Discontinuities in Driven Spin-Boson Systems due to Coherent Destruction of Tunneling: Breakdown of the Floquet-Gibbs Distribution

If an open quantum system is periodically driven with high frequency and the driving commutes with the system-bath coupling operator, it is known that the system approaches a Floquet-Gibbs state, a generalization of Gibbs states to periodically driven systems. Here, we investigate the stationary sta...

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Main Author: Cao, Jianshu
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Language:English
Published: American Physical Society (APS) 2020
Online Access:https://hdl.handle.net/1721.1/126056
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author Cao, Jianshu
author2 Massachusetts Institute of Technology. Department of Chemistry
author_facet Massachusetts Institute of Technology. Department of Chemistry
Cao, Jianshu
author_sort Cao, Jianshu
collection MIT
description If an open quantum system is periodically driven with high frequency and the driving commutes with the system-bath coupling operator, it is known that the system approaches a Floquet-Gibbs state, a generalization of Gibbs states to periodically driven systems. Here, we investigate the stationary state of an ac-driven system when the driving and dissipation are noncommutative. Then, the resulting stationary state does not obey the Floquet-Gibbs distribution, and the system dynamics is determined by inelastic scattering processes of the driving field. Based on the Floquet-Redfield formalism, we show that the probability distribution can exhibit population inversion and discontinuities, i.e., jumps, for parameters at which coherent destruction of tunneling takes place. These discontinuities can be observed as intensity jumps in the emission into the bath.
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spelling mit-1721.1/1260562021-09-10T19:25:50Z Discontinuities in Driven Spin-Boson Systems due to Coherent Destruction of Tunneling: Breakdown of the Floquet-Gibbs Distribution Cao, Jianshu Massachusetts Institute of Technology. Department of Chemistry If an open quantum system is periodically driven with high frequency and the driving commutes with the system-bath coupling operator, it is known that the system approaches a Floquet-Gibbs state, a generalization of Gibbs states to periodically driven systems. Here, we investigate the stationary state of an ac-driven system when the driving and dissipation are noncommutative. Then, the resulting stationary state does not obey the Floquet-Gibbs distribution, and the system dynamics is determined by inelastic scattering processes of the driving field. Based on the Floquet-Redfield formalism, we show that the probability distribution can exhibit population inversion and discontinuities, i.e., jumps, for parameters at which coherent destruction of tunneling takes place. These discontinuities can be observed as intensity jumps in the emission into the bath. National Science Foundation (U.S.) (Grant CHE 180030) National Science Foundation (U.S.) (Grant CHE 1836913) National Natural Science Foundation of China (Grant U1930402) 2020-07-07T12:23:42Z 2020-07-07T12:23:42Z 2019-09 2019-12-13T18:47:15Z Article http://purl.org/eprint/type/JournalArticle 2331-7019 https://hdl.handle.net/1721.1/126056 Engelhard, Georg, Gloria Platero and Jianshu Cao. “Discontinuities in Driven Spin-Boson Systems due to Coherent Destruction of Tunneling: Breakdown of the Floquet-Gibbs Distribution.” Physical review letters, vol. 123, 2019, 120602 © 2019 The Author(s) en 10.1103/PhysRevLett.123.120602https://dx.doi.org/ Physical review letters Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. application/octet-stream American Physical Society (APS) APS
spellingShingle Cao, Jianshu
Discontinuities in Driven Spin-Boson Systems due to Coherent Destruction of Tunneling: Breakdown of the Floquet-Gibbs Distribution
title Discontinuities in Driven Spin-Boson Systems due to Coherent Destruction of Tunneling: Breakdown of the Floquet-Gibbs Distribution
title_full Discontinuities in Driven Spin-Boson Systems due to Coherent Destruction of Tunneling: Breakdown of the Floquet-Gibbs Distribution
title_fullStr Discontinuities in Driven Spin-Boson Systems due to Coherent Destruction of Tunneling: Breakdown of the Floquet-Gibbs Distribution
title_full_unstemmed Discontinuities in Driven Spin-Boson Systems due to Coherent Destruction of Tunneling: Breakdown of the Floquet-Gibbs Distribution
title_short Discontinuities in Driven Spin-Boson Systems due to Coherent Destruction of Tunneling: Breakdown of the Floquet-Gibbs Distribution
title_sort discontinuities in driven spin boson systems due to coherent destruction of tunneling breakdown of the floquet gibbs distribution
url https://hdl.handle.net/1721.1/126056
work_keys_str_mv AT caojianshu discontinuitiesindrivenspinbosonsystemsduetocoherentdestructionoftunnelingbreakdownofthefloquetgibbsdistribution