High-frequency rectification via chiral Bloch electrons

Rectification is a process that converts electromagnetic fields into a direct current. Such a process underlies a wide range of technologies such as wireless communication, wireless charging, energy harvesting, and infrared detection. Existing rectifiers are mostly based on semiconductor diodes, wit...

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Main Authors: Isobe, Hiroki, Xu, Suyang, Fu, Liang
Other Authors: Massachusetts Institute of Technology. Department of Physics
Format: Article
Language:English
Published: American Association for the Advancement of Science (AAAS) 2020
Online Access:https://hdl.handle.net/1721.1/128685
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author Isobe, Hiroki
Xu, Suyang
Fu, Liang
author2 Massachusetts Institute of Technology. Department of Physics
author_facet Massachusetts Institute of Technology. Department of Physics
Isobe, Hiroki
Xu, Suyang
Fu, Liang
author_sort Isobe, Hiroki
collection MIT
description Rectification is a process that converts electromagnetic fields into a direct current. Such a process underlies a wide range of technologies such as wireless communication, wireless charging, energy harvesting, and infrared detection. Existing rectifiers are mostly based on semiconductor diodes, with limited applicability to small-voltage or high-frequency inputs. Here, we present an alternative approach to current rectification that uses the intrinsic electronic properties of quantum crystals without using semiconductor junctions. We identify a previously unknown mechanism for rectification from skew scattering due to the inherent chirality of itinerant electrons in time-reversal invariant but inversion-breaking materials. Our calculations reveal large, tunable rectification effects in graphene multilayers and transition metal dichalcogenides. Our work demonstrates the possibility of realizing high-frequency rectifiers by rational material design and quantum wave function engineering.
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spelling mit-1721.1/1286852022-09-26T14:18:55Z High-frequency rectification via chiral Bloch electrons Isobe, Hiroki Xu, Suyang Fu, Liang Massachusetts Institute of Technology. Department of Physics MIT Materials Research Laboratory Rectification is a process that converts electromagnetic fields into a direct current. Such a process underlies a wide range of technologies such as wireless communication, wireless charging, energy harvesting, and infrared detection. Existing rectifiers are mostly based on semiconductor diodes, with limited applicability to small-voltage or high-frequency inputs. Here, we present an alternative approach to current rectification that uses the intrinsic electronic properties of quantum crystals without using semiconductor junctions. We identify a previously unknown mechanism for rectification from skew scattering due to the inherent chirality of itinerant electrons in time-reversal invariant but inversion-breaking materials. Our calculations reveal large, tunable rectification effects in graphene multilayers and transition metal dichalcogenides. Our work demonstrates the possibility of realizing high-frequency rectifiers by rational material design and quantum wave function engineering. 2020-11-30T17:27:04Z 2020-11-30T17:27:04Z 2020-03 2019 2020-10-23T17:04:46Z Article http://purl.org/eprint/type/JournalArticle 2375-2548 https://hdl.handle.net/1721.1/128685 Isobe, Hiroki, Su-Yang Xu and Liang Fu. “High-frequency rectification via chiral Bloch electrons.” Science Advances, 6, 13 (March 2020): eaay2497 © 2020 The Author(s) en 10.1126/SCIADV.AAY2497 Science Advances Creative Commons Attribution NonCommercial License 4.0 https://creativecommons.org/licenses/by-nc/4.0/ application/pdf American Association for the Advancement of Science (AAAS) Science Advances
spellingShingle Isobe, Hiroki
Xu, Suyang
Fu, Liang
High-frequency rectification via chiral Bloch electrons
title High-frequency rectification via chiral Bloch electrons
title_full High-frequency rectification via chiral Bloch electrons
title_fullStr High-frequency rectification via chiral Bloch electrons
title_full_unstemmed High-frequency rectification via chiral Bloch electrons
title_short High-frequency rectification via chiral Bloch electrons
title_sort high frequency rectification via chiral bloch electrons
url https://hdl.handle.net/1721.1/128685
work_keys_str_mv AT isobehiroki highfrequencyrectificationviachiralblochelectrons
AT xusuyang highfrequencyrectificationviachiralblochelectrons
AT fuliang highfrequencyrectificationviachiralblochelectrons