Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor
The efficient simulation of quantum systems is a primary motivating factor for developing controllable quantum machines. For addressing systems with underlying bosonic structure, it is advantageous to utilize a naturally bosonic platform. Optical photons passing through linear networks may be config...
| Glavni autori: | , , , , , , , , , , , , |
|---|---|
| Daljnji autori: | |
| Format: | Članak |
| Jezik: | English |
| Izdano: |
American Physical Society (APS)
2021
|
| Online pristup: | https://hdl.handle.net/1721.1/129823 |
| _version_ | 1826207048486879232 |
|---|---|
| author | Wang, Christopher S. Curtis, Jacob C. Lester, Brian J. Zhang, Yaxing Gao, Yvonne Y. Freeze, Jessica Batista, Victor S. Vaccaro, Patrick H. Chuang, Isaac L. Frunzio, Luigi Jiang, Liang Girvin, S. M. Schoelkopf, Robert J. |
| author2 | Massachusetts Institute of Technology. Department of Physics |
| author_facet | Massachusetts Institute of Technology. Department of Physics Wang, Christopher S. Curtis, Jacob C. Lester, Brian J. Zhang, Yaxing Gao, Yvonne Y. Freeze, Jessica Batista, Victor S. Vaccaro, Patrick H. Chuang, Isaac L. Frunzio, Luigi Jiang, Liang Girvin, S. M. Schoelkopf, Robert J. |
| author_sort | Wang, Christopher S. |
| collection | MIT |
| description | The efficient simulation of quantum systems is a primary motivating factor for developing controllable quantum machines. For addressing systems with underlying bosonic structure, it is advantageous to utilize a naturally bosonic platform. Optical photons passing through linear networks may be configured to perform quantum simulation tasks, but the efficient preparation and detection of multiphoton quantum states of light in linear optical systems are challenging. Here, we experimentally implement a boson sampling protocol for simulating molecular vibronic spectra [J. Huh et al., Nat. Photonics 9, 615 (2015)NPAHBY1749-488510.1038/nphoton.2015.153] in a two-mode superconducting device. In addition to enacting the requisite set of Gaussian operations across both modes, we fulfill the scalability requirement by demonstrating, for the first time in any platform, a high-fidelity single-shot photon number resolving detection scheme capable of resolving up to 15 photons per mode. Furthermore, we exercise the capability of synthesizing non-Gaussian input states to simulate spectra of molecular ensembles in vibrational excited states. We show the reprogrammability of our implementation by extracting the spectra of photoelectron processes in H₂O, O₃, NO₂, and SO₂. The capabilities highlighted in this work establish the superconducting architecture as a promising platform for bosonic simulations, and by combining them with tools such as Kerr interactions and engineered dissipation, enable the simulation of a wider class of bosonic systems. |
| first_indexed | 2024-09-23T13:42:42Z |
| format | Article |
| id | mit-1721.1/129823 |
| institution | Massachusetts Institute of Technology |
| language | English |
| last_indexed | 2024-09-23T13:42:42Z |
| publishDate | 2021 |
| publisher | American Physical Society (APS) |
| record_format | dspace |
| spelling | mit-1721.1/1298232022-10-01T16:43:08Z Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor Wang, Christopher S. Curtis, Jacob C. Lester, Brian J. Zhang, Yaxing Gao, Yvonne Y. Freeze, Jessica Batista, Victor S. Vaccaro, Patrick H. Chuang, Isaac L. Frunzio, Luigi Jiang, Liang Girvin, S. M. Schoelkopf, Robert J. Massachusetts Institute of Technology. Department of Physics MIT-Harvard Center for Ultracold Atoms Massachusetts Institute of Technology. Research Laboratory of Electronics The efficient simulation of quantum systems is a primary motivating factor for developing controllable quantum machines. For addressing systems with underlying bosonic structure, it is advantageous to utilize a naturally bosonic platform. Optical photons passing through linear networks may be configured to perform quantum simulation tasks, but the efficient preparation and detection of multiphoton quantum states of light in linear optical systems are challenging. Here, we experimentally implement a boson sampling protocol for simulating molecular vibronic spectra [J. Huh et al., Nat. Photonics 9, 615 (2015)NPAHBY1749-488510.1038/nphoton.2015.153] in a two-mode superconducting device. In addition to enacting the requisite set of Gaussian operations across both modes, we fulfill the scalability requirement by demonstrating, for the first time in any platform, a high-fidelity single-shot photon number resolving detection scheme capable of resolving up to 15 photons per mode. Furthermore, we exercise the capability of synthesizing non-Gaussian input states to simulate spectra of molecular ensembles in vibrational excited states. We show the reprogrammability of our implementation by extracting the spectra of photoelectron processes in H₂O, O₃, NO₂, and SO₂. The capabilities highlighted in this work establish the superconducting architecture as a promising platform for bosonic simulations, and by combining them with tools such as Kerr interactions and engineered dissipation, enable the simulation of a wider class of bosonic systems. 2021-02-18T18:54:14Z 2021-02-18T18:54:14Z 2020-06 2020-03 2020-12-04T19:56:04Z Article http://purl.org/eprint/type/JournalArticle 2160-3308 https://hdl.handle.net/1721.1/129823 Wang, Christopher S. et al. "Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor." Physical Review X 10, 2 (June 2020): 021060 © 2020 The Authors en http://dx.doi.org/10.1103/physrevx.10.021060 Physical Review X Creative Commons Attribution 4.0 International license https://creativecommons.org/licenses/by/4.0/ application/pdf American Physical Society (APS) APS |
| spellingShingle | Wang, Christopher S. Curtis, Jacob C. Lester, Brian J. Zhang, Yaxing Gao, Yvonne Y. Freeze, Jessica Batista, Victor S. Vaccaro, Patrick H. Chuang, Isaac L. Frunzio, Luigi Jiang, Liang Girvin, S. M. Schoelkopf, Robert J. Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor |
| title | Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor |
| title_full | Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor |
| title_fullStr | Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor |
| title_full_unstemmed | Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor |
| title_short | Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor |
| title_sort | efficient multiphoton sampling of molecular vibronic spectra on a superconducting bosonic processor |
| url | https://hdl.handle.net/1721.1/129823 |
| work_keys_str_mv | AT wangchristophers efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT curtisjacobc efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT lesterbrianj efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT zhangyaxing efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT gaoyvonney efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT freezejessica efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT batistavictors efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT vaccaropatrickh efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT chuangisaacl efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT frunzioluigi efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT jiangliang efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT girvinsm efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor AT schoelkopfrobertj efficientmultiphotonsamplingofmolecularvibronicspectraonasuperconductingbosonicprocessor |