Continued Emissions of the Ozone‐Depleting Substance Carbon Tetrachloride From Eastern Asia

Carbon tetrachloride (CCl4) is an ozone-depleting substance, accounting for about 10% of the chlorine in the troposphere. Under the terms of the Montreal Protocol, its production for dispersive uses was banned from 2010. In this work we show that, despite the controls on production being introduced,...

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Main Authors: Lunt, M. F., Park, S., Li, S., Henne, S., Manning, A. J., Ganesan, A. L., Simpson, I. J., Blake, D. R., Liang, Q., O'Doherty, S., Harth, C. M., Mühle, J., Salameh, P. K., Weiss, R. F., Krummel, P. B., Fraser, P. J., Prinn, Ronald G, Reimann, S., Rigby, M.
Other Authors: Massachusetts Institute of Technology. Center for Global Change Science
Format: Article
Language:English
Published: American Geophysical Union (AGU) 2021
Online Access:https://hdl.handle.net/1721.1/129458
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author Lunt, M. F.
Park, S.
Li, S.
Henne, S.
Manning, A. J.
Ganesan, A. L.
Simpson, I. J.
Blake, D. R.
Liang, Q.
O'Doherty, S.
Harth, C. M.
Mühle, J.
Salameh, P. K.
Weiss, R. F.
Krummel, P. B.
Fraser, P. J.
Prinn, Ronald G
Reimann, S.
Rigby, M.
author2 Massachusetts Institute of Technology. Center for Global Change Science
author_facet Massachusetts Institute of Technology. Center for Global Change Science
Lunt, M. F.
Park, S.
Li, S.
Henne, S.
Manning, A. J.
Ganesan, A. L.
Simpson, I. J.
Blake, D. R.
Liang, Q.
O'Doherty, S.
Harth, C. M.
Mühle, J.
Salameh, P. K.
Weiss, R. F.
Krummel, P. B.
Fraser, P. J.
Prinn, Ronald G
Reimann, S.
Rigby, M.
author_sort Lunt, M. F.
collection MIT
description Carbon tetrachloride (CCl4) is an ozone-depleting substance, accounting for about 10% of the chlorine in the troposphere. Under the terms of the Montreal Protocol, its production for dispersive uses was banned from 2010. In this work we show that, despite the controls on production being introduced, CCl4 emissions from the eastern part of China did not decline between 2009 and 2016. This finding is in contrast to a recent bottom-up estimate, which predicted a significant decrease in emissions after the introduction of production controls. We find eastern Asian emissions of CCl4 to be 16 (9–24) Gg/year on average between 2009 and 2016, with the primary source regions being in eastern China. The spatial distribution of emissions that we derive suggests that the source distribution of CCl4 in China changed during the 8-year study period, indicating a new source or sources of emissions from China's Shandong province after 2012.
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spelling mit-1721.1/1294582022-09-30T07:20:01Z Continued Emissions of the Ozone‐Depleting Substance Carbon Tetrachloride From Eastern Asia Lunt, M. F. Park, S. Li, S. Henne, S. Manning, A. J. Ganesan, A. L. Simpson, I. J. Blake, D. R. Liang, Q. O'Doherty, S. Harth, C. M. Mühle, J. Salameh, P. K. Weiss, R. F. Krummel, P. B. Fraser, P. J. Prinn, Ronald G Reimann, S. Rigby, M. Massachusetts Institute of Technology. Center for Global Change Science Massachusetts Institute of Technology. Department of Earth, Atmospheric, and Planetary Sciences Carbon tetrachloride (CCl4) is an ozone-depleting substance, accounting for about 10% of the chlorine in the troposphere. Under the terms of the Montreal Protocol, its production for dispersive uses was banned from 2010. In this work we show that, despite the controls on production being introduced, CCl4 emissions from the eastern part of China did not decline between 2009 and 2016. This finding is in contrast to a recent bottom-up estimate, which predicted a significant decrease in emissions after the introduction of production controls. We find eastern Asian emissions of CCl4 to be 16 (9–24) Gg/year on average between 2009 and 2016, with the primary source regions being in eastern China. The spatial distribution of emissions that we derive suggests that the source distribution of CCl4 in China changed during the 8-year study period, indicating a new source or sources of emissions from China's Shandong province after 2012. NASA (Grants NNX16AC98G, NNX07AE89G, NNX11AF17G) 2021-01-19T21:51:19Z 2021-01-19T21:51:19Z 2018-10 2018-09 2020-04-27T16:39:00Z Article http://purl.org/eprint/type/JournalArticle 0094-8276 1944-8007 https://hdl.handle.net/1721.1/129458 Lunt, M. F. et al. "Continued Emissions of the Ozone‐Depleting Substance Carbon Tetrachloride From Eastern Asia." Geophysical Research Letters 45, 20 (October 2018): 11,423-11,430 © 2018 The Authors en http://dx.doi.org/10.1029/2018gl079500 Geophysical Research Letters Creative Commons Attribution 4.0 International license https://creativecommons.org/licenses/by/4.0/ application/pdf American Geophysical Union (AGU) American Geophysical Union (AGU)
spellingShingle Lunt, M. F.
Park, S.
Li, S.
Henne, S.
Manning, A. J.
Ganesan, A. L.
Simpson, I. J.
Blake, D. R.
Liang, Q.
O'Doherty, S.
Harth, C. M.
Mühle, J.
Salameh, P. K.
Weiss, R. F.
Krummel, P. B.
Fraser, P. J.
Prinn, Ronald G
Reimann, S.
Rigby, M.
Continued Emissions of the Ozone‐Depleting Substance Carbon Tetrachloride From Eastern Asia
title Continued Emissions of the Ozone‐Depleting Substance Carbon Tetrachloride From Eastern Asia
title_full Continued Emissions of the Ozone‐Depleting Substance Carbon Tetrachloride From Eastern Asia
title_fullStr Continued Emissions of the Ozone‐Depleting Substance Carbon Tetrachloride From Eastern Asia
title_full_unstemmed Continued Emissions of the Ozone‐Depleting Substance Carbon Tetrachloride From Eastern Asia
title_short Continued Emissions of the Ozone‐Depleting Substance Carbon Tetrachloride From Eastern Asia
title_sort continued emissions of the ozone depleting substance carbon tetrachloride from eastern asia
url https://hdl.handle.net/1721.1/129458
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