent whose value depends on spatial symmetries. The agreement with experiments indicates that a fraction of spins form random valence bonds and that these are surrounded by a quantum paramagnetic phase. We also discuss distinct scaling for magnetization with a q-dependent subdominant term enforced by Maxwell’s relations. ©2018