Large-Scale Characterization of Quantum Emitters in High-Purity Diamond

Solid state quantum memories, such as color centers in diamond, are a leading platform for the distribution of quantum information. Quantum repeaters will require many qubit registers at every quantum network node, each with long-lived spin states and high-quality single photon emissions. Here, we p...

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Main Author: Sutula, Madison M.
Other Authors: Englund, Dirk R.
Format: Thesis
Published: Massachusetts Institute of Technology 2022
Online Access:https://hdl.handle.net/1721.1/143261
https://orcid.org/0000-0001-9676-5611
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author Sutula, Madison M.
author2 Englund, Dirk R.
author_facet Englund, Dirk R.
Sutula, Madison M.
author_sort Sutula, Madison M.
collection MIT
description Solid state quantum memories, such as color centers in diamond, are a leading platform for the distribution of quantum information. Quantum repeaters will require many qubit registers at every quantum network node, each with long-lived spin states and high-quality single photon emissions. Here, we present techniques for large-scale characterization of color centers in diamond. We first demonstrate automated confocal microscopy and apply it to characterize silicon vacancies in diamond overgrown via chemical vapor deposition and tin vacancies in overgrown and high pressure high temperature treated diamond, yielding narrow inhomogeneous distributions of both emitters. We then demonstrate widefield photoluminescence excitation microscopy as a tool to multiplex the characterization of color center optical properties, and apply it to measure the optical properties of silicon vacancies in a sample implanted with a focused ion beam. These techniques pave the way for future large-scale characterization efforts necessary to construct quantum memory nodes.
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spelling mit-1721.1/1432612022-06-16T03:27:42Z Large-Scale Characterization of Quantum Emitters in High-Purity Diamond Sutula, Madison M. Englund, Dirk R. Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science Solid state quantum memories, such as color centers in diamond, are a leading platform for the distribution of quantum information. Quantum repeaters will require many qubit registers at every quantum network node, each with long-lived spin states and high-quality single photon emissions. Here, we present techniques for large-scale characterization of color centers in diamond. We first demonstrate automated confocal microscopy and apply it to characterize silicon vacancies in diamond overgrown via chemical vapor deposition and tin vacancies in overgrown and high pressure high temperature treated diamond, yielding narrow inhomogeneous distributions of both emitters. We then demonstrate widefield photoluminescence excitation microscopy as a tool to multiplex the characterization of color center optical properties, and apply it to measure the optical properties of silicon vacancies in a sample implanted with a focused ion beam. These techniques pave the way for future large-scale characterization efforts necessary to construct quantum memory nodes. S.M. 2022-06-15T13:07:59Z 2022-06-15T13:07:59Z 2022-02 2022-03-04T20:59:50.370Z Thesis https://hdl.handle.net/1721.1/143261 https://orcid.org/0000-0001-9676-5611 In Copyright - Educational Use Permitted Copyright MIT http://rightsstatements.org/page/InC-EDU/1.0/ application/pdf Massachusetts Institute of Technology
spellingShingle Sutula, Madison M.
Large-Scale Characterization of Quantum Emitters in High-Purity Diamond
title Large-Scale Characterization of Quantum Emitters in High-Purity Diamond
title_full Large-Scale Characterization of Quantum Emitters in High-Purity Diamond
title_fullStr Large-Scale Characterization of Quantum Emitters in High-Purity Diamond
title_full_unstemmed Large-Scale Characterization of Quantum Emitters in High-Purity Diamond
title_short Large-Scale Characterization of Quantum Emitters in High-Purity Diamond
title_sort large scale characterization of quantum emitters in high purity diamond
url https://hdl.handle.net/1721.1/143261
https://orcid.org/0000-0001-9676-5611
work_keys_str_mv AT sutulamadisonm largescalecharacterizationofquantumemittersinhighpuritydiamond