State space distribution and dynamical flow for closed and open quantum systems

We present a general formalism for studying the effects of heterogeneity in open quantum systems. We develop this formalism in the state space of density operators, on which ensembles of quantum states can be conveniently represented by probability distributions. We describe how this representation...

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Main Authors: Dodin, Amro, Willard, Adam P.
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Language:English
Published: AIP Publishing 2020
Online Access:https://hdl.handle.net/1721.1/125411
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author Dodin, Amro
Willard, Adam P.
author2 Massachusetts Institute of Technology. Department of Chemistry
author_facet Massachusetts Institute of Technology. Department of Chemistry
Dodin, Amro
Willard, Adam P.
author_sort Dodin, Amro
collection MIT
description We present a general formalism for studying the effects of heterogeneity in open quantum systems. We develop this formalism in the state space of density operators, on which ensembles of quantum states can be conveniently represented by probability distributions. We describe how this representation reduces ambiguity in the definition of quantum ensembles by providing the ability to explicitly separate classical and quantum sources of probabilistic uncertainty. We then derive explicit equations of motion for state space distributions of both open and closed quantum systems and demonstrate that resulting dynamics take a fluid mechanical form analogous to a classical probability fluid on Hamiltonian phase space, thus enabling a straightforward quantum generalization of Liouville's theorem. We illustrate the utility of our formalism by analyzing the dynamics of an open two-level system using the state-space formalism that is shown to be consistent with the derived analytical results.
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spelling mit-1721.1/1254112022-09-27T21:47:56Z State space distribution and dynamical flow for closed and open quantum systems Dodin, Amro Willard, Adam P. Massachusetts Institute of Technology. Department of Chemistry We present a general formalism for studying the effects of heterogeneity in open quantum systems. We develop this formalism in the state space of density operators, on which ensembles of quantum states can be conveniently represented by probability distributions. We describe how this representation reduces ambiguity in the definition of quantum ensembles by providing the ability to explicitly separate classical and quantum sources of probabilistic uncertainty. We then derive explicit equations of motion for state space distributions of both open and closed quantum systems and demonstrate that resulting dynamics take a fluid mechanical form analogous to a classical probability fluid on Hamiltonian phase space, thus enabling a straightforward quantum generalization of Liouville's theorem. We illustrate the utility of our formalism by analyzing the dynamics of an open two-level system using the state-space formalism that is shown to be consistent with the derived analytical results. 2020-05-22T14:16:29Z 2020-05-22T14:16:29Z 2019-04 2020-01-14T15:28:45Z Article http://purl.org/eprint/type/JournalArticle 0021-9606 https://hdl.handle.net/1721.1/125411 Dodin, Amro and Adam P. Willard. “State space distribution and dynamical flow for closed and open quantum systems.” The Journal of chemical physics 15 (2019): 064106. en 10.1063/1.5100736 The Journal of chemical physics Creative Commons Attribution-Noncommercial-Share Alike http://creativecommons.org/licenses/by-nc-sa/4.0/ application/pdf AIP Publishing arXiv
spellingShingle Dodin, Amro
Willard, Adam P.
State space distribution and dynamical flow for closed and open quantum systems
title State space distribution and dynamical flow for closed and open quantum systems
title_full State space distribution and dynamical flow for closed and open quantum systems
title_fullStr State space distribution and dynamical flow for closed and open quantum systems
title_full_unstemmed State space distribution and dynamical flow for closed and open quantum systems
title_short State space distribution and dynamical flow for closed and open quantum systems
title_sort state space distribution and dynamical flow for closed and open quantum systems
url https://hdl.handle.net/1721.1/125411
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