Tellurene: A Multifunctional Material for Midinfrared Optoelectronics

The mid-infrared spectral band (2-20 μm) is of significant technological importance for thermal imaging, spectroscopic sensing, and free-space communications. Lack of optical materials compatible with common semiconductor substrates, however, presents a standing hurdle for integrated photonic device...

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Main Authors: Deckoff-Jones, Skylar, Wang, Yixiu, Lin, Hongtao, Wu, Wenzhuo, Hu, Juejun
Other Authors: Massachusetts Institute of Technology. Department of Materials Science and Engineering
Format: Article
Language:English
Published: American Chemical Society (ACS) 2020
Online Access:https://hdl.handle.net/1721.1/128112
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author Deckoff-Jones, Skylar
Wang, Yixiu
Lin, Hongtao
Wu, Wenzhuo
Hu, Juejun
author2 Massachusetts Institute of Technology. Department of Materials Science and Engineering
author_facet Massachusetts Institute of Technology. Department of Materials Science and Engineering
Deckoff-Jones, Skylar
Wang, Yixiu
Lin, Hongtao
Wu, Wenzhuo
Hu, Juejun
author_sort Deckoff-Jones, Skylar
collection MIT
description The mid-infrared spectral band (2-20 μm) is of significant technological importance for thermal imaging, spectroscopic sensing, and free-space communications. Lack of optical materials compatible with common semiconductor substrates, however, presents a standing hurdle for integrated photonic device development in the mid-infrared domain. Tellurene, atomically thin crystals of elemental tellurium, is an emerging 2-D material amenable to scalable solution-based synthesis. It uniquely combines small and tunable bandgap energies, high carrier mobility, exceptionally large electro-optic activity, and superior chemical stability, making it a promising and versatile material platform for mid-infrared photonics. With these material properties in mind, we propose and design a waveguide-integrated tellurene photodetector and Pockels effect modulator. The photodetector boasts a record room temperature noise equivalent power of 0.03 fW/Hz1/2 at 3 μm wavelength, while the optimized modulator device claims a half-wave voltage-length product (V[subscript π]L) of 2.7 V·cm and a switching energy of 12.0 pJ/bit, both representing substantial improvements to current state-of-the-art devices.
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spelling mit-1721.1/1281122022-10-01T11:04:26Z Tellurene: A Multifunctional Material for Midinfrared Optoelectronics Deckoff-Jones, Skylar Wang, Yixiu Lin, Hongtao Wu, Wenzhuo Hu, Juejun Massachusetts Institute of Technology. Department of Materials Science and Engineering The mid-infrared spectral band (2-20 μm) is of significant technological importance for thermal imaging, spectroscopic sensing, and free-space communications. Lack of optical materials compatible with common semiconductor substrates, however, presents a standing hurdle for integrated photonic device development in the mid-infrared domain. Tellurene, atomically thin crystals of elemental tellurium, is an emerging 2-D material amenable to scalable solution-based synthesis. It uniquely combines small and tunable bandgap energies, high carrier mobility, exceptionally large electro-optic activity, and superior chemical stability, making it a promising and versatile material platform for mid-infrared photonics. With these material properties in mind, we propose and design a waveguide-integrated tellurene photodetector and Pockels effect modulator. The photodetector boasts a record room temperature noise equivalent power of 0.03 fW/Hz1/2 at 3 μm wavelength, while the optimized modulator device claims a half-wave voltage-length product (V[subscript π]L) of 2.7 V·cm and a switching energy of 12.0 pJ/bit, both representing substantial improvements to current state-of-the-art devices. National Science Foundation (Awards 1453218, 1506605, 1122374) 2020-10-19T18:42:22Z 2020-10-19T18:42:22Z 2019-06 2019-05 2020-10-06T14:54:13Z Article http://purl.org/eprint/type/JournalArticle 2330-4022 https://hdl.handle.net/1721.1/128112 Deckoff-Jones, Skylar et al. "Tellurene: A Multifunctional Material for Midinfrared Optoelectronics." ACS Photonics 6, 7 (June 2019): 1632–1638 © 2019 American Chemical Society en http://dx.doi.org/10.1021/acsphotonics.9b00694 ACS Photonics Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. application/pdf American Chemical Society (ACS) Prof. Hu via Ye Li
spellingShingle Deckoff-Jones, Skylar
Wang, Yixiu
Lin, Hongtao
Wu, Wenzhuo
Hu, Juejun
Tellurene: A Multifunctional Material for Midinfrared Optoelectronics
title Tellurene: A Multifunctional Material for Midinfrared Optoelectronics
title_full Tellurene: A Multifunctional Material for Midinfrared Optoelectronics
title_fullStr Tellurene: A Multifunctional Material for Midinfrared Optoelectronics
title_full_unstemmed Tellurene: A Multifunctional Material for Midinfrared Optoelectronics
title_short Tellurene: A Multifunctional Material for Midinfrared Optoelectronics
title_sort tellurene a multifunctional material for midinfrared optoelectronics
url https://hdl.handle.net/1721.1/128112
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AT wuwenzhuo tellureneamultifunctionalmaterialformidinfraredoptoelectronics
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