Chemically active nanodroplets in a multi-component fluid

We introduce a model of chemically active particles of a multi-component fluid that can change their interactions with other particles depending on their state. Since such switching of interactions can only be maintained by the input of chemical energy, the system is inherently non-equilibrium. Focu...

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Main Authors: Osmanovic, Dino, Rabin, Yitzhak
Other Authors: Massachusetts Institute of Technology. Department of Physics
Format: Article
Published: Royal Society of Chemistry (RSC) 2020
Subjects:
Online Access:https://hdl.handle.net/1721.1/124875
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author Osmanovic, Dino
Rabin, Yitzhak
author2 Massachusetts Institute of Technology. Department of Physics
author_facet Massachusetts Institute of Technology. Department of Physics
Osmanovic, Dino
Rabin, Yitzhak
author_sort Osmanovic, Dino
collection MIT
description We introduce a model of chemically active particles of a multi-component fluid that can change their interactions with other particles depending on their state. Since such switching of interactions can only be maintained by the input of chemical energy, the system is inherently non-equilibrium. Focusing on a scenario where the equilibrium interactions would lead to condensation into a liquid droplet, and despite the relative simplicity of the interaction rules, these systems display a wealth of interesting and novel behaviors such as oscillations of droplet size and molecular sorting, and raise the possibility of spatio-temporal control of chemical reactions on the nanoscale. ©2019
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spelling mit-1721.1/1248752022-09-26T12:57:09Z Chemically active nanodroplets in a multi-component fluid Osmanovic, Dino Rabin, Yitzhak Massachusetts Institute of Technology. Department of Physics General Chemistry Condensed Matter Physics We introduce a model of chemically active particles of a multi-component fluid that can change their interactions with other particles depending on their state. Since such switching of interactions can only be maintained by the input of chemical energy, the system is inherently non-equilibrium. Focusing on a scenario where the equilibrium interactions would lead to condensation into a liquid droplet, and despite the relative simplicity of the interaction rules, these systems display a wealth of interesting and novel behaviors such as oscillations of droplet size and molecular sorting, and raise the possibility of spatio-temporal control of chemical reactions on the nanoscale. ©2019 2020-04-24T20:31:08Z 2020-04-24T20:31:08Z 2019-07 2019-04 Article http://purl.org/eprint/type/JournalArticle 1744-683X 1744-6848 https://hdl.handle.net/1721.1/124875 Osmanovic, Dino, and Yitzhak Rabin, "Chemically active nanodroplets in a multi-component fluid." Soft Matter 15, 29 (July 2019): no. 5965 doi 10.1039/c9sm00826h ©2019 Author(s) 10.1039/c9sm00826h Soft Matter Creative Commons Attribution 4.0 International license https://creativecommons.org/licenses/by/4.0/ application/pdf Royal Society of Chemistry (RSC) Royal Society of Chemistry (RSC)
spellingShingle General Chemistry
Condensed Matter Physics
Osmanovic, Dino
Rabin, Yitzhak
Chemically active nanodroplets in a multi-component fluid
title Chemically active nanodroplets in a multi-component fluid
title_full Chemically active nanodroplets in a multi-component fluid
title_fullStr Chemically active nanodroplets in a multi-component fluid
title_full_unstemmed Chemically active nanodroplets in a multi-component fluid
title_short Chemically active nanodroplets in a multi-component fluid
title_sort chemically active nanodroplets in a multi component fluid
topic General Chemistry
Condensed Matter Physics
url https://hdl.handle.net/1721.1/124875
work_keys_str_mv AT osmanovicdino chemicallyactivenanodropletsinamulticomponentfluid
AT rabinyitzhak chemicallyactivenanodropletsinamulticomponentfluid